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The nonlinear process of second harmonic generation (SHG) in monolayer (1L) transition metal dichalcogenides (TMD), like $WS_2$, strongly depends on the polarization state of the excitation light. Combining plasmonic nanostructures with…

Optics · Physics 2021-10-08 Florian Spreyer , Claudia Ruppert , Philip Georgi , Thomas Zentgraf

We analyze second-harmonic generation (SHG) at a thin effectively quadratic nonlinear interface between two linear optical media. We predict multistability of SHG for both plane and localized waves, and also describe two-color localized…

patt-sol · Physics 2007-05-23 Andrey A. Sukhorukov , Yuri S. Kivshar , Ole Bang

We show that second harmonic generation can be enhanced by Fano resonant coupling of asymmetric plasmonic metal nanostructures. We develop a theoretical model examining the effects of electromagnetic interaction between two metal…

Second harmonic generation (SHG) is a powerful optical tool for identifying non-centrosymmetric crystalline structures. Here, we analyze SHG in multilayer graphenes (MLG), with a focus on its dependence on the stacking order, encapsulation…

Mesoscale and Nanoscale Physics · Physics 2026-03-25 Patrick Johansen Sarsfield , Takaaki V. Joya , Takuto Kawakami , Mikito Koshino , Vladimir Fal'ko

Nonlinear second harmonic optical activity of graphene covering a gold photon sieve was determined for different polarizations. The photon sieve consists of a subwavelength gold nanohole array placed on glass. It combines the benefits of…

Mesoscale and Nanoscale Physics · Physics 2016-01-14 Michael Lobet , Michael Sarrazin , Francesca Cecchet , Nicolas Reckinger , Alexandru Vlad , Jean-François Colomer , Dan Lis

A comparative experimental investigation of the dependence of second harmonic generation (SHG) on applied external voltage between the standard nematic liquid crystalline material and an analogue ferromagnetic nematic liquid crystalline…

Soft Condensed Matter · Physics 2019-09-30 Jure Brence , Luka Cmok , Nerea Sebastian , Alenka Mertelj , Darja Lisjak , Irena Drevensek-Olenik

Second harmonic generation (SHG) is a nonlinear optical response arising exclusively from broken inversion symmetry in the electric-dipole limit. Recently, SHG has attracted widespread interest as a versatile and noninvasive tool for…

The surface sensitivity and probe depth in the x-ray regime of diamond for second harmonic generation (SHG) was investigated both analytically and computationally with velocity gauge real-time time-dependent density functional theory…

Materials Science · Physics 2026-04-22 Daniel Schacher , Tod A. Pascal , Keith V. Lawler , Craig P. Schwartz

We theoretically predict efficient optical second-harmonic generation (SHG) from a few hundred nanometer thick slab consisting of a quadratic nonlinear anisotropic medium whose linear principal permittivities are, at the fundamental…

Optics · Physics 2011-03-16 Alessandro Ciattoni

The interface between two different semiconductors is crucial in determining the electronic properties at the heterojunction, therefore novel techniques that can probe these regions are of particular interest. Recently it has been shown…

Mesoscale and Nanoscale Physics · Physics 2021-09-01 Frederico B. Sousa , Lucas Lafeta , Alisson R. Cadore , Prasana K. Sahoo , Leandro M. Malard

The optimization of nonlinear optical processes at the nanoscale is a crucial step for the development of nanoscale photon sources for quantum-optical networks. The development of innovative plasmonic nanoantenna designs and hybrid…

The generation process of second harmonic (SH) radiation from holes periodically arranged on a metal surface is investigated. Three main modulating factors affecting the optical response are identified: the near-field distribution at the…

Mesoscale and Nanoscale Physics · Physics 2015-01-08 Sergio G. Rodrigo , V. Laliena , L. Martín-Moreno

It is generally argued that material classes with inversion symmetry do not produce bulk dipole related second harmonic generation (SHG). So, SHG is then either ascribed to surface effects or bulk related electric quadrupole or magnetic…

Surfaces and interfaces of magnetic nanostructures can reveal rather interesting and unusual properties that differ substantially from those of bulky materials. Here we apply the surface-sensitive method of optical second harmonic…

Mesoscale and Nanoscale Physics · Physics 2018-12-13 T. V. Murzina , K. A. Lazareva , E. E. Shalygina , I. A. Kolmychek , E. A. Karashtin , N. S. Gusev , A. A. Fraerman

We report on theoretical study of second-harmonic generation (SHG) in plasmonic nanostructures interacting with two-level quantum emitters (QE) under incoherent energy pump. We generalize driven-dissipative Tavis-Cummings model by…

Optics · Physics 2021-03-17 Maxim Sukharev , Oleksiy Roslyak , Andrei Piryatinski

Second harmonic generation (SHG) is prohibited in centrosymmetric crystals such as silicon or germanium due to the presence of inversion symmetry. However, the structuring of such materials makes it possible to break the inversion symmetry,…

We investigate Second Harmonic Generation from individual silicon nanowires and study the influence of resonant optical modes on the far-field nonlinear emission. We find that the polarization of the Second Harmonic has a size-dependent…

Mesoscale and Nanoscale Physics · Physics 2016-03-18 Peter R. Wiecha , Arnaud Arbouet , Christian Girard , Thierry Baron , Vincent Paillard

We conduct a theoretical and numerical study on the second-harmonic (SH) optical response of a nano-structured metamaterial composed of a periodic array of inclusions. Both the inclusions and their surrounding matrix are made of…

Mesoscale and Nanoscale Physics · Physics 2019-03-13 Ulises R. Meza , Bernardo S. Mendoza , W. Luis Mochán

We derive an expression for the effective second-harmonic coefficient of a dilute suspension of coated spherical particles. It is assumed that the coating material, but not the core or the host, has a nonlinear susceptibility for…

Disordered Systems and Neural Networks · Physics 2009-11-10 P. M. Hui , C. Xu , D. Stroud

Second harmonic (SH) radiation in metal nanoparticles is generated by both nonlocal-bulk and local-surface SH sources, induced by the electromagnetic field at the fundamental frequency. We propose a surface integral equation (SIE) method…

Optics · Physics 2014-01-21 Carlo Forestiere , Antonio Capretti , Giovanni Miano