Related papers: Theory of Quantum-Enhanced Stimulated Raman Scatte…
The range of stimulated Raman scattering (SRS) frequencies covers a domain which at the low end abuts half the laser frequency, omega_0 / 2, according to the simplest SRS theories, corresponding to scatter from electron densities near 1/4…
Stimulated Raman scattering (SRS) in its strongly nonlinear, kinetic regime is controlled by a technique of deterministic, strong temporal modulation and spatial scrambling of laser speckle patterns, called Spike Trains of Uneven Duration…
Raman spectroscopy reveals chemically specific information and provides label-free insight into the molecular world. However, the signals are intrinsically weak and call for enhancement techniques. Here, we demonstrate Purcell enhancement…
Quantum physics has brought enhanced capability in various sensing applications. Despite challenges from noise and loss in the radio-frequency (RF) domain, [Phys. Rev. Lett. 124, 150502 (2020)] demonstrates a route for enhanced RF-receiver…
Label-free optical microscopy through absorption or scattering spectroscopy provides fundamental insights across biology and materials science, yet its sensitivity remains fundamentally limited by photon shot noise. While recent…
We present a three-dimensional theory of stimulated Raman scattering (SRS) or superradiance. In particular we address how the spatial and temporal properties of the generated SRS beam, or Stokes beam, of radiation depends on the spatial…
The principles of quantum optics have yielded a plethora of ideas to surpass the classical limitations of sensitivity and resolution in optical microscopy. While some ideas have been applied in proof-of-principle experiments, imaging a…
The Raman scattering of light by molecular vibrations offers a powerful technique to 'fingerprint' molecules via their internal bonds and symmetries. Since Raman scattering is weak, methods to enhance, direct and harness it are highly…
This paper presents a study on quantum radar technology developments, design Consideration for its integration, and quantum radar cross-section, QRCS based on quantum electrodynamics and interferometric considerations. Quantum radar systems…
The inelastic scatterings of matter systems, such as Raman scattering, contain rich information on mechanical vibrations like as resonant frequencies, which lead to various applications, for example, a sensor for specific molecules.…
Today's cutting-edge optical spectroscopic exploratory tools, such as Raman or infrared spectroscopy, rely on methods of signal enhancement as a route for their development. These methods are indispensable for substance identification and…
Quantitative Magnetic Resonance Imaging (qMRI) provides researchers insight into pathological and physiological alterations of living tissue, with the help of which researchers hope to predict (local) therapeutic efficacy early and…
Spontaneous Raman spectroscopy (SRS) is a conventional in-situ laser diagnostic method that has been widely used for measurements of temperature and major species. However, SRS in sooting flames suffers from strong interference including…
Quantum-optical spectrometry is a recently developed shot-to-shot photon correlation-based method, namely using a quantum spectrometer (QS), that has been used to reveal the quantum optical nature of intense laser-matter interactions and…
Absorption measurement is an exceptionally versatile tool for many applications in science and engineering. For absorption measurements using laser beams of light, the sensitivity is theoretically limited by the shot noise due to the…
The reliable characterization of quantum states is a fundamental task in quantum information science. For this purpose, quantum state tomography provides a standard framework for reconstructing quantum states from measurement data, yet it…
Raman spectroscopy enables non-destructive, label-free molecular analysis with high specificity, making it a powerful tool for biomedical diagnostics. However, its application to biological tissues is challenged by inherently weak Raman…
We present a method for deriving limits on Raman scattering in structured media and exploit it to constrain the maximum Raman signal resulting from a planewave incident on either a single Raman molecule in the vicinity of a structured…
We present an in-depth analysis of the experimental estimation of cross sections in Surface Enhanced Raman Scattering (SERS) by vibrational pumping. The paper highlights the advantages and disadvantages of the technique, pinpoints the main…
Nanofibers functionalized by metal nanostructures and particles are exploited as effective flexible substrates for SERS analysis. Their complex three-dimensional structure may provide Raman signals enhanced by orders of magnitude compared…