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It is well-known from numerical and experimental results that the fraction of Rydberg states (excited neutral atoms) created by tunnel ionization declines dramatically with increasing ellipticity of laser light. We present a method to…

The dynamics of autoionizing Rydberg states of oxygen are studied using attosecond transient absorption technique, where extreme ultraviolet (XUV) initiates molecular polarization and near infrared (NIR) pulse perturbs its evolution.…

We report on the measurement of electron emission after the interaction of strong laser pulses with atoms and molecules. These electrons originate from high-lying Rydberg states with quantum numbers up to $n \lesssim 120$ formed by…

The yield of neutral excited atoms and low-energy photoelectrons generated by the electron dynamics in the combined Coulomb and laser field after tunneling is investigated. We present results of Monte-Carlo simulations built on the two-step…

Atomic Physics · Physics 2015-05-13 N. I. Shvetsov-Shilovski , S. P. Goreslavski , S. V. Popruzhenko , W. Becker

We extend a recently developed three-dimensional semiclassical model [\href{https://journals.aps.org/pra/abstract/10.1103/PhysRevA.109.033106}{Phys. Rev. \textbf{A} 109, 033106 (2024)}] to study multielectron ionization and the formation of…

Atomic Physics · Physics 2026-02-17 Georgios Petros Katsoulis , Agapi Emmanouilidou

High Harmonic Generation (HHG) creates coherent high frequency radiation via the process of strong field ionization followed by recombination. Recently, a complementary approach based on Frustrated Tunnel Ionization (FTI) was demonstrated…

Atomic Physics · Physics 2022-04-15 L. Ortmann , C. Hofmann , I. A. Ivanov , A. S. Landsman

We formulate a three-dimensional semi-classical model to treat three-electron escape dynamics in a strongly-driven linear triatomic molecule, HeH$_{2}^{+}$. Our model includes the Coulomb singularities. Hence, to avoid unphysical…

Atomic Physics · Physics 2021-04-21 M. B. Peters , V. P. Majety , A. Emmanouilidou

We introduce a scheme to entangle Rydberg ions in a linear ion crystal, using the high electric polarizability of the Rydberg electronic states in combination with mutual Coulomb coupling of ions that establishes common modes of motion.…

Atomic Physics · Physics 2019-10-16 Jonas Vogel , Weibin Li , Arezoo Mokhberi , Igor Lesanovsky , Ferdinand Schmidt-Kaler

We demonstrate sub-cycle control of frustrated double ionization (FDI) in the two-electron triatomic molecule D$_3^+$ when driven by two orthogonally polarized two-color laser fields. We employ a three-dimensional semi-classical model that…

Atomic Physics · Physics 2018-05-22 A. Vilà , G. P. Katsoulis , A. Emmanouilidou

Precise control of the electron phase accumulated during its sub-cycle motion within intense laser fields is essential in strong-field physics, yet remains mostly indirect and complicated so far. In this Letter, we develop a novel approach…

Penning ionization releases electrons in a state-selected Rydberg gas of nitric oxide entrained in a supersonic molecular beam. Subsequent processes of electron impact avalanche, bifurcation, and quench form a strongly coupled, spatially…

Atomic Physics · Physics 2021-01-05 R. Wang , M. Aghigh , K. L. Marroquín , K. M. Grant , J. Sous , F. B. V. Martins , J. S. Keller , E. R. Grant

We study a model for frustrated tunneling ionization using ultrashort laser pulses. The model is based on the strong field approximation and it employs the saddle point approximation to predict quasiclassical trajectories that are captured…

Quantum Physics · Physics 2021-09-22 Edvin Olofsson , Stefanos Carlström , Jan Marcus Dahlström

We demonstrate the control of electron-electron correlation in frustrated double ionization (FDI) of the two-electron triatomic molecule D$_{3}^{+}$ when driven by two orthogonally polarized two-color laser fields. We employ a…

Atomic Physics · Physics 2017-09-13 A. Chen , M. F. Kling , A. Emmanouilidou

High-harmonic generation is typically thought of as a sub-laser-cycle process, with the electron's excursion in the continuum lasting a fraction of the optical cycle. However, it was recently suggested that long-lived Rydberg states can…

We investigate the dynamics of electron-electron recollisions in the double ionization of atoms in strong laser fields. The statistics of recollisions can be reformulated in terms of an area-preserving map from the observation that the…

Atomic Physics · Physics 2010-06-30 Francois Mauger , Cristel Chandre , Turgay Uzer

Population dynamics in weakly-excited clouds of ultracold $^{87}$Rb Rydberg atoms were studied by means of trap loss, fluorescence detection, and state dependent stimulated emission. Rydberg atoms were excited to various nl Rydberg states…

Quantum Physics · Physics 2009-11-13 J. O. Day , E. Brekke , T. G. Walker

Using ab-initio non-Born-Oppenheimer simulations, we demonstrate amplification of XUV radiation in a high-harmonic generation type process using the example of the hydrogen molecular ion. A small fraction of the molecules is pumped to a…

Atomic Physics · Physics 2016-03-23 Timm Bredtmann , Szczepan Chelkowski , Andre. D. Bandrauk , Misha Ivanov

We consider the dynamics of electrons in combined strong laser and Coulomb fields. Under a timescale separation condition, we reduce this dynamics to a guiding-center framework. More precisely, we derive a hierarchy of models for the…

Chaotic Dynamics · Physics 2018-11-28 Jonathan Dubois , S. Berman , C. Chandre , T. Uzer

We studied alignment-to-orientation conversion caused by excited-state level crossings in a nonzero magnetic field of both atomic rubidium isotopes. Experimental measurements were performed on the transitions of the $D_2$ line of rubidium.…

Atomic Physics · Physics 2015-05-27 M. Auzinsh , A. Berzins , R. Ferber , F. Gahbauer , L. Kalvans , A. Mozers , A. Spiss

We report on the observation of interactions between ultracold Rydberg atoms and ions in a Paul trap. The rate of observed inelastic collisions, which manifest themselves as charge transfer between the Rydberg atoms and ions, exceeds that…

Atomic Physics · Physics 2019-07-03 N. V. Ewald , T. Feldker , H. Hirzler , H. Fürst , R. Gerritsma
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