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A new methodology of simulating nonadiabatic dynamics using frozen-width Gaussian wavepackets within the moving crude adiabatic representation with the on-the-fly evaluation of electronic structure is presented. The main feature of the new…

Chemical Physics · Physics 2018-04-04 Loïc Joubert-Doriol , Artur F. Izmaylov

Quantum molecular dynamics requires an accurate representation of the molecular potential energy surface from a minimal number of electronic structure calculations, particularly for nonadiabatic dynamics where excited states are required.…

Chemical Physics · Physics 2016-08-24 Charles W. Heaps , David A. Mazziotti

Bosonic quantum devices offer a novel approach to realize quantum computations, where the quantum two-level system (qubit) is replaced with the quantum (an)harmonic oscillator (qumode) as the fundamental building block of the quantum…

Current simulations of ultraviolet-visible absorption lineshapes, and dynamics of condensed phase systems, largely adopt a harmonic description to model vibrations. Often, this involves a model of displaced harmonic oscillators that have…

Chemical Physics · Physics 2020-01-08 Luke D. Smith , Arend G. Dijkstra

Modeling open quantum dynamics without full knowledge of the system Hamiltonian or noise model is a key challenge in quantum control and quantum state estimation. We introduce an Augmented Quantum Neural Ordinary Differential Equation…

Quantum Physics · Physics 2025-09-10 Shahid Qamar , Rana Imran Mushtaq , Bo Li , Ho-Kin Tang

The quantum geometric tensor has established itself as a general framework for the analysis and detection of equilibrium phase transitions in isolated quantum systems. We propose a novel generalization of the quantum geometric tensor, which…

Quantum Physics · Physics 2025-02-27 Pavel Orlov , Georgy V. Shlyapnikov , Denis V. Kurlov

We discuss monitoring the time evolution of an analog quantum simulator via a quantum non-demolition (QND) coupling to an auxiliary `clock' qubit. The QND variable of interest is the `energy' of the quantum many-body system, represented by…

Quantum Physics · Physics 2020-10-14 Denis V. Vasilyev , Andrey Grankin , Mikhail A. Baranov , Lukas M. Sieberer , Peter Zoller

Anharmonic potential quantum system play crucial role in physics as they provide a more realistic description of oscillatory phenomena, which often deviate from the idealized harmonic model. However, simulating such system on classical…

Quantum Physics · Physics 2025-10-08 Saurav Suman , Bikash K. Behera , Vivek Vyas , Prasanta k. Panigrahi

The simulation of out-of-equilibrium dissipative quantum many body systems is a problem of fundamental interest to a number of fields in physics, ranging from condensed matter to cosmology. For unitary systems, tensor network methods have…

Quantum Physics · Physics 2019-10-30 Edward Gillman , Federico Carollo , Igor Lesanovsky

A numerical method is proposed for simulation of composite open quantum systems. It is based on Lindblad master equations and adiabatic elimination. Each subsystem is assumed to converge exponentially towards a stationary subspace, slightly…

Quantum Physics · Physics 2023-11-10 François-Marie Le Régent , Pierre Rouchon

We find that feedback control may induce "pseudo" nonlinear dynamics in a damped harmonic oscillator, whose centroid trajectory in the phase space behaves like a classical nonlinear system. Thus, similar to nonlinear amplifiers (e.g.,…

Quantum Physics · Physics 2015-05-14 Jing Zhang , Yu-xi Liu , Re-Bing Wu , Chun-Wen Li , Tzyh-Jong Tarn

Accurate description of nonadiabatic dynamics of molecules at metal surfaces involving electron transfer has been a longstanding challenge for theory. Here, we tackle this problem by first constructing high-dimensional neural network…

Materials Science · Physics 2024-01-05 Gang Meng , James Gardner , Wenjie Dou , Reinhard J. Maurer , Bin Jiang

Controllable adiabatic evolution of a multi-qubit system can be used for adiabatic quantum computation (AQC). This evolution ends at a configuration where the Hamiltonian of the system encodes the solution of the problem to be solved. As a…

Digital quantum simulation uses the capabilities of quantum computers to determine the dynamics of quantum systems, which are beyond the computability of modern classical computers. A notoriously challenging task in this field is the…

Quantum Physics · Physics 2021-04-19 Benedikt Fauseweh , Jian-Xin Zhu

We experimentally perform the simulation of open quantum dynamics in single-qudit systems. Using a spatial light modulator as a dissipative optical device, we implement dissipative-dynamical maps onto qudits encoded in the transverse…

Quantum Physics · Physics 2015-11-10 B. Marques , A. A. Matoso , W. M. Pimenta , A. J. Gutiérrez-Esparza , M. F. Santos , S. Pádua

The recent advancement of quantum computer hardware offers the potential to simulate quantum many-body systems beyond the capability of its classical counterparts. However, most current works focus on simulating the ground-state properties…

Quantum Physics · Physics 2022-06-14 Chee Kong Lee , Shi-Xin Zhang , Chang-Yu Hsieh , Shengyu Zhang , Liang Shi

We quantitatively analyze the dynamics of the quantum phase distribution associated with the reduced density matrix of a system, as the system evolves under the influence of its environment with an energy-preserving quantum nondemolition…

Quantum Physics · Physics 2009-11-13 Subhashish Banerjee , Joyee Ghosh , R. Ghosh

We present a new formulation of the correlated electron-ion dynamics (CEID) scheme, which systematically improves Ehrenfest dynamics by including quantum fluctuations around the mean-field atomic trajectories. We show that the method can…

Materials Science · Physics 2007-12-13 L. Stella , M. Meister , A. J. Fisher , A. P. Horsfield

We investigate a resonantly modulated harmonic mode, dispersively coupled to a nonequilibrium few-level quantum system. We focus on the regime where the relaxation rate of the system greatly exceeds that of the mode, and develop a quantum…

Mesoscale and Nanoscale Physics · Physics 2015-06-18 Z. Maizelis , M. Rudner , M. I. Dykman

Electron transfer is an important and fundamental process in chemistry, biology and physics, and has received significant attention in recent years. Perhaps one of the most intriguing questions concerns with the realization of the…

Mesoscale and Nanoscale Physics · Physics 2023-05-30 Bokang Hou , Michael Thoss , Uri Banin , Eran Rabani