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In time-resolved photoemission experiments, more than one electron can be emitted from the solid by a single ultra-short pulse. We theoretically demonstrate how correlations between the momenta of outgoing electrons relate to time-dependent…

Strongly Correlated Electrons · Physics 2019-06-26 Christopher Stahl , Martin Eckstein

Extracting information from stochastic fields or textures is a ubiquitous task in science, from exploratory data analysis to classification and parameter estimation. From physics to biology, it tends to be done either through a power…

Instrumentation and Methods for Astrophysics · Physics 2021-12-03 Sihao Cheng , Brice Ménard

We numerically investigate nucleation processes in the transient dynamics of the two-dimensional complex Ginzburg-Landau equation towards its "frozen" state with quasi-stationary spiral structures. We study the transition kinetics from…

Statistical Mechanics · Physics 2019-11-27 Weigang Liu , Uwe C. Täuber

We experimentally demonstrate spatiotemporal steering of photoelectron emission in multiphoton above-threshold single ionization of atoms exposed to a phase-controlled orthogonally polarized two-color (OTC) laser pulse. Spatial and energy…

Light-induced molecular dynamics often involve the excitation of several electronic, vibrational, and rotational states. Since the ensuing electronic and nuclear motion determines the pathways and outcomes of photoinduced reactions, our…

Layered transition metal dichalcogenides (TMDs) offer many attractive features for next-generation low-dimensional device geometries. Due to the practical and fabrication challenges related to in situ methods, the atomistic dynamics that…

This chapter gives an introduction to qualitative and quantitative topological analyses of molecular electronic transitions. Among the possibilities for qualitatively describing how the electronic structure of a molecule is reorganized upon…

Chemical Physics · Physics 2018-11-27 Thibaud Etienne

Sub-laser cycle time scale of electronic response to strong laser fields enables attosecond dynamical imaging in atoms, molecules and solids. Optical tunneling and high harmonic generation are the hallmarks of attosecond imaging in optical…

Optics · Physics 2019-10-22 R. E. F. Silva , Á. Jiménez-Galán , B. Amorim , O. Smirnova , M. Ivanov

Excitons -- two-particle correlated electron-hole pairs -- are the dominant low-energy optical excitation in the broad class of semiconductor materials, which range from classical silicon to perovskites, and from two-dimensional to organic…

Materials Science · Physics 2025-11-25 Marcel Reutzel , G. S. Matthijs Jansen , Stefan Mathias

Giant strides in ultrashort laser pulse technology have enabled real-time observation of dynamical processes in complex molecular systems. Specifically, the discovery of oscillatory transients in the two-dimensional electronic spectra of…

Chemical Physics · Physics 2021-03-08 Akihito Ishizaki , Graham R. Fleming

Electronic coherences are key to understanding and controlling photo-induced molecular transformations. We identify a crucial quantum-mechanical feature of electron-nuclear correlation, the projected nuclear quantum momenta, essential to…

Chemical Physics · Physics 2024-11-13 Evaristo Villaseco Arribas , Neepa T. Maitra

The dipole moment is a crucial molecular property linked to a molecular system's bond polarity and overall electronic structure. To that end, the electronic dipole moment, which results from the electron density of a system, is often used…

The evolution of both information and energy technology is intimately connected to complex condensed matter systems, the properties of which are determined by electronic and chemical interactions and processes on a broad range of length and…

Materials Science · Physics 2015-03-19 Martina Müller , Slavomir Nemsak , Lukasz Plucinski , Claus M. Schneider

Electrostriction, the deformation of dielectric materials under the influence of an electric field, is of continuous interest in optics. The classic experiment by Hakim and Higham [Proc. Phys. Soc. 80, 190 (1962)] for a stationary field…

We report the site-specific probing of charge-transfer dynamics in a prototype system for organic photovoltaics (OPV) by picosecond time-resolved X-ray photoelectron spectroscopy. A layered system consisting of approximately two monolayers…

Natural optical activity is the paradigmatic example of an effect originating in the weak spatial inhomogeneity of the electromagnetic field on the atomic scale. In molecules, such effects are well described by the multipole theory of…

Materials Science · Physics 2023-05-31 Óscar Pozo , Ivo Souza

Spectropolarimetric inversions are routinely used in the field of Solar Physics for the extraction of physical information from observations. The application to two-dimensional fields of view often requires the use of supercomputers with…

Solar and Stellar Astrophysics · Physics 2019-06-26 A. Asensio Ramos , C. Diaz Baso

We investigate the effect of nuclear spins on the phase shift and polarisation rotation of photons scattered off a quantum dot-cavity system. We show that as the phase shift depends strongly on the resonance energy of an electronic…

Quantum Physics · Physics 2019-06-05 Thomas Nutz , Petros Androvitsaneas , Andrew Young , Ruth Oulton , Dara P. S. McCutcheon

Quantum material systems upon applying ultrashort laser pulses provide a rich platform to access excited material phases and their transformations that are not entirely like their equilibrium counterparts. The addressability and potential…

Strongly Correlated Electrons · Physics 2021-08-19 Xiaoyi Sun , Shuaishuai Sun , Chong-Yu Ruan

The spectra (rotational, rotation-vibrational or electronic) of diatomic molecules due to transitions involving only closed-shell ($^1\Sigma$) electronic states follow very regular, simple patterns and their theoretical analysis is usually…

Chemical Physics · Physics 2016-05-10 Jonathan Tennyson , Lorenzo Lodi , Laura K. McKemmish , Sergei N Yurchenko