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A thorough in situ characterization of materials at extreme conditions is challenging, and computational tools such as crystal structural search methods in combination with ab initio calculations are widely used to guide experiments by…

Materials Science · Physics 2018-11-14 Maximilian Amsler , Vinay I. Hegde , Steven D. Jacobsen , Chris Wolverton

Photocatalytic water splitting has emerged as a sustainable pathway for hydrogen production, leveraging sunlight to drive chemical reactions. This review explores the integration of density functional theory (DFT) with machine learning (ML)…

Computational Physics · Physics 2025-12-30 Dennis Delali Kwesi Wayo , Leonardo Goliatt , Darvish Ganji

Quantitative predictions of the release of volatile radiocontaminants of ruthenium (Ru) in the environment from either nuclear power plants (NPP) or fuel recycling accidents present significant uncertainties while estimated by severe…

Chemical Physics · Physics 2021-11-23 Faoulat Miradji , Sidi M. O. Souvi , Laurent Cantrel , Florent Louis , Valérie Vallet

We present a scale-bridging approach based on a multi-fidelity (MF) machine-learning (ML) framework leveraging Gaussian processes (GP) to fuse atomistic computational model predictions across multiple levels of fidelity. Through the…

Computational Physics · Physics 2020-08-06 Anh Tran , Julien Tranchida , Tim Wildey , Aidan P. Thompson

Efficient synthesis recipes are needed both to streamline the manufacturing of complex materials and to accelerate the realization of theoretically predicted materials. Oftentimes the solid-state synthesis of multicomponent oxides is…

Materials Science · Physics 2024-04-10 Jiadong Chen , Samuel R. Cross , Lincoln J. Miara , Jeong-Ju Cho , Yan Wang , Wenhao Sun

We propose a concise stochastic mechanics framework for chemical reaction systems that allows to formulate evolution equations for three general types of data: the probability generating functions, the exponential moment generating…

Mathematical Physics · Physics 2018-02-23 Nicolas Behr , Gérard H. E. Duchamp , Karol A. Penson

We use Bayesian optimization in combination with three-dimensional particle-in-cell simulations to determine the optimal laser and plasma parameters that, for a given laser pulse energy, maximize the cut-off energy of an electron beam…

Plasma Physics · Physics 2025-09-16 P. Valenta , T. Zh. Esirkepov , J. D. Ludwig , S. C. Wilks , S. V. Bulanov

In this work, we introduce a polymer discovery platform to efficiently design polymers with tailored properties, exemplified by the discovery of high-performance polymer electrolytes. The platform integrates three core components: a…

Chemical Physics · Physics 2025-04-04 Arash Khajeh , Xiangyun Lei , Weike Ye , Zhenze Yang , Daniel Schweigert , Ha-Kyung Kwon

The discovery of synthetically accessible organic semiconductors with exceptional performance remains a critical bottleneck in materials science. While these materials offer compelling advantages - structural modularity, mechanical…

The discovery of peptides having high biological activity is very challenging mainly because there is an enormous diversity of compounds and only a minority have the desired properties. To lower cost and reduce the time to obtain promising…

Quantitative Methods · Quantitative Biology 2014-04-11 Sébastien Giguère , François Laviolette , Mario Marchand , Denise Tremblay , Sylvain Moineau , Éric Biron , Jacques Corbeil

We compile data and machine learned models of solid Li-ion electrolyte performance to assess the state of materials discovery efforts and build new insights for future efforts. Candidate electrolyte materials must satisfy several…

Materials Science · Physics 2019-04-22 Austin D. Sendek , Gowoon Cheon , Mauro Pasta , Evan J. Reed

Development of cost-effective hydrogen evolution reaction (HER) catalysts with outstanding catalytic activity, replacing cost-prohibitive noble metal-based catalysts, is critical for practical green hydrogen production. A popular strategy…

In many product development problems, the performance of the product is governed by two types of parameters called design parameter and environmental parameter. While the former is fully controllable, the latter varies depending on the…

Machine Learning · Statistics 2020-06-23 Shogo Iwazaki , Yu Inatsu , Ichiro Takeuchi

High Power Targetry (HPT) R&D is critical in the context of increasing beam intensity and energy for next generation accelerators. Many target concepts and novel materials are being developed and tested for their ability to withstand…

Accelerator Physics · Physics 2024-06-04 W. Asztalos , Y. Torun , S. Bidhar , F. Pellemoine , P. Rath

In this paper, we obtain a Sn-Bi-In-Pb quaternary near eutectic alloy composition from machine learning model. The eutectic points and the alloy composition were evaluated and continuously improved by experimental input. The actual…

Applied Physics · Physics 2021-10-12 Zhenhua Guo , Xintong Ren , Jiahua Jiang , Haoyang Liu , Yongjun Huo , Xiuchen Zhao , K. N. Tu , Yingxia Liu

Efficient electro-catalytic water-splitting technologies require suitable catalysts for the oxygen evolution reaction (OER). The development of novel catalysts could benefit from the achievement of a complete understanding of the reaction…

Materials Science · Physics 2020-04-22 Francesco Nattino , Nicola Marzari

Elucidating the catalytic descriptor that accurately characterizes the structure-activity relationships of typical catalysts for various important heterogeneous catalytic reactions is pivotal for designing high-efficient catalytic systems.…

Chemical Physics · Physics 2025-10-23 Zhen Zhu , Shan Gao , Jing Zhang , Xuxin Kang , Shunfang Li , Xiangmei Duan

Here, we present a study combining Bayesian optimisation structural inference with the machine learning interatomic potential NequIP to accelerate and enable the study of the adsorption of the conformationally flexible lignocellulosic…

Chemical Physics · Physics 2024-02-28 Joakim S. Jestilä , Nian Wu , Fabio Priante , Adam S. Foster

The Li-Air battery is a very promising candidate for powering future mobility, but finding a suitable electrolyte solvent for this technology turned out to be a major problem. We present a systematic computational investigation of the known…

Chemical Physics · Physics 2015-10-28 Tamara Husch , Martin Korth

The Linac Coherent Light Source changes configurations multiple times per day, necessitating fast tuning strategies to reduce setup time for successive experiments. To this end, we employ a Bayesian approach to transport optics tuning to…

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