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We present a depletion imaging technique to map out the spatial and temporal dependency of the density distribution of an ultracold gas of Rydberg atoms. Locally resolved absorption depletion, observed through differential ground state…

High-fidelity entangled Bell states are of great interest in quantum physics. Entanglement of ultracold neutral atoms in two spatially separated optical dipole traps is promising for implementation of quantum computing and quantum…

Atomic Physics · Physics 2018-03-14 I. I. Beterov , G. N. Hamzina , E. A. Yakshina , D. B. Tretyakov , V. M. Entin , I. I. Ryabtsev

Optical trapping of molecules with long coherence times is crucial for many protocols in quantum information and metrology. However, the factors that limit the lifetimes of the trapped molecules remain elusive and require improved…

Atomic Physics · Physics 2020-10-14 K. H. Leung , I. Majewska , H. Bekker , C. -H. Lee , E. Tiberi , S. S. Kondov , R. Moszynski , T. Zelevinsky

A Rydberg and a ground-state atom can form ultralong range diatomic molecules provided the interaction between the ground-state atom and the Rydberg electron is attractive [C. H. Greene, et al., Phys. Rev. Lett. 85, 2458 (2000)]. A…

Atomic Physics · Physics 2008-07-15 Ivan C. H. Liu , Jovica Stanojevic , Jan M. Rost

Rydberg excitons (analogues of Rydberg atoms in condensed matter systems) are highly excited bound electron-hole states with large Bohr radii. The interaction between them as well as exciton coupling to light may lead to strong optical…

We present photo-excitation of ultra-long-range Rydberg molecules as a probe of spatial correlations in quantum gases. Rydberg molecules can be created with well-defined internuclear spacing, set by the radius of the outer lobe of the…

Highly excited Rydberg atoms inherit their level structure, symmetries, and scaling behavior from the hydrogen atom. We demonstrate that these fundamental properties enable a thermodynamic limit of a single Rydberg atom subjected to…

Atomic Physics · Physics 2023-06-23 Matthew T. Eiles , Alexander Eisfeld , Jan M. Rost

Interaction between Rydberg atoms can significantly modify Rydberg excitation dynamics. Under a resonant driving field the Rydberg-Rydberg interaction in high-lying states can induce shifts in the atomic resonance such that a secondary…

We introduce the Rydberg Composite, a new class of Rydberg matter where a single Rydberg atom is interfaced with a dense environment of neutral ground state atoms. The properties of the Composite depend on both the Rydberg excitation, which…

Atomic Physics · Physics 2020-09-02 Andrew L. Hunter , Matthew T. Eiles , Alex Eisfeld , Jan M. Rost

We report the observation of dipole-forbidden, but quadrupole-allowed, one-photon transitions to high Rydberg states in Rb. Using pulsed UV excitation of ultracold atoms in a magneto-optical trap, we excite $5s \to nd$ transitions over a…

We propose and analyze a robust implementation of Rydberg antiblockade based on rapid adiabatic passage. Although Rydberg antiblockade offers key opportunities in quantum information processing and sensing, its sensitivity to position…

Quantum Physics · Physics 2025-10-03 Xinghan Wang , Yupeng Wang , Qi-Yu Liang

We calculate interspecies Rydberg-Rydberg interaction strengths for the heavy alkalis Rb and Cs. The presence of strong F\"orster resonances makes interspecies coupling a promising approach for long range entanglement generation. We also…

Quantum Physics · Physics 2016-07-26 I. I. Beterov , M. Saffman

Pulsed laser excitation of a dense ultracold Cs vapor has been used to study the pairwise interactions between Cs atoms excited to $n$p$_{3/2}$ Rydberg states of principal quantum numbers in the range $n=22-36$. Molecular resonances were…

Atomic Physics · Physics 2015-09-14 Heiner Saßmannshausen , Frédéric Merkt , Johannes Deiglmayr

Dipole-dipole interactions between helium atoms in Rydberg-Stark states with principal quantum number $n=53$ and approximately linear Stark energy shifts, resulting from induced electric dipole moments of approximately 7900 D, have been…

Atomic Physics · Physics 2015-07-14 V. Zhelyazkova , S. D. Hogan

We investigate the long-range, two-body interactions between rubidium and potassium atoms in highly excited ($n=70$) Rydberg states. After establishing properly symmetrized asymptotic basis states, we diagonalize an interaction Hamiltonian…

Atomic Physics · Physics 2023-05-09 Nolan Samboy

High Rydberg states of nitric oxide (NO) with principal quantum numbers between 40 and 100 and lifetimes in excess of 10 $\mu$s have been prepared by resonance enhanced two-color two-photon laser excitation from the X $^2\Pi_{1/2}$ ground…

Chemical Physics · Physics 2020-05-04 A. Deller , S. D Hogan

We suggest a novel way to use strong Rydberg dipole-dipole interactions in order to induce non-trivial conditional dynamics in individual-atom systems and mesoscopic ensembles. Contrary to previous works, we suggest to excite atoms into…

Quantum Physics · Physics 2009-11-13 E. Brion , A. S. Mouritzen , K. Molmer

A quantum-feedback-based scheme is proposed for generating multipartite entanglements of Rydberg atoms in a dissipative optical cavity. The Rydberg blockade mechanism efficiently prevents double excitations of the system, which is further…

Quantum Physics · Physics 2017-02-15 X. Q. Shao , J. H. WU , X. X. Yi

We investigated resonant multiphoton excitation of high-angular-momentum planetary states of the strontium atom, a quasi-three-body Coulomb system, both experimentally and theoretically. A series of highly doubly excited electronic states…

Atomic Physics · Physics 2025-09-26 Matthieu Génévriez , Maxence Jungers , Christian Rosen , Ulrich Eichmann

We propose an experimentally realizable scheme to produce triatomic ultralong-range Rydberg molecules (TURM), formed in ultracold KRb traps. A near resonant coupling of the non-zero quantum defect Rydberg levels with the KRb molecule in N=0…