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A two level model of a single molecule undergoing spectral diffusion dynamics and interacting with a sequence of two short laser pulses is investigated. Analytical solution for the probability of n=0,1,2 photon emission events for the…

Chemical Physics · Physics 2009-11-13 F. Shikerman , E. Barkai

Ultrafast optical pump-probe spectroscopy is used to track carrier dynamics in the large magnetoresistance material WTe$_{2}$. Our experiments reveal a fast relaxation process occurring on a sub-picosecond time scale that is caused by…

Pulsed plasmas in liquids exhibit complex interaction between three phases of matter (liquids, gas, plasmas) and are currently used in a wide range of applications across several fields, however significant knowledge gaps in our…

Plasma Physics · Physics 2021-06-16 Christopher Campbell , Xin Tang , Yancey Sechrest , Kamel Fezzaa , Zhehui Wang , David Staack

The route towards manipulation of the optoelectronic properties of matter beyond the current limits of electronics starts from a comprehensive study of the ultrafast dynamics triggered by interaction with light. Among them, a fundamental…

Dynamical encirclement of an Exceptional Point (EP) and corresponding time-asymmetric mode evolution properties due to breakdown in adiabatic theorem have been a key to range of exotic physical effects in various open atomic, molecular and…

Optics · Physics 2019-04-17 Arnab Laha , Sibnath Dey , Harsh K. Gandhi , Abhijit Biswas , Somnath Ghosh

Applications of metallic metamaterials have generated significant interest in recent years. Electromagnetic behavior of metamaterials in the optical range is usually characterized by a local-linear response. In this article, we develop a…

Quantitative knowledge of electron-phonon coupling is important for many applications as well as for the fundamental understanding of nonequilibrium relaxation processes. Time-resolved diffraction provides direct access to this knowledge…

Materials Science · Physics 2021-11-18 Daniela Zahn , Hélène Seiler , Yoav William Windsor , Ralph Ernstorfer

Quantum material systems upon applying ultrashort laser pulses provide a rich platform to access excited material phases and their transformations that are not entirely like their equilibrium counterparts. The addressability and potential…

Strongly Correlated Electrons · Physics 2021-08-19 Xiaoyi Sun , Shuaishuai Sun , Chong-Yu Ruan

We experimentally demonstrate hyperfine optical pumping of rubidium atoms probed by an evanescent electromagnetic field at a dielectric-vapor interface. This light-atom interaction at the nanoscale is investigated using a right angle prism…

Quantum Physics · Physics 2020-01-08 Eliran Talker , Pankaj Arora , Yefim Barash , David Wilkowski , Uriel Levy

The field of attosecond physics has expanded significantly in recent years, yet experimental facilities supporting attosecond pump attosecond probe spectroscopy remain rare. Here, we present a newly constructed beamline for the generation…

In pump-probe spectroscopy, two laser pulses are employed to garner dynamical information from the sample of interest. The pump initiates the optical process by exciting a portion of the sample from the electronic ground state to an…

Materials Science · Physics 2023-05-18 D. Sangalli , M. D'Alessandro , C. Attaccalite

Attosecond streaking of photoelectrons emitted by extreme ultraviolet light has begun to reveal how electrons behave during their transport within simple crystalline solids. Many sample types within nanoplasmonics, thin-film physics, and…

Ultrafast optical pump - optical probe and optical pump - terahertz probe spectroscopy were performed on vanadium dioxide (VO2) and vanadium sesquioxide (V2O3) thin films over a wide temperature range. A comparison of the experimental data…

Optical quadratic nonlinearity is ultrafast in nature, while parametric interaction usually manifests only the broadband characteristic. Enormous progress has been made toward broadband phase-matching for parametric amplification and wide…

Collisional relaxation of Coulomb systems is studied in the strongly coupled regime. We use an optical pump-probe approach to manipulate and monitor the dynamics of ions in an ultracold neutral plasma, which allows direct measurement of…

Plasma Physics · Physics 2013-02-26 G. Bannasch , J. Castro , P. McQuillen , T. Pohl , T. C. Killian

When studying the motion of optically trapped particles on the $\mu s$ time scale, in low viscous media such as air, inertia cannot be neglected. Resolution of unusual and interesting behaviour not seen in colloidal trapping experiments is…

Soft Condensed Matter · Physics 2015-03-13 D. R. Burnham , P. J. Reece , D. McGloin

This work investigates the effects of time-varying media, where optical properties change over time, on electromagnetic wave propagation, focusing on plane waves and free-electron evanescent waves. We introduce a switching parameter,…

The non-equilibrium dynamics of matter excited by light may produce electronic phases that do not exist in equilibrium, such as laser-induced high-transition-temperature superconductivity. Here we simulate the dynamics of a metal driven at…

Strongly Correlated Electrons · Physics 2022-12-05 John Sous , Benedikt Kloss , Dante M. Kennes , David R. Reichman , Andrew J. Millis

Electrochemical energy systems rely on particulate porous electrodes to store or convert energies. While the three-dimensional porous structures were introduced to maximize the interfacial area for better overall performance of the system,…

Applied Physics · Physics 2021-02-16 Shubham Agrawal , Peng Bai
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