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We investigate the physical mechanisms for spin-dependent recombination of a strongly bound pair of triplet excitons generated by singlet fission and forming a spin quintet (total spin of two) bi-exciton. For triplet excitons the…

Mesoscale and Nanoscale Physics · Physics 2024-02-16 Yan Sun , L. R. Weiss , V. Derkach , J. E. Anthony , M. Monteverde , A. D. Chepelianskii

Molecular spin systems based on photoexcited triplet pairs formed via singlet fission (SF) are attractive as carriers of quantum information because of their potentially pure and controllable spin polarization, but developing systems that…

Mesoscale and Nanoscale Physics · Physics 2022-11-09 Gajadhar Joshi , Ryan D. Dill , Karl J. Thorley , John E. Anthony , Obadiah G. Reid , Justin C. Johnson

We report on a direct measurement of the pair-wise anti-symmetric exchange interaction, known as the Dzyaloshinsky-Moriya interaction (DMI), in a Nd3+-doped YVO4 crystal. To this end we introduce a broadband electron spin resonance…

Mesoscale and Nanoscale Physics · Physics 2017-03-20 Cyril Laplane , Emmanuel Zambrini Cruzeiro , Florian Fröwis , Philippe Goldner , Mikael Afzelius

Spin triplet exciton formation sets limits on technologies using organic semiconductors that are confined to singlet-triplet photophysics. In contrast, excitations in the spin doublet manifold in organic radical semiconductors can show…

Chemical Physics · Physics 2023-12-19 Qinying Gu , Sebastian Gorgon , Alexander S. Romanov , Feng Li , Richard H. Frienda , Emrys Evansd

The nonreciprocal propagation of spin waves in an ultrathin Pt/Co/Ni film has been measured by Brillouin light scattering. The frequency nonreciprocity, due to the interfacial Dzyaloshinskii-Moriya interaction (DMI), has a sinusoidal…

The Dzyaloshinskii-Moriya Interaction (DMI) between spins is induced by spin-orbit coupling in magnetic materials lacking inversion symmetry. DMI is recognized to play a crucial role at the interface between ferromagnetic (FM) and heavy…

Materials Science · Physics 2015-12-31 Hongxin Yang , André Thiaville , Stanislas Rohart , Albert Fert , Mairbek Chshiev

We investigate the chiral magnetic order in free-standing planar 3$d$-5$d$ bi-atomic metallic chains (3$d$: Fe, Co; 5$d$: Ir, Pt, Au) using first-principles calculations based on density functional theory. We found that the antisymmetric…

Mesoscale and Nanoscale Physics · Physics 2015-06-19 Vikas Kashid , Timo Schena , Bernd Zimmermann , Yuriy Mokrousov , Stefan Blügel , Vaishali Shah , H. G. Salunke

The magnetic exchange interaction is the one of the key factors governing the basic characteristics of magnetic systems. Unlike the symmetric nature of the Heisenberg exchange interaction, the interfacial Dzyaloshinskii-Moriya interaction…

Broken inversion symmetry in combination with the spin-orbit interaction generates a finite Dzyaloshinskii-Moriya interaction (DMI), which can induce noncollinear spin textures of chiral nature. The DMI is characterized by an interaction…

Mesoscale and Nanoscale Physics · Physics 2020-09-09 Flaviano José dos Santos , Manuel dos Santos Dias , Samir Lounis

Interacting impurity spins adsorbed on surfaces have been suggested as basic components for applications in quantum computation and spintronics. Such spins usually prefer a parallel or antiparallel configuration, but weakly non-collinear…

Superconductivity · Physics 2025-08-06 Jabir Ali Ouassou , Takehito Yokoyama , Jacob Linder

We have studied far infrared transmission spectra of alpha'-NaV2O5 between 3 and 200cm-1 in polarizations of incident light parallel to a, b, and c crystallographic axes in magnetic fields up to 33T. The triplet origin of an excitation at…

Strongly Correlated Electrons · Physics 2009-11-10 T. Rõõm , D. Hüvonen , U. Nagel , Y. -J. Wang , R. K. Kremer

The photo-driven process of singlet fission generates coupled triplet pairs (TT) with fundamentally intriguing and potentially useful properties. The quintet 5TT0 sublevel is particularly interesting for quantum information because it is…

Proposals for novel spin-orbitronic logic1 and memory devices2 are often predicated on assumptions as to how materials with large spin-orbit coupling interact with ferromagnets when in contact. Such interactions give rise to a host of novel…

Mesoscale and Nanoscale Physics · Physics 2015-08-05 Hans T. Nembach , Justin M. Shaw , Mathias Weiler , Emilie Jué , Thomas J. Silva

The Dzyaloshinskii-Moriya interaction (DMI) that arises in the magnetic systems with broken inversion symmetry plays an essential role in topological spintronics. Here, by means of atomistic spin calculations, we study an intriguing type of…

Materials Science · Physics 2022-12-13 Jinghua Liang , Mairbek Chshiev , Albert Fert , Hongxin Yang

Spins in quantum dots can act as the qubit for quantum computation. In this context we point out that spins on neighboring dots will experience an anisotropic form of the exchange coupling, called the Dzyaloshinskii-Moriya (DM) interaction,…

Materials Science · Physics 2009-11-11 Sucismita Chutia , Mark Friesen , Robert Joynt

We show that the recent experimental realization of spin-orbit coupling in ultracold atomic gases can be used to study different types of spin spiral order and resulting multiferroic effects. Spin-orbit coupling in optical lattices can give…

Quantum Gases · Physics 2015-06-01 Ming Gong , Yinyin Qian , Mi Yan , V. W. Scarola , Chuanwei Zhang

The interfacial Dzyaloshinskii Moriya Interaction (DMI) in ultrathin magnetic thin film heterostructures provides a new approach for controlling spin textures on mesoscopic length scales. Here we investigate the dependence of the…

From organic electronics to biological systems, understanding the role of intermolecular interactions between spin pairs is a key challenge. Here we show how such pairs can be selectively addressed with combined spin and optical…

Electric control of magnetism is a prerequisite for efficient and low power spintronic devices. More specifically, in heavy metal/ ferromagnet/ insulator heterostructures, voltage gating has been shown to locally and dynamically tune…

The search for chiral magnetic textures in systems lacking spatial inversion symmetry has attracted a massive amount of interest in the recent years with the real space observation of novel exotic magnetic phases such as skyrmions lattices,…

Materials Science · Physics 2015-11-06 Abderrezak Belabbes , Gustav Bihlmayer , Stefan Blügel , Aurelien Manchon
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