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There is a growing interest in identifying the origin of single-photon emission in hexagonal boron nitride (hBN), with proposed candidates including boron and nitrogen vacancies as well as carbon substitutional dopants. Because photon…

Hexagonal boron nitride (hBN) has recently emerged as a fascinating platform for room-temperature quantum photonics due to the discovery of robust visible light single-photon emitters. In order to utilize these emitters, it is necessary to…

In conventional optical Stark-shift spectroscopy, molecules are exposed to spatially homogeneous static electric fields that shift the energies of their spectral lines. These shifts are attributed to the molecular electronic properties,…

A key advantage of utilizing van der Waals materials as defect-hosting platforms for quantum applications is the controllable proximity of the defect to the surface or the substrate for improved light extraction, enhanced coupling with…

We report on multicolor excitation experiments with color centers in hexagonal boron nitride at cryogenic temperatures. We demonstrate controllable optical switching between bright and dark states of color centers emitting around 2eV.…

Mesoscale and Nanoscale Physics · Physics 2020-05-13 Prince Khatri , Andrew J. Ramsay , Ralph N. E. Malein , Harold M. H. Chong , Isaac J. Luxmoore

The negatively charged boron vacancy (VB-) in hexagonal boron nitride (hBN) has been extensively investigated as it offers a novel playground for two-dimensional quantum sensing, with ultimate proximity to target samples. However, its…

Spin defects in hexagonal boron nitride (hBN) are promising quantum systems for the design of flexible two-dimensional quantum sensing platforms. Here we rely on hBN crystals isotopically enriched with either $^{10}$B or $^{11}$B to…

Materials Science · Physics 2023-10-03 A. Haykal , R. Tanos , N. Minotto , A. Durand , F. Fabre , J. Li , J. H. Edgar , V. Ivady , A. Gali , T. Michel , A. Dréau , B. Gil , G. Cassabois , V. Jacques

This report summarizes progress made in understanding properties such as zero-phonon-line energies, emission and absorption polarizations, electron-phonon couplings, strain tuning and hyperfine coupling of single photon emitters in…

Materials Science · Physics 2020-04-22 A. Sajid , Michael J. Ford , Jeffrey R. Reimers

Color centers in hexagonal boron nitride (hBN) have attracted significant interest due to their potential applications in future optical quantum technologies. For most applications, scalable on-demand fabrication is a key requirement.…

Color center is a promising platform for quantum technologies, but their application is hindered by the typically random defect distribution and complex mesoscopic environment. Employing cathodoluminescence, we demonstrate that an…

We theoretically study physical properties of the most promising color center candidates for the recently observed single-photon emissions in hexagonal boron nitride (h-BN) monolayers. Through our group theory analysis combined with density…

Mesoscale and Nanoscale Physics · Physics 2018-05-21 Mehdi Abdi , Jyh-Pin Chou , Adam Gali , Martin B. Plenio

We present comprehensive optical studies of recently discovered single photon sources in boron nitride, which appear in form of narrow lines emitting centres. Here, we aim to compactly characterise their basic optical properties, including…

Mesoscale and Nanoscale Physics · Physics 2018-01-17 Maciej Koperski , Karol Nogajewski , Marek Potemski

Atom-like defects in two-dimensional (2D) hexagonal boron nitride (hBN) have recently emerged as a promising platform for quantum information science. Here we investigate single-photon emissions from atomic defects in boron nitride…

Hexagonal boron nitride (hBN) has emerged as a promising material platform for nanophotonics and quantum sensing, hosting optically-active defects with exceptional properties such as high brightness and large spectral tuning. However,…

Optically addressable spins associated with defects in wide-bandgap semiconductors are versatile platforms for quantum information processing and nanoscale sensing, where spin-dependent inter-system crossing (ISC) transitions facilitate…

Quantum Physics · Physics 2019-07-23 Annemarie L. Exarhos , David A. Hopper , Raj N. Patel , Marcus W. Doherty , Lee C. Bassett

Many quantum emitters have been measured close or near the grain boundaries of the two-dimensional hexagonal boron nitride where various Stone-Wales defects appear. We show by means of first principles density functional theory calculations…

Materials Science · Physics 2021-01-12 Hanen Hamdi , Gergő Thiering , Zoltán Bodrog , Viktor Ivády , Adam Gali

Single defect centers in layered hexagonal boron nitride (hBN) are promising candidates as single photon sources for quantum optics and nanophotonics applications. However, until today spectral instability hinders many applications. Here,…

Mesoscale and Nanoscale Physics · Physics 2018-09-12 A. Dietrich , M. Bürk , E. S. Steiger , L. Antoniuk , T. T. Tran , M. Nguyen , I. Aharonovich , F. Jelezko , A. Kubanek

Point defects significantly influence the optical and electrical properties of solid-state materials due to their interactions with charge carriers, which reduce the band-to-band optical transition energy. There has been a demand for…

Mesoscale and Nanoscale Physics · Physics 2018-04-04 Jiandong Feng , Hendrik Deschout , Sabina Caneva , Stephan Hofmann , Ivor Lončarić , Predrag Lazić , Aleksandra Radenovic

Point defects in semiconductors are attractive candidates for quantum information science applications owing to their ability to act as spin-photon interface or single-photon emitters. However, the coupling between the change of dipole…

Materials Science · Physics 2024-09-10 Louis Alaerts , Yihuang Xiong , Sinéad Griffin , Geoffroy Hautier

Atom-like defects in hexagonal boron nitride (hBN) provide room-temperature single-photon emission and coherent spin states, making them attractive for quantum-computing and -sensing applications. However, their random spatial and spectral…