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Related papers: Delocalized Excitation Transfer in Open Quantum Sy…

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A generic and intuitive model for coherent energy transport in multiple minima systems coupled to a quantum mechanical bath is shown. Using a simple spin-boson system, we illustrate how a generic donor-acceptor system can be brought into…

Biological Physics · Physics 2014-06-24 Tristan Farrow , Vlatko Vedral

We investigate exciton transport through one-dimensional molecular aggregates interacting strongly with a cavity mode. Unlike several prior theoretical studies treating the monomers as simple two-level systems, exciton-vibration coupling is…

Mesoscale and Nanoscale Physics · Physics 2019-03-14 Jingyu Liu , Qing Zhao , Ning Wu

A remarkable amount of theoretical research has been carried out to elucidate the physical origins of the recently observed long-lived quantum coherence in the electronic energy transfer process in biological photosynthetic systems.…

Quantum Physics · Physics 2015-03-19 Sangwoo Shim , Patrick Rebentrost , Stéphanie Valleau , Alan Aspuru-Guzik

Exact diagonalisations of the extended Hubbard model are performed. In the insulating regime it is shown that the nearest neighbour copper-oxygen repulsion, $V$, leads to Frenkel excitons in the charge transfer gap at values of $V$ of the…

Condensed Matter · Physics 2009-10-28 C. Vermeulen , W. Barford , E. R. Gagliano

The non-hermitian quantum dynamics of excitonic energy transfer in photosynthetic systems is investigated using a dissipative two-level dimer model. The approach is based on the Green's function formalism which permits consideration of…

Quantum Physics · Physics 2012-04-03 A. Thilagam

In a network of interacting quantum systems achieving fast coherent energy transfer is a challenging task. While quantum systems are susceptible to a wide range of environmental factors, in many physical settings their interactions with…

Quantum Physics · Physics 2014-05-09 James Lim , Mark Tame , Ki Hyuk Yee , Joong-Sung Lee , Jinhyoung Lee

Using methods of condensed matter and statistical physics, we examine the transport of excitons through the Fenna-Matthews-Olson (FMO) complex from a receiving antenna to a reaction center. Writing the equations of motion for the exciton…

Biological Physics · Physics 2016-02-23 Lev Mourokh , Franco Nori

We present a theory that efficiently describes the quantum dynamics of an electronic excitation that is coupled to a continuous, highly structured phonon environment. Based on a stochastic approach to non-Markovian open quantum systems, we…

Quantum Physics · Physics 2009-11-05 Jan Roden , Alexander Eisfeld , Wolfgang Wolff , Walter T. Strunz

We present a simple quantum open system to show quantitatively how entanglement decoherence is related to the energy transfer between the system of interest and its environment. Particularly, in the case of the exact entanglement…

Quantum Physics · Physics 2007-05-23 Ting Yu

The role of noise in the transport properties of quantum excitations is a topic of great importance in many fields, from organic semiconductors for technological applications to light-harvesting complexes in photosynthesis. In this paper we…

Quantum Physics · Physics 2016-11-22 Stefano Iubini , Octavi Boada , Yasser Omar , Francesco Piazza

Open quantum system approaches are widely used in the description of physical, chemical and biological systems. A famous example is electronic excitation transfer in the initial stage of photosynthesis, where harvested energy is transferred…

An atom-waveguide system, which presents one of the quantum interfaces that enable strong couplings between light and atoms, can support tightly-confined guided modes of light. In this distinctive quantum interface, we theoretically…

Quantum Physics · Physics 2021-05-18 H. H. Jen , J. -S. You

The accurate description of the interaction of a quantum system with a its environment is a challenging problem ubiquitous across all areas of physics, and lies at the foundation of quantum mechanics theory. Here we pioneer a new strategy…

Quantum Physics · Physics 2024-10-21 Hideaki Takahashi , Raffaele Borrelli

F\"orster theory describes electronic exciton energy migration in molecular assemblies as an incoherent hopping process between donor and acceptor molecules. The rate is expressed in terms of the overlap integral between donor fluorescence…

Chemical Physics · Physics 2018-10-17 Marco Schröter , Tõnu Pullerits , Oliver Kühn

It is shown that energy transfer in a homogeneous fully connected quantum network is assisted by a decohering interaction with environmental spins. Analytic expressions for the transfer probabilities are obtained for the zero temperature…

Quantum Physics · Physics 2014-01-28 A. Marais , I. Sinayskiy , A. Kay , F. Petruccione , A. Ekert

Resonant energy transfer mechanisms have been observed in the sensitized luminescence of solids, in quantum dots and in molecular nanostructures, and they also play a central role in light harvesting processes in photosynthetic organisms.…

Quantum Physics · Physics 2009-11-07 Brendon Lovett , John H. Reina , Ahsan Nazir , Beeneet Kothari , Andrew Briggs

We consider models in which two sets of matched two-level systems are coupled to a common oscillator in the case where the oscillator energy is small relative to the two-level transition energies. Since the two sets of two-level systems are…

Other Condensed Matter · Physics 2007-05-23 Peter L. Hagelstein , Irfan U. Chaudhary

Computationally tractable and reliable, albeit approximate, methods for studying exciton transport in molecular aggregates immersed in structured bosonic environments have been actively developed. Going beyond the lowest-order (Born)…

Chemical Physics · Physics 2024-11-28 Veljko Janković , Tomáš Mančal

We consider the reduced dynamics of a molecular chain weakly coupled to a phonon bath. With a small and constant inhomogeneity in the coupling, the excitation relaxation rates are obtained in closed form. They are dominated by transitions…

Statistical Mechanics · Physics 2021-04-16 B. A. Tay

Noise-assisted transport in quantum systems occurs when quantum time-evolution and decoherence conspire to produce a transport efficiency that is higher than what would be seen in either the purely quantum or purely classical cases. In…

Quantum Physics · Physics 2012-08-30 Ivan Kassal , Alán Aspuru-Guzik