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Laser frequency combs are coherent light sources that emit a broad spectrum consisting of discrete, evenly spaced narrow lines, each having an absolute frequency measurable within the accuracy of an atomic clock. Their development, a decade…

Optics · Physics 2017-06-13 Albert Schliesser , Nathalie Picqué , Theodor W. Hänsch

The highly energetic photons of ultraviolet light drive electronic and rovibronic transitions in all molecular species. This radiation is thus a prime tool for strongly selective spectroscopic fingerprinting and real-time environmental…

We demonstrate the use of dual-comb spectroscopy for isotope ratio measurements. We show that the analysis spectral range of a free-running near-infrared dual-comb spectrometer can be extended to the mid-infrared by difference frequency…

Instrumentation and Detectors · Physics 2022-05-10 Alexandre Parriaux , Kamal Hammani , Christophe Thomazo , Olivier Musset , Guy Millot

Optical frequency combs based on semiconductor lasers are a promising technology for monolithic integration of dual-comb spectrometers. However, the stabilization of the offset frequency fceo remains a challenging feat due the lack of…

Tunable mid-infrared lasers are essential for optical sensing and imaging. Existing technologies, however, face challenges in simultaneously achieving broadband spectral tunability and ultra-rapid scan rates, limiting their utility in…

Optics · Physics 2025-01-20 Xiaoshuai Ma , Tianjian Lv , Xudong Zhu , Ming Yan , Heping Zeng

We present a versatile mid-infrared frequency comb spectroscopy system based on a doubly resonant optical parametric oscillator tunable in the 3-5.4 {\mu}m range and two detection methods, a Fourier transform spectrometer (FTS) and a…

Mid-infrared (mid-IR) frequency combs have broad applications in molecular spectroscopy and chemical/biological sensing. Recently developed microresonator-based combs in this wavelength regime could enable portable and robust devices using…

Dual-comb interferometry harnesses the interference of two laser frequency combs to provide unprecedented capability in spectroscopy applications. In the past decade, the state-of-the-art systems have reached a point where the…

Quantum Physics · Physics 2023-09-20 Haowei Shi , Zaijun Chen , Scott E. Fraser , Mengjie Yu , Zheshen Zhang , Quntao Zhuang

An outstanding challenge for deployable quantum technologies is the availability of high-resolution laser spectroscopy at the specific wavelengths of ultranarrow transitions in atomic and solid-state quantum systems. Here, we demonstrate a…

Optics · Physics 2023-09-29 David A. Long , Jordan R. Stone , Yi Sun , Daron Westly , Kartik Srinivasan

We demonstrate a dual optical frequency comb concept that down-converts arbitrary narrowband D-band (110-170 GHz) signals to baseband without any filter or optical/RF frequency tuning, using low frequency RF components.

Optics · Physics 2025-12-24 Callum Deakin , Zichuan Zhou , Ronit Sohanpal , Zhixin Liu

Spectral analysis is one of the most powerful technologies for studying and understanding matter. As the devices for spectral analysis, spectrometers are widely used in material detection, isotope analysis, trace gas detection, and the…

Molecular spectroscopy in the mid-infrared portion of the electromagnetic spectrum (3--25 um) has been a cornerstone interdisciplinary analytical technique widely adapted across the biological, chemical, and physical sciences. Applications…

Instrumentation and Detectors · Physics 2018-09-18 Abijith S. Kowligy , Henry Timmers , Alex Lind , Ugaitz Elu , Flavio C. Cruz , Peter G. Schunemann , Jens Biegert , Scott A. Diddams

Fourier transform spectroscopy based on incoherent light sources is a well-established tool in research fields from molecular spectroscopy and atmospheric monitoring to material science and biophysics. It provides broadband molecular…

Dual-comb interferometry utilizes two optical frequency combs to map the optical field's spectrum to a radio-frequency signal without using moving parts, allowing improved speed and accuracy. However, the method is compounded by the…

Holography has always held special appeal, for it is able to record and display spatial information in three dimensions. Here, we show how to augment the capabilities of digital holography by using a large number of narrow laser lines at…

Dual-comb spectroscopy enables broadband analysis of key molecules with unparalleled frequency resolution and exceptional signal-to-noise ratios across various spectral regions. However, fully harnessing its potential for broadband…

Nanophotonic waveguides with sub-wavelength mode confinement and engineered dispersion profiles are an excellent platform for application-tailored nonlinear optical interactions at low pulse energies. Here, we present fully air clad…

Optical frequency combs based on mode-locked lasers have proven to be invaluable tools for a wide range of applications in precision spectroscopy and metrology. A novel principle of optical frequency comb generation in whispering-gallery…

Optics · Physics 2015-06-12 Pascal Del'Haye , Scott B. Papp , Scott A. Diddams

Spectroscopy in the molecular fingerprint spectral region (6.5-20 $\mu$m) yields critical information on material structure for physical, chemical and biological sciences. Despite decades of interest and effort, this portion of the…

Frequency combs have revolutionized time and frequency metrology and in recent years, new frequency comb lasers that are highly compact or even on-chip have been demonstrated in the mid-infrared and THz regions of the electromagnetic…

Optics · Physics 2019-07-17 Giacomo Scalari , Jérôme Faist , Nathalie Picqué
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