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Biomolecular computers, along with quantum computers, may be a future alternative for traditional, silicon-based computers. Main advantages of biomolecular computers are massive parallel processing of data, expanded capacity of storing…

Emerging Technologies · Computer Science 2011-09-28 Janusz Blasiak , Tadeusz Krasinski , Tomasz Poplawski , Sebastian Sakowski

In quantum chemistry, the price paid by all known efficient model chemistries is either the truncation of the Hilbert space or uncontrolled approximations. Theoretical computer science suggests that these restrictions are not mere…

Chemical Physics · Physics 2017-03-15 James D. Whitfield , Peter J. Love , Alan Aspuru-Guzik

In the paper we define three new complexity classes for Turing Machine undecidable problems inspired by the famous Cook/Levin's NP-complete complexity class for intractable problems. These are U-complete (Universal complete), D-complete…

Computational Complexity · Computer Science 2023-06-22 Eugene Eberbach

The computational cost of exact methods for quantum simulation using classical computers grows exponentially with system size. As a consequence, these techniques can only be applied to small systems. By contrast, we demonstrate that quantum…

Quantum Physics · Physics 2008-12-17 Ivan Kassal , Stephen P. Jordan , Peter J. Love , Masoud Mohseni , Alán Aspuru-Guzik

We give an effective procedure that produces a natural number in its output from any natural number in its input, that is, it computes a total function. The elementary operations of the procedure are Turing-computable. The procedure has a…

Artificial Intelligence · Computer Science 2013-02-06 Kurt Ammon

We demonstrate the first end-to-end integration of high-performance computing (HPC), reliable quantum computing, and AI in a case study on catalytic reactions producing chiral molecules. We present a hybrid computation workflow to determine…

A long-standing goal of science is to accurately solve the Schr\"odinger equation for large molecular systems. The poor scaling of current quantum chemistry algorithms on classical computers imposes an effective limit of about a few dozen…

Chemical Physics · Physics 2022-02-11 Joshua A. Rackers , Lucas Tecot , Mario Geiger , Tess E. Smidt

We describe a method to axiomatize computations in deterministic Turing machines. When applied to computations in non-deterministic Turing machines, this method may produce contradictory (and therefore trivial) theories, considering…

Quantum Physics · Physics 2008-07-27 Juan C. Agudelo , Walter Carnielli

The Turing completeness result for continuous chemical reaction networks (CRN) shows that any computable function over the real numbers can be computed by a CRN over a finite set of formal molecular species using at most bimolecular…

Quantitative Methods · Quantitative Biology 2021-07-01 Mathieu Hemery , François Fages , Sylvain Soliman

Instruction sequence is a key concept in practice, but it has as yet not come prominently into the picture in theoretical circles. This paper concerns instruction sequences, the behaviours produced by them under execution, the interaction…

Logic in Computer Science · Computer Science 2012-05-07 J. A. Bergstra , C. A. Middelburg

Numerous reports claim that quantum advantage, which should emerge as a direct consequence of the advent of quantum computers, will herald a new era of chemical research because it will enable scientists to perform the kinds of quantum…

Quantum Physics · Physics 2020-09-29 V. E. Elfving , B. W. Broer , M. Webber , J. Gavartin , M. D. Halls , K. P. Lorton , A. Bochevarov

Robustness to a wide variety of negative factors and the ability to self-repair is an inherent and natural characteristic of all life forms on earth. As opposed to nature, man-made systems are in most cases not inherently robust and a…

Neural and Evolutionary Computing · Computer Science 2016-11-15 Christof Teuscher

Natural language processing models have emerged that can generate usable software and automate a number of programming tasks with high fidelity. These tools have yet to have an impact on the chemistry community. Yet, our initial testing…

Statistical Mechanics · Physics 2023-01-11 Glen M. Hocky , Andrew D. White

Chaitin's work, in its depth and breadth, encompasses many areas of scientific and philosophical interest. It helped establish the accepted mathematical concept of randomness, which in turn is the basis of tools that I have developed to…

Information Theory · Computer Science 2021-06-11 Hector Zenil

Machine-learning potentials (MLPs) for atomistic simulations are a promising alternative to conventional classical potentials. Current approaches rely on descriptors of the local atomic environment with dimensions that increase…

Materials Science · Physics 2017-12-05 Nongnuch Artrith , Alexander Urban , Gerbrand Ceder

The recent advances in neural language models have also been successfully applied to the field of chemistry, offering generative solutions for classical problems in molecular design and synthesis planning. These new methods have the…

Machine Learning · Computer Science 2023-05-19 Dimitrios Christofidellis , Giorgio Giannone , Jannis Born , Ole Winther , Teodoro Laino , Matteo Manica

Large language models (LLMs) are beginning to reshape how chemists plan and run reactions in organic synthesis. Trained on millions of reported transformations, these text-based models can propose synthetic routes, forecast reaction…

Artificial Intelligence · Computer Science 2025-08-08 Kartar Kumar Lohana Tharwani , Rajesh Kumar , Sumita , Numan Ahmed , Yong Tang

Instead of producing quantum languages that are fit for current quantum computers, we build a language from standard classical assembler and augment it with quantum capabilities so that quantum algorithms become a subset of it. This paves…

Quantum Physics · Physics 2022-06-29 Thomas Gabor , Marian Lingsch Rosenfeld , Claudia Linnhoff-Popien

The dramatic increase in the efficiency of a quantum computer over a classical computer, raises a natural question asking, how much of this success could be attributed to its quantum nature and how much to its probabilistic content. To…

Statistical Mechanics · Physics 2007-05-23 Anjan Kundu

Quantum computers promise to efficiently solve important problems classical computers never will. However, in order to capitalize on these prospects, a fully automated quantum software stack needs to be developed. This involves a multitude…

Quantum Physics · Physics 2023-01-12 Robert Wille , Lukas Burgholzer , Stefan Hillmich , Thomas Grurl , Alexander Ploier , Tom Peham