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This study examines the Raman scattering and charge transfer properties of molecules adsorbed on the surface of a tetrahedral Au$_{120}$ nanoparticle based on the time-dependent density functional tight-binding (TD-DFTB) method. We study…

Chemical Physics · Physics 2024-09-18 Sajal Kumar Giri , George C. Schatz

Silicon photodetectors operating at near-infrared wavelengths with high-speed and high sensitivity are becoming critical for emerging applications, such as Light Detection and Ranging Systems (LIDAR), quantum communications, and medical…

This paper proposes a framework for fast signal acquisition based on deterministic non-uniform sampling, with emphasis on multi-coset architectures and receivers driven by known synchronization sequences, pilots, or preambles. Unlike…

Signal Processing · Electrical Eng. & Systems 2026-05-19 Alejandro Gonzalez Garrido , Carla Amatetti

Accurate knowledge of absorption coefficient of a sample is a prerequisite for measuring the third order optical nonlinearity of materials, which could become a serious limitation for unknown samples. We introduce a new method, which…

Optics · Physics 2007-05-23 S. Abbas Hosseini , A. Sharan , D. Goswami

We present the result of our calculations of ultrafast electron diffraction (UED) for cyclobutanone excited into $S_2$ electronic state, which are based on the non-adiabatic dynamics simulations with \textit{Ab Initio} Multiple Cloning…

Chemical Physics · Physics 2024-02-19 Dmitry V. Makhov , Adam Kirrander , Dmitrii V. Shalashilin

Spectroscopy is an important tool for probing the properties of materials, chemicals and biological samples. We design a practical transmitter-receiver system that exploits entanglement to achieve a provable quantum advantage over all…

Quantum Physics · Physics 2020-11-03 Haowei Shi , Zheshen Zhang , Stefano Pirandola , Quntao Zhuang

One-dimensional (1D) metal-dielectric (MD) periodic structures take advantage of large refractive index contrast between metal and dielectrics to invoke extremely high nonlinear ultrafast responses of metal. These structures are also…

Absorption imaging of ultracold atoms is the foundation for quantitative extraction of information from experiments with ultracold atoms. Due to the limited exposure time available in these systems, the signal-to-noise ratio is largest for…

We demonstrate a photon-sensitive, three-dimensional camera by active near-infrared illumination and fast time-of-flight gating. It uses pico-second pump pulses to selectively up-convert the backscattered photons according to their…

Optics · Physics 2022-11-01 He Zhang , Santosh Kumar , Yong Meng Sua , Shenyu Zhu , Yu-Ping Huang

With the incorporation of the UNet architecture, diffusion probabilistic models have become a dominant force in image generation tasks. One key design in UNet is the skip connections between the encoder and decoder blocks. Although skip…

Machine Learning · Computer Science 2024-02-26 Jiajun Ma , Shuchen Xue , Tianyang Hu , Wenjia Wang , Zhaoqiang Liu , Zhenguo Li , Zhi-Ming Ma , Kenji Kawaguchi

To obtain the best resolution for any measurement there is an ever-present challenge to achieve maximal differentiation between signal and noise over as fine of sampling dimensions as possible. In diffraction science these issues are…

Instrumentation and Detectors · Physics 2023-10-23 James Weng , Niklas B. Thompson , Christopher Folmar , James D. Martin , Christina Hoffman

In the last decade, the development of Ultrafast Electron Diffraction (UED) and Microscopy (UEM) has enabled the imaging of atomic motion in real time and space. These pivotal table-top tools opened the door for a vast range of applications…

Chemical Physics · Physics 2018-01-16 Mohammed Th. Hassan

We present diffraction patterns from micron-sized areas of mono-crystalline graphite obtained with an ultracold and ultrafast electron source. We show that high spatial coherence is manifest in the visibility of the patterns even for…

Accelerator Physics · Physics 2014-01-07 M. W. van Mourik , W. J. Engelen , E. J. D. Vredenbregt , O. J. Luiten

The signal half of an entangled twin-beam, generated using spontaneous parametric downconversion, interrogates a region of space that is suspected of containing a target, and has high loss and high (entanglement-breaking) background noise.…

Quantum Physics · Physics 2009-11-11 Saikat Guha , Baris I. Erkmen

The absorption of broadband photons in atomic ensembles requires either an effective broadening of the atomic transition linewidth, or an off-resonance Raman interaction. Here we propose a scheme for a quantum memory capable of storing and…

Quantum Physics · Physics 2017-01-18 G. S. Thekkadath , K. Heshami , D. G. England , P. J. Bustard , B. J. Sussman , M. Spanner

Ultrabroadband electro-optic sampling with few-cycle optical pulses is known to be an extremely sensitive technique to detect electric field amplitudes. By combining this method with dual-comb spectroscopy and with a new class of ultrafast…

Neutron direct-geometry time-of-flight chopper spectroscopy is instrumental in studying fundamental excitations of vibrational and/or magnetic origin. We report here that techniques in super-resolution optical imagery (which is in…

Data Analysis, Statistics and Probability · Physics 2020-01-08 Fahima Islam , Jiao Y. Y. Lin , Richard Archibald , Douglas L. Abernathy , Iyad Al-Qasir , Anne A. Campbell , Matthew B. Stone , Garrett E. Granroth

Quarter sampling is a novel sensor concept that enables the acquisition of higher resolution images without increasing the number of pixels. This is achieved by covering three quarters of each pixel of a low-resolution sensor such that only…

Image and Video Processing · Electrical Eng. & Systems 2022-03-02 Simon Grosche , Kristian Fischer , Fabian Brand , Jürgen Seiler , André Kaup

We demonstrate a non-invasive time-sorting method for ultrafast electron diffraction (UED) experiments with radio-frequency (rf) compressed electron beams. We show that electron beam energy and arrival time at the sample after rf…

Accelerator Physics · Physics 2021-08-24 Lingrong Zhao , Jun Wu , Zhe Wang , Heng Tang , Xiao Zou , Tao Jiang , Pengfei Zhu , Dao Xiang , Jie Zhang

To absorb the photons below the band-gap energy effectively, we proposed a quantum dot (QD) photocell modeled by multi-level system for the quantum yields and photo-to-charge efficiency limits. The theoretical results show the quantum…

Mesoscale and Nanoscale Physics · Physics 2024-02-26 Shun-Cai Zhao , Jing-Yi Chen