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Microscopic relaxation timescales are estimated from the autocorrelation functions obtained by dynamic light scattering experiments for Laponite suspensions with different concentrations ($C_{L}$), added salt concentrations ($C_{S}$) and…

Soft Condensed Matter · Physics 2016-01-20 Debasish Saha , Yogesh M. Joshi , Ranjini Bandyopadhyay

We present x-ray photon correlation spectroscopy measurements of the atomic dynamics in a Zr67Ni33 metallic glass, well below its glass transition temperature. We find that the decay of the density fluctuations can be well described by…

Soft Condensed Matter · Physics 2015-06-12 B. Ruta , G. Baldi , G. Monaco , Y. Chushkin

We propose that the super-Arrhenius relaxation rates observed in glassy materials are determined by thermally nucleated rearrangements of increasing numbers of molecules at decreasing temperatures. In our model of this mechanism,…

Materials Science · Physics 2016-08-16 J. S. Langer , Anaël Lemaître

We show that the various crossovers between dynamical regimes observed in experiments and simulations of supercooled liquids can be explained in simple terms from the existence and statistical properties of dynamical heterogeneities. We…

Statistical Mechanics · Physics 2009-11-10 Ludovic Berthier , Juan P. Garrahan

If quenched fast enough, a liquid is able to avoid crystallization and will remain in a metastable supercooled state down to the glass transition, with an important increase in viscosity upon further cooling. There are important differences…

Disordered Systems and Neural Networks · Physics 2016-06-01 C. Yildirim , J. -Y. Raty , M. Micoulaut

The physics of active systems of self-propelled particles, in the regime of a dense liquid state, is an open puzzle of great current interest, both for statistical physics and because such systems appear in many biological contexts. We…

Soft Condensed Matter · Physics 2017-10-26 Saroj Kumar Nandi , Nir S. Gov

We present a computer simulation study of glassy and crystalline states using the standard Lennard-Jones interaction potential that is truncated at a finite cut-off distance, as is typical of many computer simulations. We demonstrate that…

Soft Condensed Matter · Physics 2016-04-19 Hideyuki Mizuno , Leonardo E. Silbert , Matthias Sperl , Stefano Mossa , Jean-Louis Barrat

A multi-time extension of a density correlation function is introduced to reveal temporal information about dynamical heterogeneity in glass-forming liquids. We utilize a multi-time correlation function that is analogous to the higher-order…

Soft Condensed Matter · Physics 2010-08-03 Kang Kim , Shinji Saito

Properties of water have been well elucidated for temperatures above $\sim$230 K and yet mysteries remain in the deeply supercooled region. By performing extensive molecular dynamics simulations on this supercooled region, we find that…

Soft Condensed Matter · Physics 2018-11-15 Shinji Saito , Biman Bagchi , Iwao Ohmine

We investigate the relation between the cooperative length and the relaxation time, represented respectively by the culling time and the persistence time, in the Fredrickson-Andersen, Kob-Andersen and spiral kinetically-constrained models.…

Statistical Mechanics · Physics 2015-10-01 Eial Teomy , Yair Shokef

Using molecular dynamics simulations we study the out of equilibrium dynamic correlations in a model glass-forming liquid. The system is quenched from a high temperature to a temperature below its glass transition temperature and the decay…

Statistical Mechanics · Physics 2009-10-30 Walter Kob , Jean-Louis Barrat

A general identification of the {\em positional specific heat} as the thermodynamic response function associated with the {\em static relaxation length} is proposed, and a phenomenological description for the thermal dependence of the…

Disordered Systems and Neural Networks · Physics 2009-11-10 S. Davatolhagh

Using the activation-relaxation technique (ART), we study the nature of relaxation events in a binary Lennard-Jones system above and below the glass transition temperature (T_g). ART generates trajectories with almost identical efficiency…

Disordered Systems and Neural Networks · Physics 2007-05-23 Normand Mousseau

We examine structural relaxation in a supercooled glass-forming liquid simulated by NVE molecular dynamics. Time correlations of the total kinetic energy fluctuations are used as a comprehensive measure of the system's approach to the…

Soft Condensed Matter · Physics 2009-05-20 M. Elenius , M. Dzugutov

A theory is developed to calculate values of the potential energy barriers to structural relaxation in molecular glass formers from the data of static pair correlation function. The barrier height is shown to increase due to increase in…

Soft Condensed Matter · Physics 2019-03-13 Ankit Singh , Yashwant Singh

Molecular dynamics simulations of a Lennard-Jones binary mixture confined in a disordered array of soft spheres are presented. The single particle dynamical behavior of the glass former is examined upon supercooling. Predictions of mode…

Statistical Mechanics · Physics 2009-11-07 P. Gallo , R. Pellarin , M. Rovere

We study the glassy dynamics taking place in dense assemblies of athermal active particles that are driven solely by a nonequilibrium self-propulsion mechanism. Active forces are modeled as an Ornstein-Uhlenbeck stochastic process,…

Soft Condensed Matter · Physics 2016-09-28 Elijah Flenner , Grzegorz Szamel , Ludovic Berthier

Molecular dynamics simulations are performed to study spatially heterogeneous dynamics in a model of viscous silica above and below the critical temperature of the mode coupling theory, $T_{MCT}$. Specifically, we follow the evolution of…

Soft Condensed Matter · Physics 2009-11-10 M. Vogel , S. C. Glotzer

In this paper, we analyze the dynamics of the Coulomb Glass lattice model in three dimensions near a local equilibrium state by using mean-field approximations. We specifically focus on understanding the role of localization length ($\xi$)…

Disordered Systems and Neural Networks · Physics 2021-03-31 Preeti Bhandari , Vikas Malik , Deepak Kumar , Moshe Schechter

We present a quantitative study of strain correlations in quiescent supercooled liquids and glasses. Recent two-dimensional computer simulations and experiments indicate that even supercooled liquids exhibit long-lived, long-range strain…

Statistical Mechanics · Physics 2018-11-14 Muhammad Hassani , Elias M. Zirdehi , Kris Kok , Peter Schall , Matthias Fuchs , Fathollah Varnik