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Chiral light matter interaction enables new fundamental researches and applications of light. The interaction has traditionally faced challenges in low directionality and efficiency based on spin orbit interaction of light in microscopic…

Applied Physics · Physics 2019-12-10 Liang Fang , Haozhi Luo , Xiaoping Cao , Shuang Zheng , Xinlun Cai , Jian Wang

Surface plasmons in a centrosymmetric metal nanocrystal have been perceived as achiral, based on the quantum-mechanical theory of molecular optical activity. The one-electron theory is insufficient to describe optical activity in crystals,…

Mesoscale and Nanoscale Physics · Physics 2018-03-02 Jong-Won Park

We study the ground state structure and aspects of photoionization dynamics of the $Na_{20}@C_{240}$ endofullerene. The structure shows effects from the electronic coupling between the nested cluster and the fullerene cage. They include the…

Atomic and Molecular Clusters · Physics 2024-12-20 Rasheed Shaik , Hari R. Varma , Mohamed El-Amine Madjet , Fulu Zheng , Himadri S. Chakraborty

Electronic circular dichroism (ECD) is a powerful spectroscopical method for investigating chiral properties at the molecular level. ECD calculations with the commonly used linear-response time-dependent density functional theory (LR-TDDFT)…

The concept of chirality makes ubiquitous appearance in nature. Particularly, both a structure and its collective excitations may acquire well defined chiralities. In this work, we reveal an intrinsic connection between the chiralities of a…

Materials Science · Physics 2024-05-21 Hao Chen , Weikang Wu , Jiaojiao Zhu , Weikang Gong , Weibo Gao , Shengyuan A. Yang , Lifa Zhang

Plasmonic nanocavities enable access to the quantum properties of matter, but are often simplified to single mode models despite their complex multimode structure. Here, we show that off-resonant plasmonic modes in fact play a crucial role…

Quantum Physics · Physics 2024-11-13 Angus Crookes , Ben Yuen , Angela Demetriadou

We report on a phenomenon of plasmonic dichroism observed in magnetic materials with the transverse magnetization under the excitation of the surface plasmon polariton waves. The effect originates from the interplay of the two…

This review examines the conditions that lead to the formation of flexo-sensitive chiral polar structures in thin films and core-shell ferroelectric nanoparticles. It also analyzes possible mechanisms by which the flexoelectric effect…

Recent efforts in the field of surface-enhanced spectroscopies have focused on the paradigm of superchirality, entailing the engineering of the local electromagnetic fields to boost the enantiospecific interaction between light and chiral…

The chiral plasmon modes of relativistic matter in background magnetic and strain-induced pseudomagnetic fields are studied in detail using the consistent chiral kinetic theory. The results reveal a number of anomalous features of these…

Mesoscale and Nanoscale Physics · Physics 2017-03-27 E. V. Gorbar , V. A. Miransky , I. A. Shovkovy , P. O. Sukhachov

The first observation of tungsten disulfide liquid crystalline nanocomposites in dispersions of liquid phase-exfoliated flakes is demonstrated in a range of organic solvents. The nanocomposites demonstrate significant birefringence and…

Mirror symmetry is among the most fundamental concepts of physics and its spontaneous breaking at the molecular level allows chiral molecules to exist in two enantiomers that are mirror images of each other. The majority of chiro-optical…

Optics · Physics 2021-09-29 Alessandro Ciattoni

Molecular Circular dichroism (CD) spectroscopy faces significant limitations due to the inherent weakness of chiroptical light-matter interactions. In this view, resonant optical antennas constitute a promising solution to this problem…

We present a systematic investigation of the optical response to circularly polarized illumination in twisted stacked plasmonic nanostructures. The system consissts in two identical, parallel gold triskelia centrally aligned and rotated at…

Recently, there is growing interest in integrating alkali vapors with nanoscale photonic structures, such as nano-waveguides, resonators and nanoantennas. Nanoscale confinement of electromagnetic fields may introduce a longitudinal electric…

Optics · Physics 2021-02-10 Roy Zektzer , Eliran Talker , Yefim Barash , Noa Mazurski , Uriel Levy

Polariton states with high levels of chiral dissymmetry offer exciting prospects for quantum information, sensing, and lasing applications. Such dissymmetry must emanate from either the involved optical resonators or the quantum emitters.…

Chemical Physics · Physics 2022-09-28 Andrew H. Salij , Randall H. Goldsmith , Roel Tempelaar

We explore the interplay between tunneling process and chiral interactions in the discrimination of chiral states for an ensemble of molecules in a biological environment. Each molecule is described by an asymmetric double-well potential…

Biomolecules · Quantitative Biology 2017-04-28 Arash Tirandaz , Farhad Taher Ghahramani , Afshin Shafiee

Chirality is a structural property of molecules lacking mirror symmetry that has strong implications in diverse fields, ranging from life to materials sciences. Established spectroscopic methods that are sensitive to chirality, such as…

We investigate photon tunneling in a pair of coupled inverted circular split-ring microwave resonators with four discrete chiral orientations. By varying the spacing between the resonators, we observe strong modulation of the transmission…

We investigate the radiative coupling between two two-level atoms with arbitrarily polarized dipoles in the vicinity of a nanofiber. We present a systematic derivation for the master equation, the single- and cross-atom decay coefficients,…

Quantum Physics · Physics 2016-12-15 Fam Le Kien , Arno Rauschenbeutel