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Optical signals obtained by the material response to classical laser fields are given by nonlinear response functions which can be expressed by sums over various quantum pathways of matter. We show that some pathways can be selected by…

Materials Science · Physics 2009-02-17 O. Roslyak C. A. Marx , S. Mukamel

Two-photon excited fluorescence (TPEF) is a standard technique in modern microscopy but still affected by photo-damage of the probe. It was proposed that TPEF can be enhanced by using entangled photons, but has proven to be challenging.…

Quantum Physics · Physics 2013-10-17 Andreas Jechow , Michael Seefeldt , Henning Kurzke , Axel Heuer , Ralf Menzel

We report how the unique temporal and spectral features of pulsed entangled photons from a parametric downconversion source can be utilized for manipulating electronic excitations through the optimization of their spectral phase. A new…

Chemical Physics · Physics 2024-09-18 Sajal Kumar Giri , George C. Schatz

The paper suggest employing machine learning for resource-efficient classification of quantum correlations in entanglement distribution networks. Specifically, artificial neural networks (ANN) are utilized to classify quantum correlations…

Quantum Physics · Physics 2024-02-15 Jan Soubusta , Antonín Černoch , Karel Lemr

Excitation with entangled photon pairs may lead to an increase in the efficiency of two-photon absorption at low photon flux. The corresponding process, entangled two-photon absorption (E2PA), has been investigated in numerous theoretical…

We propose a simple, but efficient and accurate machine learning (ML) model for developing high-dimensional potential energy surface. This so-called embedded atom neural network (EANN) approach is inspired by the well-known empirical…

Chemical Physics · Physics 2019-10-23 Yaolong Zhang , Ce Hu , Bin Jiang

We experimentally demonstrate a general criterion to identify entangled states useful for the estimation of an unknown phase shift with a sensitivity higher than the shot-noise limit. We show how to exploit this entanglement on the examples…

A scheme to distinguish entangled two-photon-polarization states (ETP) from two independent entangled one-photon-polarization states (EOP) is proposed. Using this scheme, the experimental generation of ETP by parametric down-conversion is…

Quantum Physics · Physics 2009-11-10 Kenji Tsujino , Holger F. Hofmann , Shigeki Takeuchi , Keiji Sasaki

Entangled photon pairs are predicted to linearize and increase the efficiency of two-photon absorption, allowing continuous wave laser diodes to drive ultrafast time-resolved spectroscopy and nonlinear processes. Despite a range of…

Quantum Physics · Physics 2022-05-31 Bryce P. Hickam , Manni He , Nathan Harper , Szilard Szoke , Scott Cushing

We introduce the use of two machine learning algorithms to create an empirical model of an experimental apparatus, which is able to reduce the number of measurements necessary for generic optimisation tasks exponentially as compared to…

Quantum Physics · Physics 2020-05-20 Pascal Kobel , Martin Link , Michael Köhl

Entangled photon spectroscopy is a nascent field that has important implications for measurement and imaging across chemical, biology, and materials fields. Entangled photon spectroscopy potentially offers improved spatial and…

Optics · Physics 2021-07-07 Szilard Szoke , Manni He , Bryce P. Hickam , Scott K. Cushing

We design and successfully implement artificial neural networks (ANNs) to detect and classify entanglement for three-qubit systems using limited state features. The overall design principle is a feed forward neural network (FFNN), with the…

Quantum Physics · Physics 2024-11-19 Jorawar Singh , Vaishali Gulati , Kavita Dorai , Arvind

Distributed quantum metrology can enhance the sensitivity for sensing spatially distributed parameters beyond the classical limits. Here we demonstrate distributed quantum phase estimation with discrete variables to achieve Heisenberg limit…

While capable of segregating visual data, humans take time to examine a single piece, let alone thousands or millions of samples. The deep learning models efficiently process sizeable information with the help of modern-day computing.…

Computer Vision and Pattern Recognition · Computer Science 2022-09-28 Alankrit Mishra , Nikhil Raj , Garima Bajwa

In the biomedical environment, experiments assessing dynamic processes are primarily performed by a human acquisition supervisor. Contemporary implementations of such experiments frequently aim to acquire a maximum number of relevant events…

Computer Vision and Pattern Recognition · Computer Science 2023-10-10 Nils Friederich , Angelo Yamachui Sitcheu , Oliver Neumann , Süheyla Eroğlu-Kayıkçı , Roshan Prizak , Lennart Hilbert , Ralf Mikut

Entangled two-photon absorption can enable a linear scaling of fluorescence emission with the excitation power. In comparison to classical two-photon absorption with a quadratic scaling, this can allow fluorescence imaging or…

We discuss how two-photon absorption (TPA) of squeezed and coherent states of light can be detected in measurements of the transmitted light fields. Such measurements typically suffer from competing loss mechanisms such as experimental…

Quantum Physics · Physics 2022-05-24 Shahram Panahiyan , Carlos Sánchez Muñoz , Maria V. Chekhova , Frank Schlawin

We develop an ultrafast frequency-resolved Raman spectroscopy with entangled photons for polyatomic molecules in condensed phases, to probe the electronic and vibrational coherences. Using quantum correlation between the photons, the signal…

Quantum Physics · Physics 2021-06-23 Zhedong Zhang , Tao Peng , Xiaoyu Nie , Girish S. Agarwal , Marlan O. Scully

Entangled photons are a crucial resource for quantum communication and linear optical quantum computation. Unfortunately, the applicability of many photon-based schemes is limited due to the stochastic character of the photon sources.…

Quantum Physics · Physics 2012-02-07 Stefanie Barz , Gunther Cronenberg , Anton Zeilinger , Philip Walther

The Epithelial Dysplasia (ED) is a tissue alteration commonly present in lesions preceding oral cancer, being its presence one of the most important factors in the progression toward carcinoma. This study proposes a method to design a low…

Image and Video Processing · Electrical Eng. & Systems 2022-04-08 Karoline da Rocha , José C. M. Bermudez , Elena R. C. Rivero , Márcio H. Costa