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Optical harmonic generation occurs when high intensity light ($>10^{10}$W/m$^{2}$) interacts with a nonlinear material. Electrical control of the nonlinear optical response enables applications such as gate-tunable switches and frequency…

An original dispersion relation between the stationary coherent nonlinear optical responses by current and polarisation is obtained. The dispersion relation provides a new complimentary tool that can be employed to study light-induced…

Materials Science · Physics 2015-05-19 A. Pishtshev , N. Kristoffel

Optical control offers a compelling route for tailoring material properties on an ultrafast time scale. Ordered states such as charge density waves (CDWs) can be transiently melted by an ultrafast light excitation. This is also the case for…

We dismantle the previously held misconception that it is impossible for bulk rectification mechanisms to induce a net DC electric current when the frequency of the impinging radiation lies within the optical gap of a metal in the limit of…

Mesoscale and Nanoscale Physics · Physics 2023-04-05 Li-kun Shi , Oles Matsyshyn , Justin C. W. Song , Inti Sodemann Villadiego

Rectification is a process that converts electromagnetic fields into a direct current. Such a process underlies a wide range of technologies such as wireless communication, wireless charging, energy harvesting, and infrared detection.…

Materials Science · Physics 2020-03-31 Hiroki Isobe , Su-Yang Xu , Liang Fu

Nonlinear optical response is well studied in the context of semiconductors and has gained a renaissance in studies of topological materials in the recent decade. So far it mainly deals with non-magnetic materials and it is believed to root…

Mesoscale and Nanoscale Physics · Physics 2020-07-31 Tobias Holder , Daniel Kaplan , Binghai Yan

We discuss the possibility of getting rectification operation in graphene nanoribbon (GNR). For a system to be a rectifier, it must be physically asymmetric and we induce the asymmetry in GNR by introducing nanopores. The rectification…

Mesoscale and Nanoscale Physics · Physics 2022-03-23 Joydeep Majhi , Sudin Ganguly , Santanu K. Maiti

Although massless Dirac fermions in graphene constitute a centrosymmetric medium for in-plane excitations, their second-order nonlinear optical response is nonzero if the effects of spatial dispersion are taken into account. Here we present…

Mesoscale and Nanoscale Physics · Physics 2016-12-07 Yongrui Wang , Mikhail Tokman , Alexey Belyanin

Nonlinear nanophotonics leverages engineered nanostructures to funnel light into small volumes and intensify nonlinear optical processes with spectral and spatial control. Due to its intrinsically large and electrically tunable nonlinear…

Centrosymmetric materials with site inversion asymmetries possess hidden spin polarization, which remains challenging to be converted into spin currents because the global inversion symmetry is still conserved. This study demonstrates the…

Materials Science · Physics 2024-05-21 Kexin Wang , Butian Zhang , Chengyu Yan , Luojun Du , Shun Wang

Quantum geometry in centrosymmetric systems has motivated the search for photocurrent responses beyond second order. In particular, electric field-induced nonlinear responses may also enable intrinsic polarization-sensitive optical…

The second order optical response of centrosymmetric materials manifests itself mostly at their surface, being strongly suppressed in their bulk. However, the overall surface response is also suppressed in nanoparticles with a…

Optics · Physics 2021-09-22 Raksha Singla , W. Luis Mochán

The existence of large nonlinear optical coefficients is one of the preconditions for using nonlinear optical materials in nonlinear optical devices. For a crystal, such large coefficients can be achieved by matching photon energies with…

Materials Science · Physics 2018-12-27 J. L. Cheng , J. E. Sipe , S. W. Wu , Chunlei Guo

In a solid, the electronic subsystem can exhibit incipient order with lower point group symmetry than the crystal lattice. External fields that couple to electronic order parameters have rarely been investigated, however, despite their…

Strongly Correlated Electrons · Physics 2024-01-11 Xinshu Zhang , Tyler Carbin , Adrian B. Culver , Kai Du , Kefeng Wang , Sang-Wook Cheong , Rahul Roy , Anshul Kogar

Nonlinear optical responses are often used as a probe for studying electronic properties of materials. For topological materials, studies so far focused on the photogalvanic electric current, which requires breaking inversion symmetry. In…

Materials Science · Physics 2022-03-21 Margarita Davydova , Maksym Serbyn , Hiroaki Ishizuka

Ultrafast optical control of ferroelectricity based on short and intense light can be utilized to achieve accurate manipulations of ferroelectric materials, which may pave a basis for future breakthrough in nonvolatile memories. Here, we…

We show that, under the effect of an external magnetic field, a photogalvanic effect and the generation of second harmonic wave can be induced in inversion-symmetric and time reversal invariant Dirac semimetals. The mechanism responsible of…

Mesoscale and Nanoscale Physics · Physics 2016-12-12 Alberto Cortijo

Graphene is a unique platform for tunable opto-electronic applications thanks to its linear band dispersion, which allows electrical control of resonant light-matter interactions. Tuning the nonlinear optical response of graphene is…

Nonlinear optical processes associated with even-order nonlinear susceptibilities are critical for both classical and quantum technologies. Inversion symmetry, however, prevents nonlinear optical responses mediated by even-order…

Optics · Physics 2022-02-24 Davis M. Welakuh , Prineha Narang

Spin-split superconductors exhibit an electron-hole asymmetric spin-resolved density of states, but the symmetry is restored upon averaging over spin. On the other hand, asymmetry appears again in tunneling junctions of spin-split…

Superconductivity · Physics 2022-05-02 Stefan Ilić , P. Virtanen , T. T. Heikkilä , F. Sebastián Bergeret
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