Related papers: Velocity-comb modulation transfer spectroscopy
We report the measurement of sub-Doppler double-resonance transitions in methane using a 3.3 $\mu$m continuous wave optical parametric oscillator to pump transitions in the fundamental $\nu_3$ band and a 1.67 $\mu$m frequency comb to probe…
Defects in solid-state materials play a central role in determining coherence, stability, and performance in quantum technologies. Although narrowband techniques can probe specific resonances with high precision, a broadband spectroscopic…
We propose a new Fourier-transform spectroscopy technique based on the rotational Doppler effect. The technique offers an application for optical vortex frequency combs, where each frequency component carries a unique amount of orbital…
We study modulation spectroscopy of the potassium D2 transitions at 766.7 nm. The vapour pressure, controlled by heating a commercial reference cell, is optimized using conventional saturated absorption spectroscopy. Subsequent heterodyne…
Dual-comb sources with equally spaced and low phase noise frequency lines are of great importance for high resolution spectroscopy and metrology. In the terahertz frequency range, electrically pumped semiconductor quantum cascade lasers…
A fully stabilized mid-infrared optical frequency comb spanning from 2.9 to 3.4 um is described. The comb is based on half-harmonic generation in a femtosecond optical parametric oscillator, which transfers the high phase coherence of a…
A new method, FM-FTS, combining Frequency Modulation heterodyne laser spectroscopy and Fourier Transform Spectroscopy is presented. It provides simultaneous sensitive measurement of absorption and dispersion profiles with broadband spectral…
Broadband precision spectroscopy is indispensable for providing high fidelity molecular parameters for spectroscopic databases. We have recently shown that mechanical Fourier transform spectrometers based on optical frequency combs can…
Dual-comb spectroscopy (DCS) with few-GHz tooth spacing that provides the optimal trade-off between spectral resolution and refresh rate is a powerful tool for measuring and analyzing rapidly evolving transient events. Despite such an…
Optical frequency combs, coherent light sources that connect optical frequencies with microwave oscillations, have become the enabling tool for precision spectroscopy, optical clockwork and attosecond physics over the past decades. Current…
Dual terahertz (THz) comb spectroscopy is a promising methods for high accuracy, high resolution, and broadband THz spectroscopy because the mode-resolved THz comb spectrum possesses both characteristics of broadband THz radiation and…
Frequency combs have revolutionized optical frequency metrology, allowing one to determine highly accurate transition frequencies of a wealth of molecular species. Despite a recognized scientific interest, these progresses have only…
Dual-comb spectroscopy allows for the rapid, multiplexed acquisition of high-resolution spectra without the need for moving parts or low-resolution dispersive optics. This method of broadband spectroscopy is most often accomplished via…
Vapour cell spectroscopy is an essential technique in many fields; in particular, nearly all atom and ion trapping experiments rely on simultaneous spectroscopy of two atomic transitions, traditionally employing separate apparatus for each…
Dual-comb spectroscopy is a promising method for precise optical spectrum analysis with fast data acquisition speed. However, its implementation and applications are often hindered by the complexity of optical comb systems. Here, as a…
We report a velocity selective bi-polarization spectroscopy (VS-BPS) technique to generate a background-free, dispersion-like reference signal which is tunable over a wide range of frequency. In this technique, a pair of linearly polarized…
Ultra-stable lasers and optical frequency combs have been the enabling technologies for the tremendous progress of precise optical spectroscopy in the last ten years. To improve laser frequency stabilization beyond the thermal-noise…
Chip-scale semiconductor laser frequency combs offer remarkable prospects for compact and power-efficient optical sensors. For the laser to be suitable for typical comb applications, its degree of coherence must first be assessed from a…
A phase-stabilized femtosecond laser comb is directly used for high-resolution spectroscopy and absolute optical frequency measurements of one- and two-photon transitions in laser-cooled \rb atoms. Absolute atomic transition frequencies,…
Advances in high-resolution laser spectroscopy have enabled many scientific breakthroughs in physics, chemistry, biology and astronomy. Optical frequency combs have pushed measurement limits with ultrahigh-frequency accuracy and…