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Evolution of magnetism in single crystals of the van der Waals compound VI3 in external pressure up to 7.3 GPa studied by measuring magnetization and ac magnetic susceptibility is reported. Four magnetic phase transitions, at T1 = 54.5 K,…

A complex interplay of different energy scales involving Coulomb repulsion, spin-orbit coupling and Hund's coupling energy in two-dimensional (2D) van der Waals (vdW) material produces novel emerging physical state. For instance,…

The van der Waals class of materials offer an approach to two-dimensional magnetism as their spin fluctuations can be tuned upon exfoliation of layers. Moreover, it has recently been shown that spin-lattice coupling and long-range magnetic…

Two-dimensional van der Waals ferromagnet Fe$_3$GeTe$_2$ (FGT) holds a great potential for applications in spintronic devices, due to its high Curie temperature, easy tunability, and excellent structural stability in air. Theoretical…

Materials Science · Physics 2025-04-03 Yonglin Wang , Xu-Tao Zeng , Bo Li , Cheng Su , Takanori Hattori , Xian-Lei Sheng , Wentao Jin

Van der Waals magnetic materials are an ideal platform to study low-dimensional magnetism. Opposed to other members of this family, the magnetic semiconductor CrSBr is highly resistant to degradation in air, which, besides its exceptional…

Since the celebrated discovery of graphene, the family of two-dimensional (2D) materials has grown to encompass a broad range of electronic properties. Recent additions include spin-valley coupled semiconductors, Ising superconductors that…

The recent experimental discovery of intrinsic ferromagnetism in single-layer CrI3 opens a new avenue to low-dimensional spintronics. However, the low Curie temperature Tc=45 K is still a large obstacle to its realistic device application.…

Materials Science · Physics 2019-06-26 Hongxing Li , Yuan-Kai Xu , Kang Lai , Wei-Bing Zhang

The magnetic structure and phase diagram of the layered ferromagnetic compound Fe$_3$GeTe$_2$ has been investigated by a combination of synthesis, x-ray and neutron diffraction, high resolution microscopy, and magnetization measurements.…

Strongly Correlated Electrons · Physics 2016-01-13 Andrew F. May , Stuart Calder , Claudia Cantoni , Huibo Cao , Michael A. McGuire

Recent experiments on van der Waals antiferrmagnets such as CrI3, CrCl3 and MnPS3 have shown that using atomically thin layers as tunnel barriers and measuring the temperature ($T$) and magnetic field ($H$) dependence of the conductance…

Recently discovered ferromagnetism of the layered van der Waals material VI$_3$ attracts much research attention. Despite substantial progress,in the following important aspects no consensus has been reached: (i) a possible deviation of the…

Materials Science · Physics 2021-07-07 L. M. Sandratskii , K. Carva

We report synthesis of hexagonal LaVxCr1-xGe3 (x = 0-0.21, 1.00) single crystals, and present a systematic study of this series by measurements of temperature and field dependent magnetic susceptibility, magnetization, resistivity, and…

Strongly Correlated Electrons · Physics 2015-06-16 Xiao Lin , Valentin Taufour , Sergey L. Bud'ko , Paul C. Canfield

Magnetoelastic coupling and uniaxial pressure dependencies of the ferromagnetic ordering temperature in the quasi-two-dimensional layered van-der-Waals material CrI$_3$ are experimentally studied and quantified by high-resolution…

Strongly Correlated Electrons · Physics 2022-02-23 J. Arneth , M. Jonak , S. Spachmann , M. Abdel-Hafiez , Y. O. Kvashnin , R. Klingeler

The unexpected discovery of intrinsic ferromagnetism in layered van der Waals materials has sparked interest in both their fundamental properties and their potential for novel applications. Recent studies suggest near room-temperature…

We present a combined study of zero-field $^{51}$V and $^{127}$I NMR at ambient pressure and specific heat and magnetization measurements under pressure up to 2.08 GPa on bulk single crystals of the van-der-Waals ferromagnet VI$_3$. At…

Strongly Correlated Electrons · Physics 2019-11-21 Elena Gati , Yuji Inagaki , Tai Kong , Robert J. Cava , Yuji Furukawa , Paul C. Canfield , Sergey L. Bud'ko

Ferromagnetism in two-dimensional materials presents a promising platform for the development of ultrathin spintronic devices with advanced functionalities. Recently discovered ferromagnetic van der Waals crystals such as CrI$_{3}$, readily…

We studied magnetic states and phase transitions in the van der Waals antiferromagnet VBr3 by specific heat and magnetization measurements of single crystals in high magnetic fields and by ab initio density functional theory calculations…

To explore the possibility of quantum phase transitions and even quantum criticality in LaCrSb$_3$ based compounds, we performed measurements under pressure as well as a vanadium substitution study. The Curie temperature of LaCrSb$_3$ was…

Materials Science · Physics 2015-06-17 Xiao Lin , Valentin Taufour , Sergey L. Bud'ko , Paul C. Canfield

Identifying intrinsic low-dimensional ferromagnets with high transition temperature and electrically tunable magnetism is crucial for the development of miniaturized spintronics and magnetoelectrics. Recently long-range 2D ferromagnetism…

Materials Science · Physics 2020-08-27 Hua Wang , Jingshan Qi , Xiaofeng Qian

Manipulation of long-range order in two-dimensional (2D) van der Waals (vdW) magnetic materials (e.g., CrI$_3$, CrSiTe$_3$ etc.), exfoliated in few-atomic layer, can be achieved via application of electric field, mechanical-constraint,…

Layered van der Waals ferromagnets, which preserve their magnetic properties down to exfoliated monolayers, are fueling an abundance of fundamental research and nanoscale device demonstration. CrGeTe$_3$ is a prime example for this class of…

Strongly Correlated Electrons · Physics 2023-09-27 Han-Xiang Xu , Makoto Shimizu , Daniel Guterding , Junya Otsuki , Harald O. Jeschke
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