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The enigmatic coupling between electronic and magnetic phenomena was one of the riddles propelling the development of modern electromagnetism. Today, the fully controlled electric field evolution of ultrashort laser pulses permits the…

The inhomogeneity of an electron spin ensemble as well as fluctuating environment acting upon individual spins drastically shorten the spin coherence time $T_2$ and hinder coherent spin manipulation. We show that this problem can be solved…

Mesoscale and Nanoscale Physics · Physics 2021-10-13 V. V. Belykh , A. R. Korotneva , D. R. Yakovlev

By comparing femtosecond laser pulse induced ferro- and antiferromagnetic dynamics in one and the same material - metallic dysprosium - we show both to behave fundamentally different. Antiferromagnetic order is considerably faster and much…

Reducing energy dissipation while increasing speed in computation and memory is a long-standing challenge for spintronics research. In the last 20 years, femtosecond lasers have emerged as a tool to control the magnetization in specific…

Understanding how fast short-range interactions build up long-range order is one of the most intriguing topics in condensed matter physics. FeRh is a test specimen for studying this problem in magnetism, where the microscopic spin-spin…

Fast and dynamical control of quantum phases is highly desired in the application of quantum phenomena in devices. On the experimental side, ultrafast laser pulses provide an ideal platform to induce femtosecond dynamics in a variety of…

Strongly Correlated Electrons · Physics 2020-10-21 Benedikt Fauseweh , Jian-Xin Zhu

Efficient and fast manipulation of antiferromagnets has to date remained a challenging task, hindering their application in spintronic devices. For ultrafast operation of such devices, it is highly desirable to be able to control the…

Materials Science · Physics 2023-05-31 Markus Weißenhofer , Francesco Foggetti , Ulrich Nowak , Peter M. Oppeneer

Lightwave quantum electronics utilizes the oscillating carrier wave of intense laser fields to control quantum materials properties. Using quantum kinetic equations of motion, we describe lightwave-driven nonlinear quantum transport of…

Strongly Correlated Electrons · Physics 2020-06-15 P. C. Lingos , M. D. Kapetanakis , J. Wang , I. E. Perakis

The diverse nodal spin structures in d/g/i-wave altermagnets (AM) may cause distinct light-induced spin responses yet remain poorly understood. Using time-dependent density functional theory (TDDFT), we reveal that laser induced ultrafast…

Materials Science · Physics 2026-02-17 Zhaobo Zhou , Sangeeta Sharma , Junjie He

Femtosecond (fs) coherent control of collective order parameters is important for non--equilibrium phase dynamics in correlated materials. Here we propose a possible scheme for fs control of a ferromagnetic order parameter based on…

Strongly Correlated Electrons · Physics 2015-05-27 P. C. Lingos , J. Wang , I. E. Perakis

Laser radiation incident on a ferromagnetic sample produces excited electrons and currents whose spin polarization must not be aligned with the magnetization -- an effect due to spin-orbit coupling that is ubiquitous in spin- and…

Materials Science · Physics 2023-11-03 Oliver Busch , Franziska Ziolkowski , Ingrid Mertig , Jürgen Henk

Employing electron spin instead of charge to develop spintronic devices holds the merits of low-power consumption in information technologies. Meanwhile, the demand for increasing speed in spintronics beyond current CMOS technology has…

Using density matrix equations of motion, we predict a femtosecond collective spin tilt triggered by nonlinear, near--ultraviolet ($\sim$3eV), coherent photoexcitation of (Ga,Mn)As ferromagnetic semiconductors with linearly polarized light.…

Strongly Correlated Electrons · Physics 2009-08-06 M. D. Kapetanakis , I. E. Perakis , K. J. Wickey , C. Piermarocchi , J. Wang

The microscopic origin of laser-induced ultrafast demagnetization remains an open question, to which the non-thermal electronic distribution plays a vital role at the initial stage. Herein, we investigate the connection between the…

Materials Science · Physics 2025-12-25 Yu-Hui Song , Huan-Cheng Yang , Kai Liu , Zhong-Yi Lu

Ultrafast non-thermal manipulation of magnetization by light relies on either indirect coupling of the electric field component of the light with spins via spin-orbit interaction or direct coupling between the magnetic field component and…

Laser-induced femtosecond demagnetization, femtomagnetism, offers a potential route to develop faster magnetic storage devices. It is generally believed that the traditional spin-wave theory, which is developed for thermally driven slow…

Materials Science · Physics 2019-12-05 G. P. Zhang , M. Murakami , Y. H. Bai , Thomas F. George , X. S. Wu

Inspired by a recent pressure experiment in fcc Ni, we propose a simple method to use pressure to investigate the laser-induced femtosecond magnetism. Since the pressure effect on the electronic and magnetic properties can be well…

Materials Science · Physics 2015-12-15 M. S. Si , J. Y. Li , D. S. Xue , G. P. Zhang

Femtosecond laser pulses can induce ultrafast demagnetization as well as generate bursts of hot electron spin currents. In trilayer spin valves consisting of two metallic ferromagnetic layers separated by a nonmagnetic one, hot electron…

Materials Science · Physics 2020-05-27 Ulrike Ritzmann , Pavel Baláž , Pablo Maldonado , Karel Carva , Peter M. Oppeneer

When a laser pulse excites a ferromagnet, its spin undergoes a dramatic change. The initial demagnetization process is very fast. Experimentally, it is found that the demagnetization time is related to the spin moment in the sample. In this…

Materials Science · Physics 2016-11-11 G. P. Zhang , M. S. Si , Thomas F. George

Laser-induced terahertz spin transport (TST) and ultrafast demagnetization (UDM) are central but so far disconnected phenomena in femtomagnetism and terahertz spintronics. Here, we use broadband terahertz emission spectroscopy to reliably…

Mesoscale and Nanoscale Physics · Physics 2021-05-27 R. Rouzegar , L. Brandt , L. Nadvornik , D. A. Reiss , A. L. Chekhov , O. Gueckstock , C. In , M. Wolf , T. S. Seifert , P. W. Brouwer , G. Woltersdorf , T. Kampfrath