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Grain boundary engineering via dopant segregation can dramatically change the properties of a material. For metallic systems, most current studies concerning interfacial segregation and subsequent transitions of grain boundary structure are…

Materials Science · Physics 2018-12-26 Yang Hu , Timothy J. Rupert

Tailoring the nanoscale distribution of chemical species at grain boundaries is a powerful method to dramatically influence the properties of polycrystalline materials. However, classical approaches to the problem have tacitly assumed that…

Materials Science · Physics 2024-11-11 Malik Wagih , Yannick Naunheim , Tianjiao Lei , Christopher A. Schuh

Alloying a material and hence segregating solutes to grain boundaries is one way to tailor a material to the demands of its application. Direct observation of solute segregation is necessary to understand how the interfacial properties are…

Materials Science · Physics 2023-05-03 Lena Langenohl , Tobias Brink , Gunther Richter , Gerhard Dehm , Christian H. Liebscher

It is believed that grain boundary segregation of light interstitials can serve as possible mechanism of thermal stability in commercially pure nanostructured titanium alloys. In this paper, using first-principles calculations, we show that…

Materials Science · Physics 2015-06-15 D. A. Aksyonov , A. G. Lipnitskii , Yu. R. Kolobov

In alloys, solute segregation at grain boundaries is classically attributed to three driving forces: a high solution enthalpy, a high size mismatch, and a high difference in interfacial energy. These effects are generally cast into a single…

Materials Science · Physics 2024-01-23 Malik Wagih , Yannick Naunheim , Tianjiao Lei , Christopher A. Schuh

Grain boundaries (GBs) trigger structure-specific chemical segregation of solute atoms. According to the three-dimensional (3D) topology of grains, GBs - although defined as planar defects - cannot be free of curvature. This implies…

This paper studies how solute segregation and its relationship to grain boundary energy in binary alloys is captured in the phase field crystal (PFC) formalism, a continuum method that incorporates atomic scale elasto-plastic effects on…

Materials Science · Physics 2013-04-10 Jonathan Stolle , Nikolas Provatas

Solute segregation in alloys is a key phenomenon which affects various material characteristics such as embrittlement, grain growth and precipitation kinetics. In this work, the segregation energies of Y, Zr, and Nb to a \textgreek{S}5…

Materials Science · Physics 2025-03-06 Hariharan Umashankar , Daniel Scheiber , Vsevolod I. Razumovskiy , Matthias Militzer

Grain Boundary (GB) deformation mechanisms such as Sliding (GBS) and Opening (GBO) are prevalent in alloys at high homologous temperatures but are hard to capture quantitatively. We propose an automated procedure to quantify 3D GB…

Materials Science · Physics 2025-07-24 C. J. A. Mornout , G. Slokker , T. Vermeij , D. König , J. P. M. Hoefnagels

Grain boundaries (GBs) and interfaces in polycrystalline materials are significant research subjects in the field of materials science. Despite a more than 50-year history of their study, there are still many open questions. The main…

Materials Science · Physics 2021-06-28 Arslan B. Mazitov , Artem R. Oganov

Grain boundary (GB) migration plays a crucial role in the thermal and mechanical responses of polycrystalline materials, particularly in ultrafine-grained and nano-grained materials exhibiting grain size-dependent properties. This study…

Materials Science · Physics 2024-04-08 Liang Yang , Xinyuan Song , Tingting Yu , Dahai Liu , Chuang Deng

In this paper, the Fe-20Ni-25Cr alloy that is used for fuel cladding or pressure vessels with various grain boundaries (GBs) was investigated by employing molecular dynamics simulations. The bi-crystals comprised of {\Sigma}3(111),…

Materials Science · Physics 2021-02-26 Zhijia Liu , Zehua Feng , Heran Wang , Yunpeng Zhang , Zheng Chen , Fanchao Meng , Jing Zhang

A systematics of grain boundary (GB) segregation transitions and critical phenomena has been derived to expand the classical GB segregation theory. Using twist GBs as an example, this study uncovers when GB layering vs. prewetting…

Materials Science · Physics 2022-01-20 Naixie Zhou , Chongze Hu , Jian Luo

We use atomistic simulations to investigate grain boundary (GB) phase transitions in el- emental body-centered cubic (bcc) metal tungsten. Motivated by recent modeling study of grain boundary phase transitions in [100] symmetric tilt…

Materials Science · Physics 2018-04-17 Timofey Frolov , Qiang Zhu , Tomas Oppelstrup , Jaime Marian , Robert E. Rudd

We derive a theory that describes homogeneous nucleation of grain boundary (GB) phases. Our analysis takes account of the energy resulting from the GB phase junction, the line defect separating two different GB structures, which is…

Materials Science · Physics 2022-02-02 Ian S. Winter , Robert E. Rudd , Tomas Oppelstrup , Timofey Frolov

There are still debates regarding the mechanisms that lead to hot cracking in parts build by additive manufacturing (AM) of non-weldable Ni-based superalloys. This lack of in-depth understanding of the root causes of hot cracking is an…

The interfacial structure of a silicon grain boundary (Si-GB) plays a decisive role on its chemical functionalization and has implications in diverse physical-chemical properties of the material. Therefore, GB interface is particularly…

Materials Science · Physics 2023-01-02 Rita Maji , Eleonora Luppi , Elena Degoli

Segregation to grain boundaries affects their cohesion, corrosion and embrittlement and plays a critical role in heterogeneous nucleation. In order to quantitatively study segregation and phase separation at grain boundaries, we derive a…

At very fine grain sizes, grain boundary segregation can deviate from conventional behavior due to triple junction effects. While this issue has been addressed in prior work for substitutional alloys, here we develop a framework that…

Materials Science · Physics 2024-11-28 Nutth Tuchinda , Malik Wagih , Christopher A. Schuh

Molecular dynamics simulations of 50 Fe grain boundaries were used to understand their interaction with vacancies and self-interstitial atoms at all atomic positions within 20 Angstroms of the boundary, which is important for designing…

Mesoscale and Nanoscale Physics · Physics 2013-09-02 M. A. Tschopp , M. F. Horstemeyer , F. Gao , X. Sun , M. Khaleel