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Ultrafast electron-photon spectroscopy in electron microscopes commonly requires ultrafast laser setups. Photoemission from an engineered electron source is used to generate pulsed electrons, interacting with a sample that is excited by the…
Attosecond pulses created by high-order harmonic generation in gases often exhibit strong chromatic aberrations, arising from the broad bandwidth and wavelength-dependent nonlinear light-matter interaction. When the driving laser intensity…
Ultrafast electron microscopy provides a movie-like access to structural dynamics of materials in space and time, but fundamental atomic motions or electron dynamics are, so far, too quick to be resolved. Here we report the all-optical…
Controlled interaction of laser light with electron beams is fundamental for ultrafast electron microscopy and electron-based quantum optics, yet their direct coupling is forbidden in free space. Here we use longitudinally polarized light…
We propose a scheme for constructing a phase plate for use in an ultrafast Zernike-type phase contrast electron microscope, based on the interaction of the electron beam with a strongly focused, high-power femtosecond laser pulse and a…
Recent progress in phase modulation using nanofabricated electron holograms has demonstrated how the phase of an electron beam can be controlled. In this paper, we apply this concept to the correction of spherical aberration in a scanning…
A model for a new electron vortex beam production method is proposed and experimentally demonstrated. The technique calls on the controlled manipulation of the degrees of freedom of the lens aberrations to achieve a helical phase front.…
Digital imaging sensor technology has continued to outpace development in optical technology in modern imaging systems. The resulting quality loss attributable to lateral chromatic aberration is becoming increasingly significant as sensor…
We develop photoelectron interferometry based on laser-assisted extreme ultraviolet ionization for flexible and robust control of photoelectron circular dichroism in randomly oriented chiral molecules. A comb of XUV photons ionizes a sample…
Coherent control of ultrafast quantum phenomena benefits from pulse-shaping capabilities allowing to modulate the envelope and instantaneous phase of optical fields on femtosecond time scales. While such control is available for optical…
Ultrafast electron diffraction (UED) is a powerful method for studying time-resolved structural changes. Currently, space charge induced temporal broadening prevents obtaining high brightness electron pulses with sub-100 fs durations…
The key to optimizing spatial resolution in a state-of-the-art scanning transmission electron microscope is the ability to precisely measure and correct for electron optical aberrations of the probe-forming lenses. Several diagnostic…
The ability to modulate free electrons with light has emerged as a powerful tool to produce attosecond electron wavepackets. However, research has so far aimed at the manipulation of the longitudinal wave function component, while the…
Here, we demonstrate the radiative polarization of high-energy electron beams in collisions with ultrashort pulsed bi-chromatic laser fields. Employing a Boltzmann kinetic approach for the electron distribution allows us to simulate the…
Precise alignment of the electron beam is critical for successful application of scanning transmission electron microscopes (STEM) to understanding materials at atomic level. Despite the success of aberration correctors, aberration…
Plasmonics, the science and technology of the interaction of light with metallic objects, is fundamentally changing the way we can detect, generate and manipulate light. Although the field is progressing swiftly, thanks to the availability…
High-throughput 2D and 3D scanning electron microscopy, which relies on automation and dependable control algorithms, requires high image quality with minimal human intervention. Classical focus and astigmatism correction algorithms attempt…
The polarization of light is critical in various applications, including quantum communication, where the photon polarization encoding a qubit can undergo uncontrolled changes when transmitted through optical fibers. Bends in the fiber,…
Dispersion decomposes compound light into monochromatic components at different spatial locations, which needs to be eliminated in imaging but utilized in spectral detection. Metasurfaces provide a unique path to modulate the dispersion…
A theoretical study of laser and plasma based electron acceleration is presented. An effective model has been used, in which the presence of an underdense plasma has been taken account via its index of refraction $n_{m}$. In the confines of…