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Plexciton is the formation of new hybridized energy states originated from the coupling between plasmon and exciton. To reveal the optical properties of both exciton and plexciton, we develop a classic oscillator model to describe the…

Optics · Physics 2022-07-12 Yuqing Cheng , Mengtao Sun

We have analyzed a dissipative two level quantum system (TLS) which is continuously and simultaneously irradiated by a high and low frequency excitation. The interaction of the TLS with a high frequency excitation is considered in the frame…

Soft Condensed Matter · Physics 2007-09-30 Ya. S. Greenberg

We consider the relaxation of an excited two-level system (TLS) positioned near a spherical plasmonic nanoparticle (NP). The transition frequency of the TLS is assumed to coincide with the frequency of the condensation point of NP plasmonic…

Mesoscale and Nanoscale Physics · Physics 2015-06-18 E. S. Andrianov , A. A. Pukhov , A. P. Vinogradov , A. V. Dorofeenko , A. A. Lisyansky

We extend the model of exciton-plasmon materials to include a ro-vibrational structure of molecules using wave-packet propagations on electronic potential energy surfaces. The new model replaces conventional two-level emitters with more…

Mesoscale and Nanoscale Physics · Physics 2017-08-18 Maxim Sukharev , Eric Charron

Atomic sized two-level systems (TLSs) in amorphous dielectrics are known as a major source of loss in superconducting devices. In addition, individual TLS are known to induce large frequency shifts due to strong coupling to the devices.…

Mesoscale and Nanoscale Physics · Physics 2017-07-05 Naftali Kirsh , Elisha Svetitsky , Alexander L. Burin , Moshe Schechter , Nadav Katz

The common model to describe exciton-plasmon interaction phenomenologically is the coupled oscillator model. Originally developed for atomic systems rather than solid-state matter, this model treats both excitons and plasmons as single…

Mesoscale and Nanoscale Physics · Physics 2024-10-23 Lara Greten , Robert Salzwedel , Diana Schutsch , Andreas Knorr

We consider a hybrid plasmon-exciton system comprised of a resonant molecular subsystem and three Au wires supporting a dipole mode which can be coupled to a dark mode in controllable fashion by variation of a symmetry parameter. The…

Optics · Physics 2015-03-25 Maxim Sukharev , Paul N. Day , Ruth Pachter

We study exciton-plasmon coupling in two-dimensional semiconductors coupled with Ag plasmonic lattices via angle-resolved reflectance spectroscopy and by solving the equations of motion (EOMs) in a coupled oscillator model accounting for…

The manipulation of coupled quantum excitations is of fundamental importance in realizing novel photonic and optoelectronic devices. We use electroluminescence to probe plasmon-exciton coupling in hybrid structures consisting of a nanoscale…

The near-field interaction due to a strong electromagnetic field induced by resonant localized plasmons can result in a strong coupling of excitonic states or formation of hybrid exciton-plasmon modes in quantum confined structures. This…

Mesoscale and Nanoscale Physics · Physics 2019-04-01 Yuba Poudel , Gary N. Lim , Mojtaba Moazzezi , Zachariah Hennighausen , Yuri Rostovtsev , Francis DSouza , Swastik Kar , Arup Neogi

The multi-scale computational method of combining first-principles calculation and finite element electromagnetic simulations is used to study plasmon-enhanced interlayer charge transfer (ICT) exciton of 2D lateral and van der Waals…

Optics · Physics 2020-03-30 Xijiao Mu , Mengtao Sun

Exciton plasmon polaritons have gained increasing interests over recent years due to their versatile properties emerging by the underlying light-matter coupling and making them potential candidates for new photonic applications. We have…

Two-dimensional semiconductors host excitons with very large oscillator strengths and binding energies due to significantly reduced carrier screening. Two-dimensional semiconductors integrated with optical cavities are emerging as a…

Monolayers of ReS2 were grown by a chemical vapor deposition technique on SiO2/Si substrates and investigated at room temperature by using micro-Raman, micro-photoluminescence (PL) and absorbance spectroscopies. The Raman scattering…

Materials Science · Physics 2024-04-23 Solomon Ojo , Juwon Onasanya , Morad Benamara , Bothina Hamad , M. O. Manasreh

Plasmon-exciton polaritons provide exciting possibilities to control light-matter interactions at the nanoscale by enabling closer investigation of quantum optical effects and facilitating novel technologies based, for instance, on…

Mesoscale and Nanoscale Physics · Physics 2020-02-25 Grigorios P. Zouros , Georgios D. Kolezas , N. Asger Mortensen , Christos Tserkezis

In quantum physics, two prototypical model systems stand out due to their wide range of applications. These are the two-level system (TLS) and the harmonic oscillator. The former is often an ideal model for confined charge or spin systems…

Mesoscale and Nanoscale Physics · Physics 2020-03-04 Thilo Hahn , Daniel Wigger , Tilmann Kuhn

Hybrid systems of excitons strongly coupled to localized surface plasmons supported by metallic nanoparticles define a new approach to control light-matter interactions. Here, we report exciton-plasmon coupling in two-dimensional (2D)…

Coupling molecular transition dipole moments to surface-plasmon polaritons (SPPs) results in the formation of new optical quasiparticles, i.e., plexcitons. Mixing the specific properties of matter excitations and light modes has proven to…

We simulate the near-field effects of strong coupling between molecular excitons and localized surface plasmons, supported by aluminum nanodisks. The simulations are done using a simple model of a two-level system, implemented in a…

Mesoscale and Nanoscale Physics · Physics 2020-01-29 Nadav Fain , Tal Ellenbogen , Tal Schwartz

Recent years have seen a growing interest in strong coupling between plasmons and excitons, as a way to generate new quantum optical testbeds and influence chemical dynamics and reactivity. Strong coupling to bright plasmonic modes has been…

Mesoscale and Nanoscale Physics · Physics 2020-02-11 Ora Bitton , Satyendra Nath Gupta , Lothar Houben , Michal Kvapil , Vlastimil Křápek , Tomas Šikola , Gilad Haran
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