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We have developed and implemented a self-consistent density functional method using standard norm-conserving pseudopotentials and a flexible, numerical LCAO basis set, which includes multiple-zeta and polarization orbitals. Exchange and…

The temperature scaling of the micromagnetic Dzyaloshinsky-Moriya exchange interaction is calculated for the whole range of temperature. We use Green's function theory to derive the finite-temperature spin wave spectrum of ferromagnetic…

Other Condensed Matter · Physics 2017-10-04 Levente Rózsa , Unai Atxitia , Ulrich Nowak

Density functional theory (DFT) provides a theoretical framework for efficient and fairly accurate calculations of the electronic structure of molecules and crystals. The main features of density functional theory are described and DFT…

Chemical Physics · Physics 2012-06-12 Hauke Paulsen , Alfred Xaver Trautwein

We propose a method for the evaluation of magnetic exchange couplings based on noncollinear spin-density functional calculations. The method employs the second derivative of the total Kohn-Sham energy of a single reference state, in…

Materials Science · Physics 2009-11-13 Juan E. Peralta , Veronica Barone

We present \texttt{ESpinS} (Esfahan Spin Simulation) package to evaluate the thermodynamic properties of spin systems described by a spin model Hamiltonian. In addition to the Heisenberg exchange term, the spin Hamiltonian can contain…

Computational Physics · Physics 2021-08-17 Nafise Rezaei , Mojtaba Alaei , Hadi Akbarzadeh

The method for calculating the isotropic exchange interactions in the paramagnetic phase is proposed. It is based on the mapping of the high-temperature expansion of the spin-spin correlation function calculated for the Heisenberg model…

Strongly Correlated Electrons · Physics 2016-11-09 O. M. Sotnikov , V. V. Mazurenko

An efficient method to compute magnetic exchange interactions in systems with strong correlations is introduced. It is based on a magnetic force theorem which evaluates linear response due to rotations of magnetic moments and uses a novel…

Strongly Correlated Electrons · Physics 2007-05-23 Xiangang Wan , Quan Yin , Sergej Y. Savrasov

A new formalism and computer code, ASTRA (AttoSecond TRAnsitions), has been developed to treat the interactions of short, intense radiation with molecules. The formalism makes extensive use of transition density matrices, computed using a…

Current-spin density functional theory (CSDFT) provides a framework to describe interacting many-electron systems in a magnetic field which couples to both spin- and orbital-degrees of freedom. Unlike in usual (spin-) density functional…

Materials Science · Physics 2015-06-25 S. Pittalis , S. Kurth , N. Helbig , E. K. U. Gross

An approach to compute exchange parameters of the Heisenberg model in plane-wave-based methods is presented. This calculation scheme is based on the Green's function method and Wannier function projection technique. It was implemented in…

Strongly Correlated Electrons · Physics 2015-06-09 Dm. M. Korotin , V. V. Mazurenko , V. I. Anisimov , S. V. Streltsov

Spin-wave excitations are fundamental to understanding the behavior of magnetic materials and hold promise for future information and communication technologies. Yet, modeling these accurately in transition-metal compounds remains…

Total energies of crystal structures can be calculated to high precision using quantum-based density functional theory (DFT) methods, but the calculations can be time consuming and scale badly with system size. Cluster expansions of total…

Materials Science · Physics 2015-12-31 Qin Gao , Sanxi Yao , Jeff Schneider , Michael Widom

Magnetism of transition metal (TM) oxides is usually described in terms of the Heisenberg model, with orientation-independent interactions between the spins. However, the applicability of such a model is not fully justified for TM oxides…

Strongly Correlated Electrons · Physics 2017-08-24 R. Logemann , A. N. Rudenko , M. I. Katsnelson , A. Kirilyuk

Magneto-oscillations in two-dimensional systems with spin-orbit interaction are typically characterized by fast Shubnikov-de~Haas (SdH) oscillations and slower spin-orbit-related beatings. The characterization of the full SdH oscillatory…

Mesoscale and Nanoscale Physics · Physics 2024-05-24 Hamed Gramizadeh , Denis R. Candido , Andrei Manolescu , J. Carlos Egues , Sigurdur I. Erlingsson

This study investigates the predictive capabilities of common DFT methods (GGA, GGA+$U$, and GGA+$U$+$V$) for determining the transition temperature of antiferromagnetic insulators. We utilize a dataset of 29 compounds and derive Heisenberg…

Computational Physics · Physics 2024-03-19 Zahra Mosleh , Mojtaba Alaei

The exchange energy of an arbitrary collinear-spin many-body system in an external magnetic field is a functional of the spin-resolved charge and current densities, $E_x[n_{\uparrow},n_{\downarrow},j_{\uparrow},j_{\downarrow}]$. Within the…

Materials Science · Physics 2015-05-13 J. M. Morbec , K. Capelle

The energy density method is generalized to include spin polarization with the full formalism derived based on spin-density functional theory, which aims at decomposing the total energy into well-defined atomic energies. The method involves…

Materials Science · Physics 2026-04-27 Yang Dan , Dallas R. Trinkle

Large scale calculations for the energy levels, transition rates, oscillator strengths, hyperfine interaction constants, Land\'e g$_J$ factors and isotope shifts have been performed for $1s^2$ and $1snl \: (n=2-8 $ and $l \leq (n-1) )$…

Atomic Physics · Physics 2024-01-15 Shikha Rathi , Lalita Sharma

Proposals for novel spin-orbitronic logic1 and memory devices2 are often predicated on assumptions as to how materials with large spin-orbit coupling interact with ferromagnets when in contact. Such interactions give rise to a host of novel…

Mesoscale and Nanoscale Physics · Physics 2015-08-05 Hans T. Nembach , Justin M. Shaw , Mathias Weiler , Emilie Jué , Thomas J. Silva

We formulate a low-energy theory for the magnetic interactions between electrons in the multi-band Hubbard model under non-equilibrium conditions determined by an external time-dependent electric field which simulates laser-induced spin…

Strongly Correlated Electrons · Physics 2013-04-11 Andrea Secchi , Sergei Brener , Alexander I. Lichtenstein , Mikhail I. Katsnelson