Related papers: Chemistry in a Cryogenic Buffer Gas Cell
Barium monohydride (BaH) is an attractive candidate for extending laser cooling and trapping techniques to diatomic hydrides. The apparatus and high-resolution optical spectroscopy presented here demonstrate progress toward this goal. A…
We produce cold and dense clouds of atomic ions (Ca$^+$, Dy$^+$) by laser ablation of metal targets and cryogenic buffer gas cooling of the resulting plasma. We measure the temperature and density of the ion clouds using laser absorption…
We study the properties of a cryogenic buffer gas source that uses a low temperature two-stage buffer gas cell to produce very slow beams of ytterbium monofluoride molecules. The molecules are produced by laser ablation inside the cell and…
We describe an instrument which can be used to analyze complex chemical mixtures at high resolution and high sensitivity. Molecules are collisionally cooled with helium gas at cryogenic temperatures (~ 4-7 K), and subsequently detected…
Cryogenic buffer gas beams are important sources of cold molecules. In this work we explore the use of a converging-diverging nozzle with a buffer-gas beam. We find that, under appropriate circumstances, the use of a nozzle can produce a…
We demonstrate that buffer-gas cooling combined with laser ablation can be used to create coherent optical media with high optical depth and low Doppler broadening that offers metastable states with low collisional and motional decoherence.…
We describe the combination of buffer-gas cooling with electrostatic velocity filtering to produce a high-flux continuous guided beam of internally cold and slow polar molecules. In a previous paper (L.D. van Buuren et al.,…
Beams of atoms and molecules are stalwart tools for spectroscopy and studies of collisional processes. The supersonic expansion technique can create cold beams of many species of atoms and molecules. However, the resulting beam is typically…
Context. In dense clouds, hydrogenation reactions on icy dust grains are key in the formation of molecules, like formaldehyde, methanol, and complex organic molecules (COMs). These species form through the sequential hydrogenation of CO…
We demonstrate production of cold atomic strontium (Sr) and strontium-containing molecules (SrOH) in a cryogenic buffer gas beam source via direct heating of strontium oxide (SrO) with 30 mJ laser pulses several milliseconds long.…
The development of cryogenic calorimeters was originally motivated by the fact that very low energy thresholds and excellent energy resolutions can be achieved by these devices. Cryogenic devices are widely used in double beta decay…
We describe experiments on the laser cooling of both helium-rubidium and argon-rubidium gas mixtures by collisional redistribution of radiation. Frequent alkali-noble gas collisions in the ultradense gas, with typically 200\,bar of noble…
The cryogenic buffer gas beam (CBGB) is an important tool in the study of cold and ultracold molecules. While there are known techniques to enhance desired beam properties, such as high flux, low velocity, or reduced divergence, they have…
We reported a detailed experimental study of the cold collision of Barium monofluoride (BaF) with buffer gas and the high-resolution spectroscopy relevant with direct laser cooling. BaF molecules are efficiently produced with laser ablation…
We have investigated the chemistry of ${\rm C + H_3^+}$ forming CH$^+$, CH$_2^+$, and CH$_3^+$. These reactions are believed to be some of the key gas-phase astrochemical processes initiating the formation of organic molecules in molecular…
A recent expansion of cold and ultracold molecule applications has led to renewed focus on molecular species preparation under ultrahigh vacuum conditions. Meanwhile, molecular beams have been used to study gas phase chemical reactions for…
Cryogenic buffer-gas beam sources are capable of producing intense beams of a wide variety of molecules, and have a number of advantages over traditional supersonic expansion sources. In this work, we report on a neon matrix isolation study…
Cryogenic buffer-gas beams are a promising method for producing bright sources of cold molecular radicals for cold collision and chemical reaction experiments. In order to use these beams in studies of reactions with controlled collision…
We investigate the formation of molecular hydrogen (H_2) in a primordial H+He gas cloud irradiated by a power-law UV flux. We find that at high densities (>1 cm^{-3}) and low temperatures (<10^4 K), the background radiation enhances the…
It has recently become possible to form molecules in ultracold gases of trapped alkali metal atoms. Once formed, the molecules may undergo elastic, inelastic and reactive collisions. Inelastic and reactive collisions are particularly…