Related papers: Rotational-hyperfine cooling of $^{205}$TlF in a c…
The Cold molecule Nuclear Time-Reversal EXperiment (CeNTREX) is a new effort aiming for a significant increase in sensitivity over the best present upper bounds on the strength of hadronic time reversal ($T$) violating fundamental…
We report high-precision measurements on the thallium fluoride $\tilde{J} = 1$ hyperfine manifold of the $B^3\Pi_1$ ($\nu = 0$) state. This state is of special interest because it is central to an optical cycling scheme that is envisioned…
Controlling the internal degrees of freedom is a key challenge for applications of cold and ultracold molecules. Here, we demonstrate rotational-state cooling of trapped methyl fluoride molecules (CH3F) by optically pumping the population…
We present a comprehensive characterization of cold molecular beams from a cryogenic buffer-gas cell, providing an insight into the physics of buffer-gas cooling. Cold molecular beams are extracted from a cryogenic cell by electrostatic…
Thallium monofluoride (TlF) is a prime candidate molecule for precision measurements aimed at discovering new physics. Optical cycling on the B $\leftarrow$ X transition around 271 nm enhances this potential. Hyperfine resolved ultraviolet…
We demonstrate cryogenic buffer-gas cooling of gas-phase methyltrioxorhenium (MTO). This molecule is closely related to chiral organometallic molecules where the parity-violating energy differences between enantiomers may be measurable. The…
Advances in cryogenic electron microscopy have opened new avenues for probing quantum phenomena in correlated materials. This study reports the installation and performance of a new side-entry condenZero cryogenic cooling system for JEOL…
The rotational and hyperfine spectrum of the $X^1\Sigma^+ \rightarrow B^3\Pi_1$ transition in TlF molecules was measured using laser-induced fluorescence from both a thermal and a cryogenic molecular beam. Rotational and hyperfine constants…
An experiment utilizing a TlF molecular beam is being developed by the CeNTREX collaboration to search for hadronic interactions that violate both time-reversal (T) and parity (P) invariance. Here we propose to use the same beam to look for…
A prerequisite for laser cooling a molecular anion, which has not been achieved so far, is the precise knowledge of the relevant transition frequencies in the cooling scheme. To determine these frequencies we present a versatile method that…
We report on the improved measurement of the hyperfine structure of $4f^{12}(^3 H_6)5d_{5/2}6s^2$ $(J=9/2)$ excited state in Tm-169 which is involved in the second-stage laser cooling of Tm. To measure the absolute value of the hyperfine…
We use two-dimensional transverse laser cooling to produce an ultracold beam of YbF molecules. Through experiments and numerical simulations, we study how the cooling is influenced by the polarization configuration, laser intensity, laser…
Next-generation cryogenic transmission electron microscopes (TEM) aim to achieve high-resolution imaging at ultracold sample temperatures (< 90 K) and over extended hold times. Lower temperatures enable atomic-scale characterization with…
Cooling the rotation and the vibration of molecules by broadband light sources was possible for trapped molecular ions or ultracold molecules. Because of a low power spectral density, the cooling timescale has never fell below than a few…
We demonstrate slowing and longitudinal cooling of a supersonic beam of CaF molecules using counter-propagating laser light resonant with a closed rotational and almost closed vibrational transition. A group of molecules are decelerated by…
We present a cold atomic beam source based on a two-dimensional (2D)+ magneto-optical trap (MOT), capable of generating a continuous cold beam of 87Rb atoms with a flux up to 4.3*10^9 atoms/s, a mean velocity of 10.96(2.20) m/s, and a…
The Luttinger surface of an organic metal (TTF-TCNQ), possessing charge order and spin-charge separation, is investigated using temperature dependent angle-resolved photoemission spectroscopy. The Luttinger surface topology, obtained from…
We report the complete characterization of various cooling grade Tm-doped crystals including the first demonstration of optical refrigeration in Tm:YLF crystals. Room temperature laser cooling efficiencies of 1% and 2% (mol) Tm:YLF, and 1%…
The AlF molecule, currently subject to laser cooling and trapping efforts, has the advantage that it can be efficiently produced in a thermochemical reaction between sublimated aluminum trifluoride and aluminum metal. Here we present a…
We investigate theoretically the application of tailored incoherent far-infrared fields in combination with laser excitation of a single rovibrational transition for rotational cooling of translationally cold polar diatomic molecules. The…