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Electronic nematic phases have been proposed to occur in various correlated electron systems and were recently claimed to have been detected in scanning tunneling microscopy (STM) conductance maps of the pseudogap states of the cuprate…

Strongly Correlated Electrons · Physics 2013-05-06 Eduardo H. da Silva Neto , Pegor Aynajian , Ryan E. Baumbach , Eric D. Bauer , John Mydosh , Shimpei Ono , Ali Yazdani

We have studied the electron hopping in a two-CdSe quantum dot system linked by an azobenzene-derived light-switching molecule. This system can be considered as a prototype of a QD supercrystal. Following the computational strategies given…

Materials Science · Physics 2014-03-17 Iek-Heng Chu , Jonathan Trinastic , Lin-Wang Wang , Hai-Ping Cheng

A new azobenzene-thiophene molecular switch is designed, synthesized and used to form self-assembled monolayers (SAM) on gold. An "on/off" conductance ratio up to 7x1E3 (with an average value of 1.5x1E3) is reported. The "on" conductance…

The state of the art ab initio calculations reveal the effect of a scanning tunnelling microscopy tip on magnetic properties and conductance of a benzene-adatom sandwich on Cu(001). We concentrate on a benzene-Co system interacting with a…

Materials Science · Physics 2009-11-13 Kun Tao , V. S. Stepanyuk , P. Bruno , D. I. Bazhanov , V. V. Maslyuk , M. Brandbyge , I. Mertig

Bare Si(100)-2$\times$1 surface atoms exhibit a buckled structure where one Si atom in a dimer is lowered while the other is raised, leading to two possible buckling configurations equivalent in energy. The relatively low energy barrier…

We study the light emission from a Ag(111) surface when the bias voltage on a scanning tunneling microscope (STM) junction is ramped into the field emission regime. Above the vacuum level, scanning tunneling spectroscopy (STS) shows a…

Mesoscale and Nanoscale Physics · Physics 2015-06-18 Jesús Martínez-Blanco , Stefan Fölsch

Azobenzene has become a ubiquitous component of functional molecules and polymeric materials because of the light-induced trans-cis isomerization of the diazene group. In contrast, there are very few applications utilizing azobenzene…

The emergent photoactive materials through photochemistry make it possible to directly convert photon energy to mechanical work. There is much recent work in developing appropriate materials and a promising new system is semi-crystalline…

Soft Condensed Matter · Physics 2021-03-24 Ruobing Bai , Eric Ocegueda , Kaushik Bhattacharya

We use a network of molecularly linked gold nanoparticles (NPSAN: nanoparticles self-assembled network) to demonstrate the electrical detection (conductance variation) of a plasmon-induced isomerization (PII) of azobenzene derivatives…

When two BN layers are stacked in parallel in an AB or BA arrangement, a spontaneous out-of-plane electric polarization arises due to charge transfer in the out-of-plane B-N bonds. The ferroelectric switching from AB to BA (or BA to AB) can…

In a first-principles study based on many-body perturbation theory, we analyze the optical excitations of azobenzene-functionalized SAMs with increasing packing density and different terminations, considering for comparison the…

Materials Science · Physics 2017-09-05 Caterina Cocchi , Claudia Draxl

We present a density-functional theory trend study addressing the binding of the trans-cis conformational switch azobenzene (C6H5-N=N-C6H5) at three coinage metal surfaces. From the reported detailed energetic, geometric, and electronic…

Materials Science · Physics 2012-01-27 Erik McNellis , Jorg Meyer , Abbas Dehghan Baghi , Karsten Reuter

Photoresponsive materials feature properties that can be adjusted near- instantaneously, reversibly, and with high spatiotemporal precision, by light. There is considerable interest in maximising the degree of switching, and in measuring…

Development of the methods to exploit nuclear hyperpolarization and search for molecules whose nuclear spins can be efficiently hyperpolarized is an active area in nuclear magnetic resonance. Of particular interest are those molecules that…

Since the first experimental observation of all-optical switching phenomena, intensive research has been focused on finding suitable magnetic systems that can be integrated as storage elements within spintronic devices and whose…

A scanning tunneling microscope (STM) can do more than atomic imaging and manipulation. Its tunneling current can also be used for the excitation of light, converting electron energy to photon energy. STM based single-molecule…

Optics · Physics 2019-01-01 Yao Zhang , Yang Zhang , Zhenchao Dong

The high carrier mobility in graphene promises its utility in electronics applications. Azobenzene is a widely studied organic molecule for switchable optoelectronic devices that can be synthesized with a wide variety of ligands and…

Materials Science · Physics 2015-06-18 Jonathan Trinastic , Hai-Ping Cheng

Strongly differing static dipole moments of the trans and cis isomers of photochromic azobenzene allow for optical switching the work function of azobenzene-functionalized self-assembled monolayers (SAMs). We apply these properties in a…

Mesoscale and Nanoscale Physics · Physics 2024-02-26 Jan Böhnke , Beatrice Andres , Larissa Boie , Angela Richter , Cornelius Gahl , Martin Weinelt , Wibke Bronsch

In a low-temperature study with a scanning tunneling microscope (STM), the irreducible lateral motion of a CO molecule adsorbed on a Si(001) surface showed a hyperlinear dependence on the tunneling current. This dependence implies that the…

We report the formation of self-assembled monolayers of a molecular photoswitch (azobenzene-bithiophene derivative, AzBT) on cobalt via a thiol covalent bond. We study the electrical properties of the molecular junctions formed with the tip…