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Resonance Raman scattering, which probes electrons, phonons and their interplay in crystals, is extensively used in two-dimensional materials. Here we investigate Raman modes in MoSe$_2$ at different laser excitation energies from 2.33 eV…

We treat resonant Raman scattering via the multiphonon exciton transitions in cylindrical quantum dots with a parabolic confinement in the lateral direction and with a finite rectangular interface-barrier confinement in the axial direction.…

Mesoscale and Nanoscale Physics · Physics 2012-05-09 S. N. Klimin , V. M. Fomin , J. T. Devreese , J. -P. Leburton

We calculate, as a function of temperature and conduction band electron density, the optical absorption of a weakly n-doped, idealized semiconductor quantum well. In particular, we focus on the absorption band due to the formation of a…

Strongly Correlated Electrons · Physics 2009-11-07 F. X. Bronold

Optical properties of heterostructures composed of layered 2D materials, such as transition metal dichalcogenides (TMDs) and graphene, are broadly explored. Of particular interest are light-induced energy transfer mechanisms in these…

Materials Science · Physics 2024-09-17 Amir Kleiner , Daniel Hernangómez-Pérez , Sivan Refaely-Abramson

Innovations in imaging technology involves finding strategies and materials suitable for detection applications over the entire infrared range. Herein, we propose a new design concept based on the unique feature of an excitonic insulator,…

Materials Science · Physics 2022-07-27 Jing Liu , Yuanchang Li

In this work, we investigate the combined influence of the nontrivial topology introduced by a disclination and non inertial effects due to rotation, in the energy levels and the wave functions of a noninteracting electron gas confined to a…

Other Condensed Matter · Physics 2017-06-21 Moises Rojas , Cleverson Figueiras , Julio Brandão , Fernando Moraes

We study the dynamics of excitonic insulators coupled to phonons. Without phonon couplings, the linear response is given by the damped amplitude oscillations of the order parameter with frequency equal to the minimum band gap. A phonon…

Strongly Correlated Electrons · Physics 2017-12-19 Yuta Murakami , Denis Golež , Martin Eckstein , Philipp Werner

Optical extinction and absorption enhancement in the infrared range of a monolayer graphene sheet by patterning split ring resonators (SRRs) is studied. It is found that the electric mode is stronger in enhancing infrared extinction and…

Optics · Physics 2014-07-31 Yuancheng Fan , Zeyong Wei , Zhengren Zhang , Hongqiang Li

Despite the weak, van-der-Waals interlayer coupling, photoinduced charge transfer vertically across atomically thin interfaces can occur within surprisingly fast, sub-50fs timescales. Early theoretical understanding of the charge transfer…

We present calculations of the absorption spectrum of semiconductors and insulators comparing various approaches: (i) the two-particle Bethe-Salpeter equation of Many-Body Perturbation Theory; (ii) time-dependent density-functional theory…

Other Condensed Matter · Physics 2009-11-13 Francesco Sottile , Marherita Marsili , Valerio Olevano , Lucia Reining

We propose a method to controllably suppress the effect of the four-wave mixing caused by the coupling of the strong control optical field to both optical transitions in the $\Lambda$ system under the conditions of electromagnetically…

Quantum Physics · Physics 2016-09-21 Gleb Romanov , Chris O'Brien , I. Novikova

Precise infrared magnetotransmission experiments have been performed in magnetic fields up to 32 T on a series of multilayer epitaxial graphene samples. We observe changes in the spectral features and broadening of the main cyclotron…

Mesoscale and Nanoscale Physics · Physics 2012-06-15 M. Orlita , Liang Z. Tan , M. Potemski , M. Sprinkle , C. Berger , W. A. de Heer , Steven G. Louie , G. Martinez

The Raman effect -- inelastic scattering of light by lattice vibrations (phonons) -- produces an optical response closely tied to a material's crystal structure. Here we show that resonant optical excitation of IR and Raman phonons gives…

Materials Science · Physics 2021-07-07 Guru Khalsa , Nicole A. Benedek , Jeffrey Moses

We propose a continuum model for the theoretical study of hybridized moir\'e excitons in transition metal dichalcogenides heterobilayers, and we use a variational method to solve the exciton wavefunction and calculate the optical absorption…

Mesoscale and Nanoscale Physics · Physics 2023-10-23 Yao-Wen Chang

We used Raman scattering for study the phonon modes of self-organized Ge/Si quantum dots, grown by a molecular-beam epitaxy method. It is revealed, that Ge-Ge and Si-Ge vibrational modes considerably intensify at excitation of exciton…

Mesoscale and Nanoscale Physics · Physics 2011-05-17 I. V. Kucherenko , V. S. Vinogradov , N. N. Melnik , L. V. Arapkina , V. A. Chapnin , K. V. Chizh , V. A. Yuryev

A general theory of electronic excitations in aggregates of molecules coupled to intramolecular vibrations and the harmonic environment is developed for simulation of the third-order nonlinear spectroscopy signals. The model is applied in…

Chemical Physics · Physics 2014-01-17 Vytautas Butkus , Leonas Valkunas , Darius Abramavicius

The concept of \textit{optical} exciton - a photo-excited bound electron-hole pair within a crystal - is routinely used to interpret and model a wealth of excited-state phenomena in semiconductors. Beside originating sub-band gap signatures…

Materials Science · Physics 2022-09-21 Fulvio Paleari , Andrea Marini

An approach is presented for theoretical calculations of the Debye-Waller factors in x-ray absorption spectra. These factors are represented in terms of the cumulant expansion up to third order. They account respectively for the net thermal…

Materials Science · Physics 2009-11-13 Fernando D. Vila , J. J. Rehr , H. H. Rossner , H. J. Krappe

We theoretically investigate the double-resonance Raman spectrum of monolayer graphene down to infrared laser excitation energies. By using first-principles density functional theory calculations, we improve upon previous theoretical…

Mesoscale and Nanoscale Physics · Physics 2025-05-21 Lorenzo Graziotto , Francesco Macheda , Thibault Sohier , Matteo Calandra , Francesco Mauri

Theoretical and numerical calculations of the optical absorption spectra of excitons interacting with longitudinal-optical phonons in quasi-2D polar semiconductors are presented. In II-VI semiconductor quantum wells, exciton binding energy…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 F. J. Rodriguez