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We demonstrate efficient optical rectification in the organic crystal BNA (N-benzyl-2-methyl-4-nitroaniline), driven by a temporally compressed, commercially available industrial Yb-laser system operating at 540 kHz repetition rate. Our THz…

We demonstrate a 13.3 MHz repetition rate, broadband THz source with milliwatt-average power, obtained by collinear optical rectification of a high-power Yb-doped thin-disk laser in the organic crystal BNA…

Increasing the average power of broadband, few-cycle terahertz (THz) sources is currently a topic of intense investigation, fueled by recent immense progress in high average power femtosecond laser driving sources at 1030 nm. However, many…

We present a terahertz time-domain spectroscopy (THz-TDS) system which accesses a broadband spectrum, efficiently covering the so-called "new THz gap" between 5 and 15 THz and extending beyond 25 THz. The system exploits nonlinear…

We report on high energy terahertz pulses by optical rectification (OR) in the organic crystal N-benzyl-2-methyl-4-nitroaniline (BNA) directly pumped by a conventional Ti:Sapphire (Ti:Sa) amplifier. The simple scheme provides an optical to…

The organic terahertz (THz) generation crystal BNA has recently gained traction as a valuable source to produce broadband THz pulses. Even when pumped with 800-nm light, thin BNA crystals can produce relatively high electric fields with…

In this work, we demonstrate BNAs high potential for efficient generation of high power THz using ytterbium laser wavelengths. We study the generation theoretically and experimentally using laser wavelength of 960-1150 nm. Broadband pulses…

Optics · Physics 2021-09-10 Hovan Lee , Claudia Gollner , Jiaqi Nie , Yan Zhang , Cedric Weber , Mostafa Shalaby

Organic nonlinear optical (NLO) crystals have emerged as efficient room-temperature emitters of broadband THz radiation with high electric field strengths. Although initially confined to high-pulse-energy excitation in the millijoule range…

Optics · Physics 2024-08-07 Lukasz A. Sterczewski , Jakub Mnich , Jaroslaw Sotor

We characterize the terahertz (THz) generation of N-benzyl-2-methyl-4-nitroaniline (BNA), with crystals ranging in thickness from 123-700 {\mu}m. We compare excitation using 800-nm and 1250 to 1500-nm wavelengths. Pumping BNA with 800-nm…

We are reporting on terahertz generation from organic crystal BNA using a 1.15 to 1.55 um near infrared pump. We observed a very large emission spectrum extending up to 7 THz, compared to 2.5 THz from Ti:Sa pump in previous reports. The…

Materials Science · Physics 2019-07-24 Hang Zhao , Yong Tan , Tong Wu , Gunther Steinfeld , Yan Zhang , Cunlin Zhang , Liangliang Zhang , Mostafa Shalaby

We construct a terahertz time-domain spectrometer (THz-TDS) system based on photoconductive antenna (PCA). A 800 nm Ti sapphire femtosecond laser with 80 MHz repetition rate provides the pump and probe laser pulse, which has a 45 fs pulse…

Optics · Physics 2014-08-11 Jitao Zhang , Wei-Ren Ng , Mingguang Tuo , Min Liang , M. E. Gehm , Hao Xin

As high-average power ultrafast lasers become increasingly available for nonlinear conversion, the temperature dependence of the material properties of nonlinear crystals becomes increasingly relevant. Here, we present temperature-dependent…

Optics · Physics 2023-08-29 Samira Mansourzadeh , Tim Vogel , Mostafa Shalaby , Clara J. Saraceno

The generation of tunable narrowband pulses is increasingly being pursued in terahertz science, for example to study the nonlinear response of individual modes of solids and molecules. Here, we extend the chirp-and-delay method to achieve…

Optics · Physics 2025-10-28 D. Pavicevic , M. Nishida , J. Song , M. Buzzi , A. Cavalleri

Scaling femtosecond terahertz (THz) and ultraviolet (UV) sources to high repetition rates is essential for high-throughput ultrafast spectroscopy and imaging applications. Yet, their efficient generation at high average power remains…

Optics · Physics 2026-01-06 Andrey Ryabov , Kasra Amini

We demonstrate a high average power terahertz time-domain (THZ-TDS) spectrometer based on optical rectification in the tilted-pulse front geometry in lithium niobate at room temperature, driven by a commercial, industrial femtosecond-laser…

Optics · Physics 2023-11-01 Celia Millon , Sarah Houver , Clara J. Saraceno

High energy terahertz pulses are produced by optical rectification (OR) in organic crystals DAST and DSTMS by a Ti:sapphire amplifier system centered at 0.8 microns. The simple scheme provides broadband spectra between 1 and 5 THz, when…

Optics · Physics 2015-06-17 B. Monoszlai , C. Vicario , M. Jazbinsek , C. P. Hauri

We report the coherent generation and detection of terahertz (THz) pulses covering the bandwidth of 0.1-9 THz in a high repetition rate, low pulse energy laser system. In this work we demonstrate the application and evaluation of…

The intense terahertz (THz) pulses facilitate the observation of various nonlinear optical effects and manipulation of material properties. In this work, we report a convenient approach that can produce strong broadband terahertz pulses…

Optics · Physics 2023-03-08 Yuxuan Wei , Jiaming Le , Chuanshan Tian

The ideal laser source for the emerging research field of nonlinear Terahertz (THz) spectroscopy should offer radiation with a large versatility and deliver both ultra-intense multi-octave spanning single-cycle pulses and user-selectable…

Mamyshev oscillators are an emerging class of ultrafast fiber lasers that support exceptionally broadband spectra and few-femtosecond pulse durations, making them well-suited for nonlinear frequency conversion. Despite this potential, THz…

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