Related papers: Indirect Zero Field NMR Spectroscopy
Development of the methods to exploit nuclear hyperpolarization and search for molecules whose nuclear spins can be efficiently hyperpolarized is an active area in nuclear magnetic resonance. Of particular interest are those molecules that…
We report Zeeman infra-red spectroscopy of electronic-nuclear levels of $^5$I$_8 \rightarrow ^5$I$_7$ transitions of Ho$^{3+}$ in the C$_{\rm 4v}$(F$^-$) centre in CaF$_2$ with the magnetic field along the $\langle 111\rangle$ direction of…
We analyze the ground-state energy, local spin correlation, impurity spin polarization, impurity-induced magnetization, and corresponding zero-field susceptibilities of the symmetric single-impurity Kondo model on a tight-binding chain with…
We resolve the real-time electric field of a femtosecond third-order nonlinear optical signal in the molecular frame. The electric field emitted by the induced third-order polarization from impulsively pre-aligned gas-phase molecules at…
We report the first experimental observation of non-adiabatic field-free orientation of a heteronuclear diatomic molecule (CO) induced by an intense two-color (800 and 400 nm) femtosecond laser field. We monitor orientation by measuring…
The work to be described falls into three parts: (1) The computer-controlled CW spectrometer was designed to supplement the Manchester pulsed microwave spectrometer in situations where rapid nuclear relaxation makes spin-echo spectroscopy…
Inverse problems in scientific sensing are often solved with either hand-designed regularizers or supervised networks trained on simulated labels, yet both can fail when the forward model is nonlinear, spectrally coupled, and physically…
Binary ferroelectric nitrides are promising materials for information technologies and power electronics. However, polarization switching in these materials is highly unusual. From the structural perspective, polarization reversal is…
Surface alignment of a recently discovered ferroelectric nematic liquid crystal (NF) is usually achieved by buffed polymer films, which produce a unidirectional polar alignment of the spontaneous electric polarization. We demonstrate that…
Chemical shifts and J-couplings are fundamental parameters in NMR spectroscopy as they provide structural information about molecules. Extracting these quantities from isotopes such as carbon or nitrogen results in reduced sensitivity due…
Signal amplification by reversible exchange (SABRE) is a nuclear spin hyperpolarization technique in which the transient interaction of parahydrogen (pH2) and a target substrate with an iridium complex leads to polarization transfer to the…
Noise measurements provide a valuable tool for revealing spin polarization effects in the electronic transport through quantum coherent conductors. We present an extension of the Landauer description of shot noise to include…
We present a comprehensive spectroscopic study of C$_{2v}$ point-group symmetry sites in Sm$^{3+}$:CaF$_2$/SrF$_2$ codoped with either NaF or LiF. Data includes electron paramagnetic resonance measurements of Zeeman and hyperfine…
Subwavelength metallic resonators provide a route to achieving strong light-matter coupling by means of tight confinement of resonant electromagnetic fields. Investigation of such resonators however often presents experimental difficulties,…
Photochemically induced dynamic nuclear polarization (photo-CIDNP) is a method to hyperpolarize nuclear spins using light. In most cases, CIDNP experiments are performed at a high magnetic field and the sample is irradiated by the light…
We develop optimised estimators of two sorts of power spectra for fields defined on the sky, in the presence of partial sky coverage. The first is the cross-power spectrum of two fields on the sky; the second is the skew spectrum of three…
We investigate nonlinear Kerr-induced coherence effect on a superluminal probing light pulse in a gain-assisted N-type 4-level atomic system via an intense monochromatic laser field. The dispersion exhibits a novel, interesting and useful…
Wideband spectrum sensing for low-altitude monitoring is critical yet challenging due to heterogeneous protocols,large bandwidths, and non-stationary SNR. Existing data-driven approaches treat spectrograms as natural images,suffering from…
19F isotropic chemical shifts for alkali, alkaline earth and rare earth of column 3 basic fluorides are measured and the corresponding isotropic chemical shieldings are calculated using the GIPAW method. When using PBE exchange correlation…
Materials imperfections in Nniobium based superconducting quantum circuits, in particular, two-level-system (TLS) defects, are a major source of decoherence, ultimately limiting the performance of quantum computation and sensing. Thus,…