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Experimental observations of the ultrafast (less than 50 fs) demagnetization of Ni have so far defied theoretical explanations particularly since its spin-flipping time is much less than that resulting from spin-orbit and electron-lattice…

Strongly Correlated Electrons · Physics 2020-07-08 Shree Ram Acharya , Volodymyr Turkowski , Guo-ping Zhang Talat S. Rahman

The ultrafast dynamics of magnetic order in a ferromagnet are governed by the interplay between electronic, magnetic and lattice degrees of freedom. In order to obtain a microscopic understanding of ultrafast demagnetization, information on…

Ultrafast magnetization dynamics probes the most fundamental properties of magnetic materials, exploring questions about the fundamental interactions responsible for magnetic phenomena. Thermal effects are known to be extremely important…

Materials Science · Physics 2019-08-26 Daniel Meilak , Sarah Jenkins , Rory Pond , Richard F. L. Evans

Femtosecond laser excitation of materials that exhibit magnetic spin textures promises advanced magnetic control via the generation of ultrafast and non-equilibrium spin dynamics. We explore such possibilities in ferrimagnetic [Fe(0.35…

Despite intense experimental effort, theoretical proposals and modeling approaches, a lack of consensus exists about the intrinsic mechanisms driving ultrafast magnetization dynamics in 3$d$ ferromagnets. In this work, we find evidence of…

Materials Science · Physics 2023-03-29 Theodor Griepe , Unai Atxitia

Ferrimagnets containing several partially compensated magnetic sublattices are considered the most promising materials for all-optical data storage and for ultrafast communications based on spin waves. There are two magnetic phases of the…

Following the demonstration of laser-induced ultrafast demagnetization in ferromagnetic nickel, several theoretical and phenomenological propositions have sought to uncover its underlying physics. In this work we revisit the three…

Strongly Correlated Electrons · Physics 2023-03-29 Suchetana Mukhopadhyay , Sudip Majumder , Surya Narayan Panda , Anjan Barman

Antiferromagnets naturally exhibit three obvious advantages over ferromagnets for memory device applications: insensitivity to external magnetic fields, much faster spin dynamics (~THz) and higher packing density due to the absence of any…

Mesoscale and Nanoscale Physics · Physics 2019-03-15 Zhiqi Liu , Zexin Feng , Han Yan , Xiaoning Wang , Xiaorong Zhou , Peixin Qin , Huixin Guo , Ronghai Yu , Chengbao Jiang

Altermagnets constitute a new class of magnetic materials that combine properties previously thought to be exclusive to either antiferromagnets or ferromagnets, and have unique properties of their own. In particular, a combination of…

The parallel or antiparallel arrangement of electron spins plays a pivotal role in determining the properties of a physical system. To meet the demands for innovative technological solutions, extensive efforts have been dedicated to…

We propose a semi-classical model for femtosecond-laser induced demagnetization due to spin-polarized excited electron diffusion in the super-diffusive regime. Our approach treats the finite elapsed time and transport in space between…

Materials Science · Physics 2011-06-14 Marco Battiato , Karel Carva , Peter M. Oppeneer

Time-dependent density functional theory is implemented in an all electron solid-state code for the case of fully non-collinear spins. We use this to study laser induced demagnetization in Fe, Co and Ni. It is shown that this…

Materials Science · Physics 2014-06-26 K. Krieger , J. K. Dewhurst , P. Elliott , S. Sharma , E. K. U. Gross

The injection of spin currents in semiconductors is one of the big challenges of spintronics. Motivated by the ultrafast demagnetisation and spin injection into metals, we propose an alternative femtosecond route based on the laser…

Materials Science · Physics 2016-05-25 M. Battiato , K. Held

We investigate ultrafast demagnetization due to electron-phonon interaction in a model band-ferromagnet. We show that the microscopic mechanism behind the spin dynamics due to electron-phonon interaction is the interplay of scattering and…

Materials Science · Physics 2017-10-25 Kai Leckron , Svenja Vollmar , Hans Christian Schneider

We study the ultrafast demagnetization of Ni/NiMn and Co/NiMn ferromagnetic/antiferromagnetic bilayer systems after excitation by a laser pulse. We probe the ferromagnetic order of Ni and Co using magnetic circular dichroism in…

Ferromagnets are key materials for sensing and memory applications. In contrast, antiferromagnets that represent the more common form of magnetically ordered materials, have so far found less practical application beyond their use for…

Mesoscale and Nanoscale Physics · Physics 2017-05-31 J. Železný , P. Wadley , K. Olejník. A. Hoffmann , H. Ohno

Ultrafast heating of FeRh by a femtosecond laser pulse launches a magneto-structural phase transition from an antiferromagnetic to a ferromagnetic state. Aiming to reveal the ultrafast kinetics of this transition, we studied magnetization…

Recent interest in developing fast spintronic devices and laser-controllable magnetic solids has sparked tremendous experimental and theoretical efforts to understand and manipulate ultrafast dynamics in materials. Studies of spin dynamics…

Optics · Physics 2022-09-21 Xinwei Li , Dasom Kim , Yincheng Liu , Junichiro Kono

Soft ferromagnetic NiFe thin films are promising for applications in spintronic devices because of their constituent electrical and magnetic properties. Electron beam evaporation and sputtering techniques have been used to deposit NiFe thin…

Materials Science · Physics 2023-04-04 H. Yan , G. J. Omar , Z. T. Zhao , Lim Zhi Shiuh , A. Ariando

The magnetization dynamics for ferrimagnets at the angular momentum compensation temperature T_A is believed to be analogous to that for antiferromagnets. We investigated the pulsed-laser-induced magnetization dynamics in amorphous…

Materials Science · Physics 2018-08-20 S. Mizukami , Y. Sasaki , D. -K. Lee , H. Yoshikawa , A. Tsukamoto , K. -J. Lee , T. Ono