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It is well known that energy-time entanglement can enhance two photon absorption (TPA) by simultaneously optimizing the two photon resonance and the coincidence rate of photons at the absorber. However, the precise relation between…

Quantum Physics · Physics 2021-08-31 Baihong Li , Holger F. Hofmann

An entangled quantum state is considered by applying a local photon excitation to each mode of an entangled coherent state. The entanglement property is investigated in terms of the entropy of entanglement. It is shown that applying a…

Quantum Physics · Physics 2023-04-13 Arpita Chatterjee

We study the dynamics of quantum matter interacting with time-energy entangled photons. We consider the stimulation of a collective mode of a two-dimensional material by means of one of the two partners of a time-energy entangled pair of…

Mesoscale and Nanoscale Physics · Physics 2026-01-15 Giovanni Citeroni , Marco Polini , Michael Dapolito , D. N. Basov , Giacomo Mazza

In virtual-state spectroscopy, information about the energy-level structure of an arbitrary sample is retrieved by Fourier transforming sets of measured two-photon absorption probabilities of entangled photon pairs where the degree of…

Quantum Physics · Physics 2021-08-04 Lutz Mertenskötter , Kurt Busch , Roberto de J. León-Montiel

We devise a theory of x-ray absorption by symmetric-top molecules which are aligned by an intense optical laser. Initially, the density matrix of the system is composed of the electronic ground state of the molecules and a thermal ensemble…

Chemical Physics · Physics 2008-02-23 Christian Buth , Robin Santra

Here we present theoretical studies of the effect of vibronic coupling on nonlinear transport characteristics (current-voltage and conductance-voltage) in molecular electronic devices. Considered device is composed of molecular quantum dot…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Kamil Walczak

Quantum hypothesis testing has been greatly advanced for the binary discrimination of two states, or two channels. In this setting, we already know that quantum entanglement can be used to enhance the discrimination of two bosonic channels.…

Quantum Physics · Physics 2020-07-30 Quntao Zhuang , Stefano Pirandola

We study the two-photon scattering processes in a one-dimensional waveguide coupled to a two- or three-level giant atom, respectively. The accumulated phase shift between the two coupling points can be utilized to alter the scattering…

Quantum Physics · Physics 2023-11-30 Wenju Gu , He Huang , Zhen Yi , Lei Chen , Lihui Sun , Huatang Tan

Predicting the response of a system to perturbations is a key challenge in mathematical and natural sciences. Under suitable conditions on the nature of the system, of the perturbation, and of the observables of interest, response theories…

Statistical Mechanics · Physics 2017-09-13 Valerio Lucarini , Jeroen Wouters

While two-photon absorption (TPA) and other forms of nonlinear interactions of molecules with isolated time-frequency-entangled photon pairs (EPP) have been predicted to display a variety of fascinating effects, their potential use in…

We develop the theory of dynamical superradiance -- the collective exchange of energy between an ensemble of initially excited emitters and a single-mode cavity -- for organic materials where electronic states are coupled to vibrational…

We calculate the rate of two-photon absorption for frequency entangled photons in a tapered optical fiber whose diameter is comparable to the wavelength of the light. The confinement of the electric field in the transverse direction…

Quantum Physics · Physics 2010-04-12 Hao You , S. M. Hendrickson , J. D. Franson

In this paper, we study two-photon interference of broadband chaotic light in a Michelson interferometer with two-photon-absorption detector. The theoretical analysis is based on two-photon interference and Feynman path integral theory. The…

Quantum Physics · Physics 2021-09-01 Y. Zhou , S. Luo , J. Liu , H. Zheng , H. Chen , Y. He , Y. Liu , F. Li , Z. Xu

Quantum light spectroscopy, providing novel molecular information non-accessible by classical light, necessitates new computational tools when applied for complex molecular systems. We introduce two computational protocols for the molecular…

Chemical Physics · Physics 2021-09-14 Bing Gu , Daniel Keefer , Shaul Mukamel

We present a microscopic quantum theory of intersubband polarons, quasiparticles originated from the coupling between intersubband transitions and longitudinal optical phonons. To this aim we develop a second quantized theory taking into…

Materials Science · Physics 2015-06-03 Simone De Liberato , Cristiano Ciuti

Motivated by recent experiments on radiative recombination of two-dimensional electrons in acceptor doped GaAs-AlGaAs heterojunctions as well as the success of a harmonic solid model in describing tunneling between two-dimensional electron…

Strongly Correlated Electrons · Physics 2016-08-31 S. Kodiyalam , H. A. Fertig , S. Das Sarma

Vibrationally resolved electronic absorption spectra including the effect of vibrational pre-excitation are computed in order to interpret and predict vibronic transitions that are probed in the Vibrationally Promoted Electronic Resonance…

Interaction of an electron system with a strong electromagnetic wave leads to rearrangement both the electron and vibrational energy spectra of a dissipative system. For instance, the optically coupled electron levels become split in the…

Other Condensed Matter · Physics 2017-09-21 Andrei Ivanov

We derive the second-order approximation (PT2) to the ensemble correlation energy functional by applying the G\"{o}rling-Levy perturbation theory on the ensemble density-functional theory (EDFT). Its performance is checked by calculating…

Computational Physics · Physics 2021-11-17 Zeng-hui Yang

Ultrafast laser excitation can create coherent superpositions of electronic states in molecules and trigger ultrafast flow of electron density on few- to sub-femtosecond time scales. While recent attosecond experiments have addressed…

Chemical Physics · Physics 2020-11-18 Yuki Kobayashi , Daniel M. Neumark , Stephen R. Leone