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We consider optical spectroscopy of molecular junctions from the quantum transport perspective when radiation field is quantized and optical response of the system is simulated as photon flux. Using exact expressions for photon and…

Mesoscale and Nanoscale Physics · Physics 2016-05-09 Yi Gao , Michael Galperin

We present a theoretical approach to optical spectroscopy of open nonequilibrium systems, which generalizes traditional nonlinear optical spectroscopy tools by imposing charge and energy conservation at all levels of approximation. Both…

Mesoscale and Nanoscale Physics · Physics 2019-12-19 Shaul Mukamel , Michael Galperin

Progress of experimental techniques at nanoscale in the last decade made optical measurements in current-carrying nanojunctions a reality thus indicating emergence of a new field of research coined as optoelectronics. Optical spectroscopy…

Mesoscale and Nanoscale Physics · Physics 2018-03-26 Michael Galperin

Two-dimensional spectroscopy is discussed for open quantum systems with multiple simultaneously measurable fluxes. In particular, we discuss a junction where optical measurements of photon flux are complemented with simultaneous transport…

Mesoscale and Nanoscale Physics · Physics 2025-02-28 Haoran Sun , Upendra Harbola , Shaul Mukamel , Michael Galperin

We study the nonlinear elastic quantum electronic transport properties of nanoscopic devices using the Nonequilibrium Green's function (NEGF) method. The Green's function method allows us to expand the $I-V$ characteristics of a given…

Mesoscale and Nanoscale Physics · Physics 2009-07-14 Alexis R. Hernández , Caio H. Lewenkopf

We discuss theoretical approaches to nonlinear optical spectroscopy of molecular junctions. Optical response functions are derived in the form convenient for implementation of Green function techniques, and their expressions in terms of…

Mesoscale and Nanoscale Physics · Physics 2016-06-28 Yi Gao , Michael Galperin

We introduce diagrammatic technique for Hubbard nonequilibrium Green functions (NEGF). The formulation is an extension of equilibrium considerations for strongly correlated lattice models to description of current carrying molecular…

Mesoscale and Nanoscale Physics · Physics 2016-11-04 Feng Chen , Maicol A. Ochoa , Michael Galperin

Nonlinear optical signals from an assembly of N noninteracting particles consist of an incoherent and a coherent component, whose magnitudes scale \sim N and \sim N(N-1), respectively. A unified microscopic description of both types of…

Quantum Physics · Physics 2009-11-13 Christoph A. Marx , Upendra Harbola , Shaul Mukamel

We present a brief pedagogical review of theoretical Green's function methods applicable to open quantum systems out of equilibrium in general, and single molecule junctions in particular. We briefly describe experimental advances in…

Mesoscale and Nanoscale Physics · Physics 2020-03-10 Guy Cohen , Michael Galperin

This article reviews the application of the non-equilibrium Green's function formalism to the simulation of novel photovoltaic devices utilizing quantum confinement effects in low dimensional absorber structures. It covers well-known…

Mesoscale and Nanoscale Physics · Physics 2012-06-14 U. Aeberhard

Non equilibrium Green's function methods are regularly used to calculate current and charge densities in nanoscale (both molecular and semiconductor) conductors under bias. This method is mainly used for ballistic conduction but may be…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 M. Paulsson

Nonlinear spectroscopy employs a series of laser pulses to interrogate dynamics in large interacting many-body systems, and has become a highly successful method for experiments in chemical physics. Current quantum optical experiments…

Quantum Physics · Physics 2016-10-19 Frank Schlawin , Manuel Gessner , Shaul Mukamel , Andreas Buchleitner

The Non-equilibrium Green's function (NEGF) formalism is a particularly powerful method to simulate the quantum transport properties of nanoscale devices such as transistors, photo-diodes, or memory cells, in the ballistic limit of…

Sub-wavelength arrays of quantum emitters offer an efficient free-space approach to coherent light-matter interfacing, using ultracold atoms or two-dimensional solid-state quantum materials. The combination of collectively suppressed…

Quantum Gases · Physics 2024-12-16 Simon Panyella Pedersen , Georg M. Bruun , Thomas Pohl

We present an overview of electronic device modeling using non-equilibrium Green function techniques. The basic approach developed in the early 1970s has become increasingly popular during the last 10 years. The rise in popularity was…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Roger K. Lake , Rajeev R. Pandey

We put forward a first-principle NonEquilibrium Green's Function (NEGF) approach to calculate the transient photoabsorption spectrum of optically thin samples. The method can deal with pump fields of arbitrary strength, frequency and…

Atomic Physics · Physics 2015-09-30 E. Perfetto , A. -M. Uimonen , R. van Leeuwen , G. Stefanucci

We study inelastic electron tunneling through a molecular junction using the non-equilibrium Green function (NEGF) formalism. The effect of the mutual influence between the phonon and the electron subsystems on the electron tunneling…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Michael Galperin , Mark A. Ratner , Abraham Nitzan

We develop a non-perturbative formulation based on the Green-function quantization method, that can describe spontaneous parametric down-conversion in the high-gain regime in nonlinear optical structures with arbitrary amount of loss and…

Quantum Physics · Physics 2023-12-13 Aleksa Krstić , Frank Setzpfandt , Sina Saravi

Due to their conceptual appeal and computational convenience, two-level systems (TLS) and their generalisations are often used to investigate nonlinear behavior in quantum optics, and to assess the applicability of theoretical methods. Here…

Quantum Physics · Physics 2023-12-22 Megha Gopalakrishna , Yaroslav Pavlyukh , Claudio Verdozzi

We give nonequilibrium Green's function (NEGF) perspective on thermodynamics formulations for open quantum systems strongly coupled to baths. Scattering approach implying thermodynamic consideration of a super-system (system plus baths)…

Mesoscale and Nanoscale Physics · Physics 2021-04-19 Nicolas Bergmann , Michael Galperin
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