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We demonstrate a coherence time of 2.1(1)~s for electron spin superposition states of a single trapped $^{40}$Ca$^+$ ion. The coherence time, measured with a spin-echo experiment, corresponds to residual rms magnetic field fluctuations…

In many important situations the dominant dephasing mechanism in cryogenic rare-earth-ion doped systems is due to magnetic field fluctuations from spins in the host crystal. Operating at a magnetic field where a transition has a zero…

Atomic Physics · Physics 2015-06-03 D. L. McAuslan , J. G. Bartholomew , M. J. Sellars , J. J. Longdell

Hidden magnetic order of Sr$_2$Ir$_{1-x}$Rh$_x$O$_4$, $x = 0.05$ and 0.1, has been studied using muon spin relaxation spectroscopy. In zero applied field and weak longitudinal fields ($\mu_0H_L \lesssim 2$~mT), muon spin relaxation data can…

Strongly Correlated Electrons · Physics 2020-05-13 C. Tan , Z. F. Ding , J. Zhang , Z. H. Zhu , O. O. Bernal , P. -C. Ho , A. D. Hillier , A. Koda , H. Luetkens , G. D. Morris , D. E. MacLaughlin , L. Shu

We explore spin dynamics of isotopically purified $^{166}$Er:$^{7}$LiYF$_4$ crystal below 1 Kelvin and at weak magnetic fields $<$0.3 T. Crystals grown in our lab demonstrate record-narrow inhomogeneous optical broadening down to 16~MHz.…

We experimentally investigate the coherence properties of a qubit stored in the Zeeman substates of the 5S1/2, F=1 hyperfine ground level of a single optically trapped Rb-87 atom. Larmor precession of a single atomic spin-1 system is…

Quantum Physics · Physics 2015-05-28 Wenjamin Rosenfeld , Jürgen Volz , Markus Weber , Harald Weinfurter

Erbium-doped solids are prime candidates for optical quantum communication networks due to erbium's telecom C-band emission. A long-lived electron spin of erbium with millisecond coherence time is highly desirable for establishing…

Quantum Physics · Physics 2023-10-16 Shobhit Gupta , Xuntao Wu , Haitao Zhang , Jun Yang , Tian Zhong

We report detailed measurements of the low temperature magnetic phase diagram of Er$_2$Ti$_2$O$_7$. Heat capacity and time-of-flight neutron scattering studies of single crystals, subject to magnetic fields applied along the…

Strongly Correlated Electrons · Physics 2012-07-16 J. P. C. Ruff , J. P. Clancy , A. Bourque , M. A. White , M. Ramazanoglu , J. S. Gardner , Y. Qiu , J. R. D. Copley , H. A. Dabkowska , B. D. Gaulin

We study the long-time decay of fourth-order electron spin correlation functions for an isolated singly charged semi-conductor quantum dot. The electron spin dynamics is governed by the applied external magnetic field as well as the…

Mesoscale and Nanoscale Physics · Physics 2017-10-23 Nina Fröhling , Frithjof B. Anders

A pronounced step-like (kink) behavior in the temperature dependence of resistivity $\rho (T)$ is observed in the optimally-doped $Sm_{1.85}Ce_{0.15}CuO_4$ thin films around $T_{sf}=87K$ and attributed to manifestation of strong spin…

Superconductivity · Physics 2007-08-30 S. Sergeenkov , A. J. C. Lanfredi , F. M. Araujo-Moreira

We address the decoherence of a localized electron spin in an external magnetic field due to the hyperfine interaction with a lattice of nuclear spins. Using a completely non-perturbative method, rigorous bounds on the T_1 and T_2 coherence…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Neil Shenvi , Rogerio de Sousa , K. Birgitta Whaley

The layered honeycomb iridate $\alpha$-Li$_2$IrO$_3$ displays an incommensurate magnetic structure with counterrotating moments on nearest-neighbor sites, proposed to be stabilized by strongly-frustrated anisotropic Kitaev interactions…

Strongly Correlated Electrons · Physics 2019-03-06 Sungkyun Choi , S. Manni , J. Singleton , C. V. Topping , T. Lancaster , S. J. Blundell , D. T. Adroja , V. Zapf , P. Gegenwart , R. Coldea

We analyze the spin anisotropy of the magnetic susceptibility of Sr$_2$RuO$4$ in presence of spin-orbit coupling and anisotropic strain using quasi-two-dimensional tight-binding parametrization fitted to the ARPES results. Similar to the…

Superconductivity · Physics 2016-12-15 Sergio Cobo , Felix Ahn , Ilya Eremin , Alireza Akbari

When superconductivity is suppressed by high magnetic fields in La2-xSrxCuO4, striped antiferromagnetic (AFM) order becomes the magnetic ground state of the entire pseudogap regime, up to its end at the doping p* [M. Frachet, I. Vinograd et…

Using neutron inelastic scattering, we investigate the role of interstitial iron on the low-energy spin fluctuations in powder samples of Fe_{1+x}Te_{0.7}Se_{0.3}. We demonstrate how combining the principle of detailed balance along with…

Superconductivity · Physics 2015-06-04 C. Stock , E. E. Rodriguez , M. A. Green

Y0.5Ca0.5BaCo4O7 was recently introduced as a possible candidate for capturing some of the predicted classical spin kagome ground state features. Stimulated by this conjecture we have taken up a more complete study of the spin correlations…

Strongly Correlated Electrons · Physics 2015-03-17 J R Stewart , G Ehlers , H Mutka , C Payen , P Fouquet , R Lortz

Frustration-induced strong quantum fluctuations accompanied by spin-orbit coupling and crystal electric field can give rise to rich and diverse magnetic phenomena associated with unconventional low-energy excitations in rare-earth based…

Strongly Correlated Electrons · Physics 2024-02-13 J. Khatua , S. Bhattacharya , A. M. Strydom , A. Zorko , J. S. Lord , A. Ozarowski , E. Kermarrec , P. Khuntia

We report microwave spectroscopy of $^{167}$Er$^{3+}$ doped in CaWO$_4$ which reveals the hyperfine splitting of the erbium electronic ground state ($Z_1$, $J_\mathrm{eff.}$=15/2) induced by the $I$=7/2 nuclear spin. From spectra measured…

The electron spin decay lifetime in materials can be characterized by relaxation (T1) and irreversible (T2) and reversible (T2*) decoherence processes. Their interplay leads to a complex dependence of spin relaxation times on the direction…

Kitaev interactions, arising from the interplay of frustration and bond anisotropy, can lead to strong quantum fluctuations and, in an ideal case, to a quantum-spin-liquid state. However, in many nonideal materials, spurious non-Kitaev…

Spins in silicon that are accessible via a telecom-compatible optical transition are a versatile platform for quantum information processing that can leverage the well-established silicon nanofabrication industry. Key to these applications…

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