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The coupling of resonant light and surface plasmons in metal layer coated optical microcavities results in the formation of hybrid photon-plasmon modes. Here, we comprehensively investigate the hybridization mechanism of photon-plasmon…

Hybrid photonic-plasmonic cavities have emerged as a new platform to increase light-matter interaction capable to enhance the Purcell factor in a singular way not attainable with either photonic or plasmonic cavities separately. In the…

Radiation-matter hybridization allows atoms to serve as mediators of effective interactions between light modes and, conversely, to interact among themselves via light. Here we exploit the spatial structure of atomic ensembles to control…

Quantum Physics · Physics 2026-05-06 Carlos E. Máximo , Romain Bachelard , Tobias Donner

From fundamental discovery to practical application, advances in the optical and quantum sciences rely upon precise control of light-matter interactions. Systems of coupled optical cavities are ubiquitous in these efforts, yet design and…

Optics · Physics 2020-04-22 Kevin C. Smith , Yueyang Chen , Arka Majumdar , David J. Masiello

Proton transfer is ubiquitous in many fundamental chemical and biological processes, and the ability to modulate and control the proton transfer rate would have a major impact on numerous quantum technological advances. One possibility to…

Chemical Physics · Physics 2021-12-07 Fabijan Pavošević , Sharon Hammes-Schiffer , Angel Rubio , Johannes Flick

Manipulation of chemical reactivity often involves changing reagents or environmental conditions. Alternatively, strong coupling between light and matter offers a way to tunably hybridize their physicochemical properties and thereby change…

Quantum Physics · Physics 2018-11-19 Matthew Du , Raphael F. Ribeiro , Joel Yuen-Zhou

Intermolecular bonds are weak compared to covalent bonds, but they are strong enough to influence the properties of large molecular systems. In this work, we investigate how strong light-matter coupling inside an optical cavity can modify…

Chemical Physics · Physics 2021-03-17 Tor S. Haugland , Christian Schäfer , Enrico Ronca , Angel Rubio , Henrik Koch

When the interaction between a molecular system and confined light modes in an optical or plasmonic cavity is strong enough to overcome the dissipative process, hybrid light-matter states (polaritons) become the fundamental excitations in…

Mesoscale and Nanoscale Physics · Physics 2020-01-08 Yu Zhang , Tammie Nelson , Sergei Tretiak

Strong coupling of molecules to vacuum fields has been widely reported to lead to modified chemical properties such as reaction rates. However, some recent attempts to reproduce infrared strong coupling results have not been successful,…

Mesoscale and Nanoscale Physics · Physics 2024-01-03 Philip A. Thomas , Wai Jue Tan , Vasyl G. Kravets , Alexander N. Grigorenko , William L. Barnes

Reversible exchange of photons between a material and an optical cavity can lead to the formation of hybrid light--matter states where material properties such as the work function\cite{Hutchison_AM2013a}, chemical…

We report that hybridizing semiconductor quantum dots with plasmonic metamaterial leads to a multi-fold intensity increase and narrowing of their photoluminescence spectrum. The luminescence enhancement is a clear manifestation of the…

Optics · Physics 2015-03-17 K. Tanaka , E. Plum , J. Y. Ou , T. Uchino , N. I. Zheludev

The standard description of cavity-modified molecular reactions typically involves a single (resonant) mode, while in reality the quantum cavity supports a range of photon modes. Here we demonstrate that as more photon modes are accounted…

Mesoscale and Nanoscale Physics · Physics 2020-07-15 Norah M. Hoffmann , Lionel Lacombe , Angel Rubio , Neepa T. Maitra

The increased decay rate of a two-level system weakly coupled to an optical cavity, known as the Purcell effect, is a cornerstone of cavity QED. However, the effect of cavity coupling is not well understood if the two-level system is…

Quantum Physics · Physics 2023-06-19 Charlie Nation , Valentina Notararigo , Alexandra Olaya-Castro

Hybrid photonic-plasmonic cavities can be tailored to display high Q-factors and extremely small mode volumes simultaneously, which results in large values of the Purcell factor, FP. Amongst the different hybrid configurations, those based…

Strong light-induced interactions between atoms are known to cause nonlinearities at a few-photon level which are crucial for applications in quantum information processing. Compared to free space, the scattering and the light-induced…

Quantum Physics · Physics 2021-12-22 Artur Skljarow , Harald Kübler , Charles S. Adams , Tilman Pfau , Robert Löw , Hadiseh Alaeian

The strong coupling between molecules and photons in resonant cavities offers a new toolbox to manipulate photochemical reactions. While the quenching of photochemical reactions in the strong coupling regime has been demonstrated before,…

Mesoscale and Nanoscale Physics · Physics 2019-12-24 Jacop Fregoni , Giovanni Granucci , Maurizio Persico , Stefano Corni

The light-matter interaction can be utilized to qualitatively alter physical properties of materials. Recent theoretical and experimental studies have explored this possibility of controlling matter by light based on driving many-body…

Mesoscale and Nanoscale Physics · Physics 2020-11-11 Yuto Ashida , Atac Imamoglu , Jerome Faist , Dieter Jaksch , Andrea Cavalleri , Eugene Demler

When two or more metallic nanoparticles are in close proximity, their plasmonic modes may interact through the near field, leading to additional resonances of the coupled system or to shifts of their resonant frequencies. This process is…

The interaction between molecules and surface plasmons in defined geometries can lead to new light mater hybrid states where light propagation is strongly influenced by molecular photon absorption. Their application range from lasing LEDs…

Physical and chemical properties of materials can be modified by a resonant optical mode. Such recent demonstrations have mostly relied on a planar cavity geometry, others have relied on a plasmonic resonator. However, the combination of…

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