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Electron-phonon (e-ph) interactions are usually treated in the lowest order of perturbation theory. Here we derive next-to-leading order e-ph interactions, and compute from first principles the associated two-phonon e-ph scattering rates.…

Mesoscale and Nanoscale Physics · Physics 2020-10-06 Nien-En Lee , Jin-Jian Zhou , Hsiao-Yi Chen , Marco Bernardi

Time-resolved diffuse scattering experiments have gained increasing attention due to their potential to reveal non-equilibrium dynamics of crystal lattice vibrations with full momentum resolution. Although progress has been made in…

From ultraviolet to mid-infrared region, light-matter interaction mechanisms in semiconductors progressively shift from electronic transitions to phononic resonances and are affected by temperature. Here, we present a parallel…

Optics · Physics 2023-06-01 Zherui Han , Changkyun Lee , Jiawei Song , Haiyan Wang , Peter Bermel , Xiulin Ruan

The calculation of electron-phonon (e-ph) coupling from first principles is a topic of great interest in materials science, offering a robust, non-empirical framework to understand and predict a wide range of physical phenomena. While…

Materials Science · Physics 2025-03-17 Savio Laricchia , Casey Eichstaedt , Dimitar Pashov , Mark van Schilfgaarde

Modeling spin-wave (magnon) dynamics in novel materials is important to advance spintronics and spin-based quantum technologies. The interactions between magnons and lattice vibrations (phonons) limit the length scale for magnon transport.…

We present a new first-principles linear-response theory of changes due to perturbations in the quasiparticle self-energy operator within the $GW$ method. This approach, named $GW$ perturbation theory ($GW$PT), is applied to calculate the…

Materials Science · Physics 2019-05-15 Zhenglu Li , Gabriel Antonius , Meng Wu , Felipe H. da Jornada , Steven G. Louie

In a polar solid, electrons or other charge carriers can interact with the phonons of the ionic lattice, leading to the formation of polaron quasiparticles. The optical conductivity and optical absorption spectrum of a material are affected…

Materials Science · Physics 2023-01-04 Matthew Houtput , Jacques Tempere

We present a novel approach to electron-lattice interaction beyond the linear-coupling regime. Based on the solution of a Holstein-Peierls-type model, we derive explicit analytical expressions for the eigenvalue spectrum of the Hamiltonian,…

Materials Science · Physics 2018-12-13 Pablo García Risueño , Dmitrii Nabok , Qiang Fu , Claudia Draxl

The study of electron-phonon interaction as a prominent inelastic effect is of great importance. In the present work, we have studied the inelastic effects due to the first order electron-phonon interactions on electronic properties of…

Mesoscale and Nanoscale Physics · Physics 2016-09-30 Mujtaba Zahidy , Fatemeh Ghadirian , Afshin Namiranian

Ab initio downfolding describes the electronic structure of materials within a low-energy subspace, often around the Fermi level. Typically starting from mean-field calculations, this framework allows for the calculation of one- and…

We use both a perturbative Green's function analysis and standard perturbative quantum mechanics to calculate the decrease in energy and the effective mass for an electron interacting with acoustic phonons. The interaction is between the…

Strongly Correlated Electrons · Physics 2011-02-11 Zhou Li , Carl J. Chandler , F. Marsiglio

Structural phase transitions and soft phonon modes pose a longstanding challenge to computing electron-phonon (e-ph) interactions in strongly anharmonic crystals. Here we develop a first-principles approach to compute e-ph scattering and…

Materials Science · Physics 2018-12-04 Jin-Jian Zhou , Olle Hellman , Marco Bernardi

$Ab-initio$ probabilities of phonon-assisted intervalley scattering of electrons in the conduction bands of ternary chalcopyrite compounds $ZnSiP_2$ and $ZnGeP_2$ between the central $\Gamma$ minima and the lowest lateral minima (valleys)…

Materials Science · Physics 2019-10-08 V. G. Tyuterev

We present a first-principles study of the temperature- and density-dependent intrinsic electrical resistivity of graphene. We use density-functional theory and density-functional perturbation theory together with very accurate Wannier…

Rutile TiO2 is a paradigmatic transition metal oxide with applications in optics, electronics, photocatalysis, etc., that are subject to pervasive electron-phonon interaction. To understand how energies of its electronic bands, and in…

The effect of Holstein electron-phonon interaction on a Hubbard model close to a Mott-Hubbard transition at half-filling is investigated by means of Dynamical Mean-Field Theory. We observe a reduction of the effective mass that we interpret…

Strongly Correlated Electrons · Physics 2007-08-07 G. Sangiovanni , M. Capone , C. Castellani , M. Grilli

Using the Feynman path-integral formalism we study the polaron effects in quantum wires above a liquid helium film. The electron interacts with two-dimensional (2D) surface phonons, i.e. ripplons, and is confined in one dimension (1D) by an…

Strongly Correlated Electrons · Physics 2009-11-07 G. A. Farias , R. N. Costa Filho , F. M. Peeters , Nelson Studart

We consider electron-electron interaction effects in quantum point contacts on the first quantization plateau, taking into account all scattering processes. We compute the low-temperature linear and nonlinear conductance, shot noise, and…

Mesoscale and Nanoscale Physics · Physics 2009-02-27 A. M. Lunde , A. De Martino , A. Schulz , R. Egger , K. Flensberg

The effect of the electron-phonon interaction on magnetization relaxation is studied within the framework of first-principles scattering theory for Fe, Co, and Ni by displacing atoms in the scattering region randomly with a thermal…

Materials Science · Physics 2011-09-06 Yi Liu , Anton A. Starikov , Zhe Yuan , Paul J. Kelly

The formation of a polaron quasiparticle from a bare electron is studied in the framework of the Holstein model of electron-phonon coupling. Using Schr\"{o}dinger's formalism, we calculate the time evolution of the distribution of the…

Strongly Correlated Electrons · Physics 2007-05-23 Li-Chung Ku , S. A. Trugman