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Non-resonant ferromagnetic x-ray diffraction has been used to separate the spin and orbital contribution to the magnetization density of the proposed zero-moment ferromagnet $Sm_{0.982}Gd_{0.018} Al_{2}$. The alignment of the spin and…

Condensed Matter · Physics 2009-11-07 J. W. Taylor , J. A. Duffy , A. M. Bebb , M. R. Lees , L. Bouchenoire , S. D. Brown , M. J. Cooper

We explore spin dynamics in Cu(1,3-bdc), a quasi-2D topological magnon insulator. The results show that the thermal evolution of Land\'e $g$-factor ($g$) is anisotropic: $g_\textrm{in-plane}$ reduces while $g_\textrm{out-plane}$ increases…

We derive a quantum-mechanical formula of the orbital magnetic quadrupole moment (MQM) in periodic systems by using the gauge-covariant gradient expansion. This formula is valid for insulators and metals at zero and finite temperature. We…

Materials Science · Physics 2018-07-25 Atsuo Shitade , Hikaru Watanabe , Youichi Yanase

The ratio of orbital (L) and spin (S) contributions to the magnetically ordered moments of a 5d transition metal oxide, Sr2IrO4 was evaluated by non-resonant magnetic x-ray diffraction. We applied a new experimental setting to minimize the…

Strongly Correlated Electrons · Physics 2014-05-26 S. Fujiyama , H. Ohsumi , K. Ohashi , D. Hirai , B. J. Kim , T. Arima , M. Takata , H. Takagi

In experiments and applications usually the spin magnetic moment of magnons is considered. In this Paper we identify an additional degree of freedom of magnons: an \emph{orbital} magnetic moment brought about by spin-orbit coupling.Our…

Strongly Correlated Electrons · Physics 2020-09-16 Robin R. Neumann , Alexander Mook , Jürgen Henk , Ingrid Mertig

We report an unusual canted magnetism due to 3d and 4f electrons, occupying two different crystallographic sites, with its consequence to electric dipole order. This is based on neutron powder diffraction measurements on Tb2BaNiO5…

The addition of magnetic impurities in topological insulators can drive ferromagnetic order that leads to novel quantum anomalous Hall transport well below the Curie temperature. The fragility of the quantized regime has been ascribed to…

The weak antiferromagnetism of URu${}_{2}$Si${}_{2}$ is discussed on the basis of a duality model which takes into account salient features of both itinerant fermions and "localized" component of spin degrees of freedom. The problem is…

Strongly Correlated Electrons · Physics 2009-10-31 Yukihiro Okuno , Kazumasa Miyake

A spin-orbital superexchange Hamiltonian in a Mott insulator with $t_{2g}$ orbital degeneracy is investigated. More specifically, we focus on a spin ferromagnetic state of the model and study a collective behavior of orbital angular…

Strongly Correlated Electrons · Physics 2009-11-11 G. Khaliullin , S. Okamoto

The role of orbital ordering on metal-insulator transition of transition-metal oxides is investigated by the cluster self-consistent field approach in the strong correlation regime. A clear dependence of the insulating gap on the orbital…

Strongly Correlated Electrons · Physics 2007-09-25 Dong-Meng Chen , Liang-Jian Zou

We apply the finite-temperature variational cluster approach to a strongly correlated and spin-orbit coupled model for four electrons (i.e. two holes) in the $t_{2g}$ subshell. We focus on parameters suitable for antiferromagnetic Mott…

Strongly Correlated Electrons · Physics 2021-07-21 Jan Lotze , Maria Daghofer

We have performed x-ray linear and circular magnetic dichroism experiments at the Mn L2,3-edge of the La0.7Sr0.3MnO3 ultra thin films. Our measurements show that the antiferromagnetic (AF) insulating phase is stabilized by the interfacial…

Strongly Correlated Electrons · Physics 2009-07-29 C. Aruta , G. Ghiringhelli , V. Bisogni , L. Braicovich , N. B. Brookes , A. Tebano , G. Balestrino

The magnetoelectric effect has been actively studied in multiferroics since the first observation in an antiferromagnetic, $\mathrm{Cr_2O_3}$. This effect appears in systems without spatial inversion symmetry and time-reversal symmetry and…

Materials Science · Physics 2023-07-05 Koki Shinada , Robert Peters

Carrying information using generation and detection of the orbital current, instead of the spin current, is an emerging field of research, where the orbital Hall effect (OHE) is an important ingredient. Here, we propose a new mechanism of…

Materials Science · Physics 2020-04-22 Sayantika Bhowal , S. Satpathy

Motivated by experimental and theoretical interest in realizing multipolar orders in $d$-orbital materials, we discuss the quantum magnetism of $J\!=\!2$ ions which can be realized in spin-orbit coupled oxides with $5d^2$ transition metal…

Strongly Correlated Electrons · Physics 2020-03-18 Arun Paramekanti , Dalini D. Maharaj , Bruce D. Gaulin

Using first-principles electronic structure calculation, we demonstrate the spin dissipation process in bulk Fe by orbital excitations within the energy bands of pure spin character. The variation of orbitals in the intraband transitions…

Mesoscale and Nanoscale Physics · Physics 2025-04-02 Yue Chen , Haoran Chen , Xi Shen , Weizhao Chen , Yi Liu , Yizheng Wu , Zhe Yuan

We present a detailed low-energy muon spin rotation and x-ray magnetic circular dichroism (XMCD) investigation of the magnetic structure in ultra-thin tetragonal (T)-CuO films. The measured muon-spin polarization decay indicates an…

The electric-field control of $d$-electron magnetism in multiferroic transition metal oxides is attracting widespread interest for the underlying fundamental physics and for next generation spintronic devices. Here, we report an extensive…

Materials Science · Physics 2021-05-26 D. Preziosi , S. Homkar , C. Lefevre , M. Salluzzo , N. Viart

We report current-direction dependent or unidirectional magnetoresistance (UMR) in magnetic/nonmagnetic topological insulator (TI) heterostructures, Cr$_x$(Bi$_{1-y}$Sb$_y$)$_{2-x}$Te$_3$/(Bi$_{1-y}$Sb$_y$)$_2$Te$_3$, that is several orders…

Materials Science · Physics 2016-11-03 K. Yasuda , A. Tsukazaki , R. Yoshimi , K. S. Takahashi , M. Kawasaki , Y. Tokura

The orbital contribution to the magnetic moment of the transition metal ion in the isostructural weak ferromagnets ACO$_3$ (A=Mn,Co,Ni) and FeBO$_3$ was investigated by a combination of first-principles calculations, non-resonant x-ray…

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