Related papers: Exploiting SU(N ) dynamical symmetry for rovibroni…
A coherent control scheme for the population distribution in the vibrational states of nonpolar molecules is proposed. Our theoretical analysis and results of numerical simulations for the interaction of the hydrogen molecular ion in its…
We formulate the theory for a diatomic molecule in a spatially degenerate electronic state interacting with a non-resonant laser field and investigate its rovibrational structure in the presence of the field. We report on \textit{ab initio}…
We propose a modified Stark-chirped rapid adiabatic passage technique for a robust rovibrational population transfer in the gas phase molecules in the presence of certain inhomogeneous electric fields. As an example application, the new…
We propose a class of schemes for robust population transfer between quantum states that utilize trains of coherent pulses and represent a generalized adiabatic passage via a wave packet. We study piecewise Stimulated Raman Adiabatic…
The controlled transfer of nuclear state population using two x-ray laser pulses is investigated theoretically. The laser pulses drive two nuclear transitions in a nuclear three-level system facilitating coherent population transfer via the…
We demonstrate a method of adiabatic population transfer from a single quantum state into a coherent superposition of states. The transfer is executed with femtosecond pulses, spectrally shaped in simple and intuitive manner, which does not…
We develop a method for executing robust and selective transfer of populations between a single level and pre-selected superpositions of energy eigenstates. Viewed in the frequency domain, our method amounts to executing a series of…
We propose and demonstrate the method of population transfer by piecewise adiabatic passage between two quantum states. Coherent excitation of a two-level system with a train of ultrashort laser pulses is shown to reproduce the effect of an…
High fidelity and robustness in population inversion is very desirable for many quantum control applications. We expand composite pulse schemes developed for two-level dynamics, and present an analytic solution for the coherent evolution of…
The transfer of weakly bound KRb molecules from levels just below the dissociation threshold into the vibrational ground state with shaped laser pulses is studied. Optimal control theory is employed to calculate the pulses. The complexity…
We consider the dynamics of a single electron in a chain of tunnel coupled quantum dots, exploring the formal analogies of this system with some of the laser-driven multilevel atomic or molecular systems studied by Bruce W. Shore and…
We derive the non-adiabatic ring polymer molecular dynamics (RPMD) approach in the phase space of the SU(N) Lie Group. This method, which we refer to as the spin mapping non-adiabatic RPMD (SM-NRPMD), is based on the spin-mapping formalism…
Accurate population transfer of uncoupled or weakly coupled spin states is crucial for many quantum information processing tasks. In this paper, we propose a fast and robust scheme for population transfer which combines invariant-based…
In the construction of diabatic vibronic Hamiltonians for quantum dynamics in the excited-state manifold of molecules, the coupling constants are often extracted solely from information on the excited-state energies. Here, a new protocol is…
Bare-state population inversion is demonstrated in a two-level system with all dipole matrix elements nonzero. A laser field is resonantly driving the sample whereas a second weaker and lower frequency coherent field additionally pumps it…
We propose a method to transfer the population and control the state of two-level and three-level atoms speeding-up Adiabatic Passage techniques while keeping their robustness versus parameter variations. The method is based on…
We propose a method for achieving highly efficient transfer between the vibrational states in a diatomic molecule. The process is mediated by strong laser pulses and can be understood in terms of light-induced potentials. In addition to…
High-fidelity coherent population transfer plays a vital role in the realization of quantum memories. However, population transfer with high performance across a broad frequency range is still challenging due to the finite Rabi coupling…
An automated and robust method for adiabatic population transfer and the preparation of an arbitrary quantum superposition state in atomic system using the oscillating dark states (ODS) is presented. Quantum state of a three-level $\Lambda$…
We propose and analyze a robust population-transfer protocol in a driven two-level system based on a sudden sign change of the detuning at the maximum of a smooth coupling pulse. Away from the jump the dynamics is adiabatic, while the sign…