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Quantum cascade laser (QCL) frequency combs have revolutionized mid-infrared (MIR) spectroscopy by their high brightness and fast temporal resolution, and are a promising technology for fully-integrated and cost-effective sensors. As for…

Robust control and stabilization of optical frequency combs enables an extraordinary range of scientific and technological applications, including frequency metrology at extreme levels of precision, novel spectroscopy of quantum gases and…

Optics · Physics 2013-08-09 Scott B. Papp , Pascal Del'Haye , Scott A. Diddams

The advent of optical frequency standards with ultimate uncertainties in the low 1x10$^{-18}$ requires femtosecond frequency combs to support a similar level of resolution in the spectral transfer and the computation of optical frequency…

Instrumentation and Detectors · Physics 2022-05-31 Matias Risaro , Paolo Savio , Marco Pizzocaro , Filippo Levi , Davide Calonico , Cecilia Clivati

Mode-resolved dual-comb spectroscopy (DCS) is an emerging spectroscopic tool with the potential to simultaneously achieve a broad spectral coverage and ultrahigh spectral resolution in terahertz (THz) spectroscopy. However, the need for two…

Instrumentation and Detectors · Physics 2020-06-02 Jie Chen , Kazuki Nitta , Xin Zhao , Takahiko Mizuno , Takeo Minamikawa , Francis Hindle , Zheng Zheng , Takeshi Yasui

Photonic analog to digital conversion offers promise to overcome the signal-to-noise ratio (SNR) and sample rate trade-off in conventional analog to digital converters (ADCs), critical for modern digital communications and signal analysis.…

Signal Processing · Electrical Eng. & Systems 2019-09-09 Callum Deakin , Zhixin Liu

We demonstrate phase locking of a 729 nm diode laser to a 1542 nm master laser via an erbium-doped-fiber frequency comb, using a transfer-oscillator feedforward scheme which suppresses the effect of comb noise in an unprecedented 1.8 MHz…

Mid-infrared high-resolution spectroscopy has proven an invaluable tool for the study of the structure and dynamics of molecules in the gas phase. The advent of frequency combs advances the frontiers of precise molecular spectroscopy. Here…

Optics · Physics 2019-02-28 Zaijun Chen , Theodor W. Hänsch , Nathalie Picqué

Dual-comb spectroscopy is a powerful technique to measure optical spectra in a wide spectral range with high-frequency resolution. The development of compact systems operating in the long-wave infrared wavelength range is of high interest…

Dual-comb spectroscopy typically requires the utilization of two independent and phase-locked femtosecond lasers, resulting in a complex and expensive system that hinders its industrial applications. Single-cavity dual-comb lasers are…

Optics · Physics 2024-04-16 Ruixin Tang , Ziyu Luo , Pengfei Li , Pengrun Ying , Haiyang Xie , Siyuan Xu , Hui Liu , Jintao Bai

We demonstrate the performance of a dual frequency comb QCL spectrometer for the application of vibrational Stark spectroscopy. Measurements performed on fluorobenzene with the dual-comb spectrometer (DCS) were compared to results obtained…

Chemical Physics · Physics 2019-11-22 Urszula Szczepaniak , Samuel H. Schneider , Raphael Horvath , Jacek Kozuch , Markus Geiser

We describe a possible new technique for precise wavelength calibration of high-resolution astronomical spectrographs using femtosecond-pulsed mode-locked lasers controlled by stable oscillators such as atomic clocks. Such `frequency combs'…

Optical frequency combs provide a phase-coherent interface between optical and microwave domains, underpinning advances in precision metrology, spectroscopy, and time-frequency transfer. Most conventional comb architectures are limited to…

Spectral analysis is one of the most powerful technologies for studying and understanding matter. As the devices for spectral analysis, spectrometers are widely used in material detection, isotope analysis, trace gas detection, and the…

Fiber-optical networks are a crucial telecommunication infrastructure in society. Wavelength division multiplexing allows for transmitting parallel data streams over the fiber bandwidth, and coherent detection enables the use of…

Signal Processing · Electrical Eng. & Systems 2020-02-19 Lars Lundberg , Mikael Mazur , Ali Mirani , Benjamin Foo , Jochen Schröder , Victor Torres-Company , Magnus Karlsson , Peter A. Andrekson

An optical frequency comb generated with an electro-optic phase modulator and a chirped radiofrequency waveform is used to perform saturation and pump-probe spectroscopy on the $D_1$ and $D_2$ transitions of atomic potassium. With a comb…

Atomic Physics · Physics 2016-12-21 David A. Long , Adam J. Fleisher , David F. Plusquellic , Joseph T. Hodges

Carrier-envelope phase stabilization of optical pulses enables exquisitely precise measurements by way of direct optical-frequency synthesis, absolute optical-to-microwave phase conversion, and control of ultrafast waveforms. We report such…

We demonstrate dual-comb spectroscopy based on difference frequency generation of frequency-agile near-infrared frequency combs, produced with the help of electro-optic modulators. The combs have a remarkably flat intensity distribution and…

A laser frequency combs is a broad spectrum composed of equidistant narrow lines. Initially invented for frequency metrology, such combs enable new approaches to spectroscopy over broad spectral bandwidths, of particular relevance to…

Optics · Physics 2019-03-01 Nathalie Picqué , Theodor W. Hänsch

Holography has always held special appeal, for it is able to record and display spatial information in three dimensions. Here, we show how to augment the capabilities of digital holography by using a large number of narrow laser lines at…

High resolution and fast detection of molecular vibrational absorption is important for organic synthesis, pharmaceutical process and environmental monitoring, and is enabled by mid-infrared (mid-IR) laser frequency combs via dual-comb…

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