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The field of attosecond physics has expanded significantly in recent years, yet experimental facilities supporting attosecond pump attosecond probe spectroscopy remain rare. Here, we present a newly constructed beamline for the generation…
A feasible method is proposed to generate isolated attosecond terawatt x-ray radiation pulses in high-gain free-electron lasers. In the proposed scheme, a frequency chirped laser pulse is employed to generate a gradually-varied spacing…
We characterized spatially resolved spectral phase interferometry with an isolated attosecond pulse (IAP). The measured spatial-spectral interferogram and spectral interference fringe visibility show a high degree of IAPs spatial and…
Natively, atomic and molecular processes develop in a sub-femtosecond time scale. In order to, for instance, track and capture the electron motion in that scale we need suitable `probes'. Attosecond pulses configure the most appropriate…
Lasers capable of generating attosecond X-ray pulses in the water window (282 to 533 eV) through high-order harmonic generation are normally based on inefficient, multi-stage optical parametric amplifiers or optical parametric chirped pulse…
We theoretically investigate the generation of higher harmonics and the construction of a single attosecond pulse by means of two oppositely polarized sinc-shaped driver pulses. In comparison to a few-cycle Gaussian pulse of the same…
We report on new routes to generating a train of attosecond pulses. The methods are extremely simple and robust; we need to place only a few thin dispersive materials in the optical path. We numerically demonstrate the generation of a train…
Attosecond pulses can be used to initiate and control electron dynamics on a sub-femtosecond time scale. The first step in this process occurs when an atom absorbs an ultraviolet photon leading to the formation of an attosecond electron…
Sub-10-attosecond pulses with half-cycle electric fields provide exceptional options to detect and manipulate electrons in the atomic timescale. However, the availability of such pulses is still challenging. Here, we propose a method to…
A practical approach is proposed for efficiently generating ultrashort attosecond pulses (APs) from realistic solid-state materials, aiming to optimize pulse width effectively. By adjusting the photon energy while maintaining a constant…
Raman amplification in plasma has been promoted as a means of compressing picosecond optical laser pulses to femtosecond duration to explore the intensity frontier. Here we show for the first time that it can be used, with equal success, to…
The birth of attosecond light sources is expected to inspire a breakthrough in ultrafast optics, which may extend human real-time measurement and control techniques into atomic-scale electronic dynamics. For applications, it is essential to…
We report the synthesis of arbitrary optical waveforms by manipulating the spectral phases of Raman sidebands with a wide frequency spacing line-by-line. Trains of rectangular and triangular pulses are stably produced at an ultrahigh…
The waveforms of attosecond pulses produced by high-harmonic generation carry information on the electronic structure and dynamics in atomic and molecular systems. Current methods for the temporal characterization of such pulses have…
We propose an idea of an electronic multi-channel arbitrary digital sequence generator with temporal granularity equal to a single clock cycle. We implement the generator with 32 channels using a low-cost ARM microcontroller and demonstrate…
Parametric amplification of attosecond coherent pulses around 100 eV at the single-atom level is demonstrated for the first time by using the 3D time-dependent Schr{\"o}dinger equation in high-harmonic generation processes from excited…
The generation of single-cycle attosecond pulses based on Thomson scattering of terahertz (THz) pulses is proposed. In the scheme, a high-quality relativistic electron beam produced by a laser-plasma wakefield accelerator (LPWA), is sent…
We demonstrate that by filtering high harmonics it is possible to obtain two different single attosecond pulses (SAP) resulting from naturally separated spectral domains formed during propagation in the macroscopic medium. We propose a…
The availability of intense, ultrashort coherent radiation sources in the infrared region of the spectrum is enabling the generation of attosecond X-ray pulses via high harmonic generation, pump-probe experiments in the "molecular…
In this work we demonstrate the generation of two intense, ultrafast laser pulses that allow a controlled interferometric measurement of higher harmonic generation pulses with 12.8 attoseconds in resolution (half the atomic unit of time)…