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Non-monotonous changes in velocity autocorrelations across the transformation from molecular to atomic fluid in hydrogen under pressure are studied by ab initio molecular dynamics simulations at the temperature 2500 K. We report diffusion…

Soft Condensed Matter · Physics 2020-05-27 G. Ruocco , T. Bryk , C. Pierleoni , A. P. Seitsonen

We present results of molecular dynamics simulations of the electron system on the surface of liquid helium. The simulations are done for 1600 electrons with periodic boundary conditions. Electron scattering by capillary waves and phonons…

Mesoscale and Nanoscale Physics · Physics 2018-09-03 K. Moskovtsev amd M. I. Dykman

We present a model for the motion of an average atom in a liquid or supercooled liquid state and apply it to calculations of the velocity autocorrelation function $Z(t)$ and diffusion coefficient $D$. The model trajectory consists of…

Statistical Mechanics · Physics 2009-10-31 Eric D. Chisolm , Brad E. Clements , Duane C. Wallace

The motion of the structure determining components is highly collective, both in amorphous solids and in undercooled liquids. This has been deduced from experimental low temperature data in the tunneling regime as well as from the vanishing…

Disordered Systems and Neural Networks · Physics 2009-11-07 H. R. Schober

Self-diffusion in a two-dimensional simple fluid is investigated by both analytical and numerical means. We investigate the anomalous aspects of self-diffusion in two-dimensional fluids with regards to the mean square displacement, the…

Soft Condensed Matter · Physics 2018-09-05 Bongsik Choi , Kyeong Hwan Han , Changho Kim , Peter Talkner , Akinori Kidera , Eok Kyun Lee

We study the contribution of advection by thermal velocity fluctuations to the effective diffusion coefficient in a mixture of two identical fluids. The steady-state diffusive flux in a finite system subject to a concentration gradient is…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 A. Donev , A. de la Fuente , J. B. Bell , A. L. Garcia

A theoretical model of the formation of an amorphous phase during the quenching of a metallic melt is proposed. It has been shown that the appearance of a significant temperature gradient during the quenching of a metallic melt leads to…

Materials Science · Physics 2025-04-29 A. I. Karasevskii , A. Yu. Naumuk

We discuss the dependence of self- and interdiffusion coefficients on temperature and composition for two prototypical binary metallic melts, Al-Ni and Zr-Ni, in molecular-dynamics (MD) computer simulations and the mode-coupling theory of…

Materials Science · Physics 2014-08-12 P. Kuhn , J. Horbach , F. Kargl , A. Meyer , Th. Voigtmann

Self-diffusion and radial distribution functions are studied in a strongly confined Lennard-Jones fluid. Surprisingly, in the solid-liquid phase transition region, where the system exhibits dynamic coexistence, the self-diffusion constants…

Statistical Mechanics · Physics 2016-02-11 N. de Sousa , J. J. Sáenz , Frank Scheffold , A. García Martín , L. S. Froufe-Pérez

A combination of experimental techniques and molecular dynamics (MD) computer simulation is used to investigate the diffusion dynamics in Al80Ni20 melts. Experimentally, the self-diffusion coefficient of Ni is measured by the long-capillary…

Disordered Systems and Neural Networks · Physics 2009-11-13 Juergen Horbach , Subir K. Das , Axel Griesche , Michael-Peter Macht , Guenter Frohberg , Andreas Meyer

The linear response description for impurity diffusion in a granular fluid undergoing homogeneous cooling is developed in the preceeding paper. The formally exact Einstein and Green-Kubo expressions for the self-diffusion coefficient are…

Soft Condensed Matter · Physics 2009-11-07 James Lutsko , J. Javier Brey , James W. Dufty

We report a study on the static and dynamic properties of several liquid 5$d$ transition metals at thermodynamic conditions near their respective melting points. This is performed by resorting to ab initio molecular dynamics simulations in…

Statistical Mechanics · Physics 2023-08-15 D. J. González , L. E. González

Using molecular dynamics simulation, we calculate the distribution of atomic jum ps in Cu$_{33}$Zr$_{67}$ in the liquid and glassy states. In both states the distribution of jump lengths can be described by a temperature independent…

Disordered Systems and Neural Networks · Physics 2009-11-11 M. Kluge , H. R. Schober

Flame propagation through a non-volatile solid-fuel suspension is studied using a simplified, time-dependent numerical model that considers the influence of both diffusional and kinetic rates on the particle combustion process. It is…

We expand on a recent study of a lattice model of interacting particles [Phys. Rev. Lett. 111, 110601 (2013)]. The adsorption isotherm and equilibrium fluctuations in particle number are discussed as a function of the interaction. Their…

Statistical Mechanics · Physics 2014-11-20 T. Becker , K. Nelissen , B. Cleuren , B. Partoens , C. Van den Broeck

Understanding the retention of hydrogen isotopes in liquid metals, such as lithium and tin, is of great importance in designing a liquid plasma-facing component in fusion reactors. However, experimental diffusivity data of hydrogen isotopes…

Soft Condensed Matter · Physics 2017-10-02 Xiaohui Liu , Daye Zheng , Xinguo Ren , Lixin He , Mohan Chen

It was found recently that the liquid dynamics of several metals (Li, Zn, Ni, Fe, Tl, Pb) under pressure is characterized by transverse spectral functions containing an additional high-frequency peak. To rationalize the pressure dependence…

Soft Condensed Matter · Physics 2023-08-15 J. -F. Wax , N. Jakse

A microemulsion of decane droplets stabilized by a non-ionic surfactant film is progressively charged by substitution of a non-ionic surfactant molecule by a cationic surfactant. We check that the microemulsion droplets remain identical…

Soft Condensed Matter · Physics 2016-08-16 Jacqueline Appell , Grégoire Porte , Eric Buhler

Reactive Rayleigh-Taylor systems are characterized by the competition between the growth of the instability and the rate of reaction between cold (heavy) and hot (light) phases. We present results from state-of-the-art numerical simulations…

Fluid Dynamics · Physics 2011-02-14 A. Scagliarini , L. Biferale , F. Mantovani , M. Sbragaglia , F. Toschi , R. Tripiccione

We investigate the collective dynamics of self-propelled droplets, confined in a one dimensional micro-fluidic channel. On one hand, neighboring droplets align and form large trains of droplets moving in the same direction. On the other…

Soft Condensed Matter · Physics 2020-05-14 Pierre Illien , Charlotte de Blois , Yang Liu , Marjolein N. van der Linden , Olivier Dauchot
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