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An electron diffraction technique is used to study the structure of clusters formed in an isentropically expanding supersonic argon jet. The formation of the hcp phase with increasing cluster size is reliably detected for the first time.…

Atomic and Molecular Clusters · Physics 2007-05-23 Spartak I. Kovalenko , Oleksandr G. Danylchenko , Vladimir N. Samovarov

Understanding the substructure of atomic nuclei, particularly the clustering of nucleons inside them, is essential for comprehending nuclear dynamics. Various cluster configurations can emerge depending on excitation energy, the number and…

This Article presents a nonequilibrium thermodynamic theory for the mean-field precipitation, aggregation and pattern formation of colloidal clusters. A variable gradient energy coefficient and the arrest of particle diffusion upon…

Soft Condensed Matter · Physics 2018-10-17 Thomas Petersen , Martin Z. Bazant , Roland J. M. Pellenq , Franz-Josef Ulm

Recent advances in attosecond spectroscopy techniques have fueled the interest in the theoretical description of electronic processes taking place in the subfemtosecond time scale. Here we study the coupled dynamic screening of a localized…

Atomic and Molecular Clusters · Physics 2013-01-28 N. E. Koval , D. Sánchez-Portal , A. G. Borisov , R. Díez Muiño

Molecular dynamics simulations of nanometer-sized lead clusters have been performed using the Lim, Ong and Ercolessi glue potential (Surf. Sci. {\bf 269/270}, 1109 (1992)). The binding energies of clusters forming crystalline (fcc),…

Condensed Matter · Physics 2009-10-31 S. C. Hendy , B. D. Hall

The optimized structure and electronic properties of neutral and singly charged magnesium clusters have been investigated using ab initio theoretical methods based on density-functional theory and systematic post-Hartree-Fock many-body…

Atomic and Molecular Clusters · Physics 2009-09-29 Andrey Lyalin , Ilia A Solov'yov , Andrey V Solov'yov , Walter Greiner

A unique property of size-resolved metal nanocluster particles is their "superatom"-like electronic shell structure. The shell levels are highly degenerate, and it has been predicted that this can enable exceptionally strong…

Superconductivity · Physics 2015-02-06 Avik Halder , Anthony Liang , Vitaly V. Kresin

We present recent theoretical investigations on the dynamics of metal clusters in contact with an environment, deposited of embedded. This concerns soft deposition as well as irradiation of the deposited/embedded clusters by intense laser…

Atomic and Molecular Clusters · Physics 2010-01-05 P. M. Dinh , P. -G. Reinhard , E. Suraud

The fermionic molecular dynamics approach uses Gaussian wave packets as single-particle basis states. Many-body basis states are Slater determinants projected on parity, angular momentum and total linear momentum. The wave-packet basis is…

Nuclear Theory · Physics 2015-06-11 Thomas Neff

When a chemical bond is broken, the molecular structure undergoes a transformation. An ideal experiment should probe the change in the electronic and nuclear structure simultaneously. Here, we present a method for the simultaneous…

Atomic Physics · Physics 2024-10-11 Saurabh Mhatre , Zack Dube , André Staudte , Stefanie Gräfe , Matthias Kübel

The dynamics following the photoexcitation of Na and Li atoms located on the surface of helium nanodroplets has been investigated in a joint experimental and theoretical study. Photoelectron spectroscopy has revealed that excitation of the…

Atomic and Molecular Clusters · Physics 2017-08-23 Alberto Hernando , Manuel Barranco , Martí Pi , Evgeniy Loginov , Marina Langlet , Marcel Drabbels

Laser excitation of nanometer-sized atomic and molecular clusters offers various opportunities to explore and control ultrafast many-particle dynamics. Whereas weak laser fields allow the analysis of photoionization, excited-state…

Atomic and Molecular Clusters · Physics 2010-06-15 Th. Fennel , K. -H. Meiwes-Broer , J. Tiggesbaumker , P. -G. Reinhard , P. M. Dinh , E. Suraud

A study has been conducted into the mechanisms of evolution of clusters and their subsequent fragmentation under energetic heavy ion bombardment of amorphous graphite. The evolving clusters and their subsequent fragmentation under…

Mesoscale and Nanoscale Physics · Physics 2016-09-14 A. Qayyum , B. Ahmad , M. N. Akhtar , Shoaib Ahmad

Molecular dynamics (MD) simulations were performed to study the cumulative bombardments of low-energy (60-200 eV) helium (He) atoms on tungsten (W) surfaces. The behaviour of He and the response of the W surface were investigated. The He…

Materials Science · Physics 2015-06-18 Min Li , Jiechao Cui , Jun Wang , Qing Hou

Chemically active colloids or enzymes cluster into dense droplets driven by their phoretic response to collectively generated chemical gradients. Employing Brownian dynamics simulation techniques, our study of the dynamics of such a…

Soft Condensed Matter · Physics 2024-01-29 K. R. Prathyusha , Suropriya Saha , Ramin Golestanian

A unique property of metal nanoclusters is the "superatom" shell structure of their delocalized electrons. The electronic shell levels are highly degenerate and therefore represent sharp peaks in the density of states. This can enable…

Superconductivity · Physics 2015-12-17 Avik Halder , Vitaly V. Kresin

Embedded atoms or molecules in a photoexcited He nanodroplet are well-known to be ionized through inter-atomic relaxation in a Penning process. In this work, we investigate the Penning ionization of acetylene oligomers occurring from the…

Atomic and Molecular Clusters · Physics 2020-06-24 S. Mandal , R. Gopal , M. Shcherbinin , A. D'Elia , H. Srinivas , R. Richter , M. Coreno , B. Bapat , M. Mudrich , S. R. Krishnan , V. Sharma

We report a new mechanism for nucleation in a monolayer of hexagonally packed monodisperse droplet arrays. Upon cooling, we observe solidified droplets to nucleate their supercooled neighbors giving rise to an autocatalytic-like mechanism…

Soft Condensed Matter · Physics 2020-04-01 Samira Abedi , Chau-Chyun Chen , Siva A. Vanapalli

The Hamiltonian Mean Field (HMF) model has a low-energy phase where $N$ particles are trapped inside a cluster. Here, we investigate some properties of the trapping/untrapping mechanism of a single particle into/outside the cluster. Since…

Chaotic Dynamics · Physics 2007-11-25 Hiroko Koyama , Tetsuro Konishi , Stefano Ruffo