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Molecular complexes are held together via a variety of bonds, but they all share the common feature that their individual entities are in contact. In this work, we introduce and demonstrate the concept of a \textit{molecular optical bond},…
When an atom is strongly coupled to a cavity, the two systems can exchange a single photon through a coherent Rabi oscillation. This process enables precise quantum-state engineering and manipulation of atoms and photons in a cavity, which…
A single quantum emitter can possess a very strong intrinsic nonlinearity, but its overall promise for nonlinear effects is hampered by the challenge of efficient coupling to incident photons. Common nonlinear optical materials, on the…
The quantum Rabi model, involving a two-level system and a bosonic field mode, is arguably the simplest and most fundamental model describing quantum light-matter interactions. Historically, due to the restricted parameter regimes of…
Resonance fluorescence from atomic systems consists of a single spectral peak that evolves into a Mollow triplet for a strong excitation field. Photons from different peaks of the triplet show distinct photon correlation that make the…
The atom-photon entanglement of dressed atom and its spontaneous emission in a Double-Lambda closed-loop atomic system is studied in multi-photon resonance condition. It is shown that, even in the absence of quantum interference due to the…
We propose a superconducting circuit to implement a two-photon quantum Rabi model in a solid-state device, where a qubit and a resonator are coupled by a two-photon interaction. We analyze the input-output relations for this circuit in the…
Tho-photon Rabi oscillations hold potential for quantum computing and quantum information processing, because during a Rabi cycle a pair of entangled photons may be created. We theoretically investigate the onset of this phenomenon in a…
The quantum Rabi model, which describes the interaction between a simplified atom and a mode of the electromagnetic field, is a cornerstone of modern quantum optics. One of the key assumptions of the model is that the `atom' is a perfect…
We analyze a photon transport through an 1D open waveguide side coupled to the $N$-photon microwave cavity with embedded artificial two- level atom (qubit). The qubit state is probed by a weak signal at the fundamental frequency of the…
Room temperature cavity quantum electrodynamics with molecular materials in optical cavities offers exciting prospects for controlling electronic, nuclear and photonic degrees of freedom for applications in physics, chemistry and materials…
The quantum Rabi model (QRM) is used to describe the light-matter interaction at the quantum level in Cavity Quantum Electrodynamics (Cavity QED). It consists of a two-level system (atom or qubit) coupled to a single-mode quantum field, and…
The prototypical system constituted by a two-level atom interacting with a quantized single-mode electromagnetic field is described by the quantum Rabi model (QRM). The QRM is potentially valid at any light-matter interaction regime,…
Multi-qubit quantum Rabi model, which is a fundamental model describing light-matter interaction, plays an important role in various physical systems. In this paper, we propose a theoretical method to simulate multi-qubit quantum Rabi model…
We demonstrate theoretically the parametric oscillator behavior of a two-level quantum system with broken inversion symmetry exposed to a strong electromagnetic field. A multitude of resonance frequencies and additional harmonics in the…
A cavity QED system is analyzed which duplicates the dynamics of a two-level atom in free space interacting exclusively with broadband squeezed light. We consider atoms in a three or four-level Lambda-configuration coupled to a high-finesse…
The strong coupling regime of photons and quantum materials inside optical cavities has emerged as a promising environment for manipulating states of matter with light. Here, in turn, we show that photons bear witness to cavity…
The precise control of light-matter interaction serves as a cornerstone for diverse quantum technologies, spanning from quantum computing to advanced atom optics. Typical experiments often feature multi-mode fields and require atoms with…
Optical microcavities and metallic nanostructures have been shown to significantly modulate the dynamics and spectroscopic response of molecular systems. We present a study of the nonlinear optics of a model consisting of $N$ anharmonic…
Coupling between molecules and vacuum photon fields inside an optical cavity has proven to be an effective way to engineer molecular properties, in particular reactivity. To ease the rationalization of cavity induced effects we introduce an…