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Quantum states with long-lived coherence are essential for quantum computation, simulation and metrology. The nuclear spin states of ultracold molecules prepared in the singlet rovibrational ground state are an excellent candidate for…

Molecules have vibrational, rotational, spin-orbit and hyperfine degrees of freedom or quantum states, each of which responds in a unique fashion to external electromagnetic radiation. The control over superpositions of these quantum states…

Quantum Physics · Physics 2024-04-29 Svetlana Kotochigova , Qingze Guan , Eite Tiesinga , Vito Scarola , Brian DeMarco , Bryce Gadway

Ultracold polar molecules uniquely combine a rich structure of long-lived internal states with access to controllable long-range, anisotropic dipole-dipole interactions. In particular, the rotational states of polar molecules confined in…

We explore the uses of ultracold molecules as a platform for future experiments in the field of quantum simulation, focusing on two molecular species, $^{40}$Ca$^{19}$F and $^{87}$Rb$^{133}$Cs. We report the development of coherent quantum…

Coherence, the stability of the relative phase between quantum states, lies at the heart of quantum mechanics. Applications such as precision measurement, interferometry, and quantum computation are enabled by physical systems that have…

Quantum Gases · Physics 2017-08-07 Jee Woo Park , Zoe Z. Yan , Huanqian Loh , Sebastian A. Will , Martin W. Zwierlein

Precision searches for time-reversal symmetry violating interactions in polar molecules are extremely sensitive probes of high energy physics beyond the Standard Model. To extend the reach of these probes into the PeV regime, long coherence…

Atomic Physics · Physics 2017-10-03 Ivan Kozyryev , Nicholas R. Hutzler

Qubit coherence times are critical to the performance of any robust quantum computing platform. For quantum information processing using arrays of polar molecules, a key performance parameter is the molecular rotational coherence time. We…

Ultracold molecules trapped in optical tweezers show great promise for the implementation of quantum technologies and precision measurements. We study a prototypical scenario where two interacting polar molecules placed in separate traps…

Polar molecules are desirable systems for quantum simulations and cold chemistry. Molecular ions are easily trapped, but a bias electric field applied to polarize them tends to accelerate them out of the trap. We present a general solution…

Ultracold polar molecules offer strong electric dipole moments and rich internal structure, which makes them ideal building blocks to explore exotic quantum matter, implement novel quantum information schemes, or test fundamental symmetries…

Polyatomic molecules provide complex internal structures that are ideal for applications in quantum information science, quantum simulation, and precision searches for physics beyond the Standard Model. A key feature of polyatomic molecules…

We construct quantum error-correcting codes that embed a finite-dimensional code space in the infinite-dimensional Hilbert state space of rotational states of a rigid body. These codes, which protect against both drift in the body's…

Quantum Physics · Physics 2020-09-09 Victor V. Albert , Jacob P. Covey , John Preskill

We suggest a protocol for the sympathetic cooling of a molecular asymmetric top rotor co-trapped with laser-cooled atomic ions, based on resonant coupling between the molecular ion's electric dipole moment and a common normal mode of the…

Quantum Physics · Physics 2026-02-04 Monika Leibscher , Alexander Blech , Christiane P. Koch

Rapid progress in cooling and trapping of molecules has enabled first experiments on high resolution spectroscopy of trapped diatomic molecules, promising unprecedented precision. Extending this work to polyatomic molecules provides unique…

Atomic Physics · Physics 2021-10-22 Alexander Prehn , Martin Ibrügger , Gerhard Rempe , Martin Zeppenfeld

We investigate the properties of two interacting ultracold polar molecules described as distinguishable quantum rigid rotors, trapped in a one-dimensional harmonic potential. The molecules interact via a multichannel two-body contact…

Atomic Physics · Physics 2018-07-03 Anna Dawid , Maciej Lewenstein , Michał Tomza

We demonstrate a collectively-encoded qubit based on a single Rydberg excitation stored in an ensemble of $N$ entangled atoms. Qubit rotations are performed by applying microwave fields that drive excitations between Rydberg states.…

Heavy polar molecules are sensitive probes of physics Beyond the Standard Model. However, uncontrolled external electromagnetic fields pose challenges to achieving precise and accurate measurements. Minimizing susceptibility to these fields…

The coherence of quantum systems is crucial to quantum information processing. While it has been demonstrated that superconducting qubits can process quantum information at microelectronics rates, it remains a challenge to preserve the…

The challenge of building a scalable quantum processor requires consolidation of the conflicting requirements of achieving coherent control and preservation of quantum coherence in a large scale quantum system. Moreover, the system should…

Quantum Physics · Physics 2007-05-23 A. Andre , D. DeMille , J. M. Doyle , M. D. Lukin , S. E. Maxwell , P. Rabl , R. Schoelkopf , P. Zoller

We present a rigorous theoretical study of low-temperature collisions of polyatomic molecular radicals with ^1S_0 atoms in the presence of an external magnetic field. Accurate quantum scattering calculations based on ab initio and scaled…

Atomic Physics · Physics 2011-03-07 T. V. Tscherbul , H-G. Yu , A. Dalgarno
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