English
Related papers

Related papers: Optical activity of chiral excitons

200 papers

Optical orientation of carrier spins by circularly polarized light is the basis of spin physics in semiconductors. Here, we demonstrate strong optical orientation of 85\%, approaching the ultimate limit of unity, for excitons in…

Chiral structures, breaking spatial inversion symmetry, exhibit non-zero chiroptical activity (COA) due to the interaction between their electric and magnetic responses under external electromagnetic fields, an effect that is otherwise…

Mesoscale and Nanoscale Physics · Physics 2023-09-06 Solmar Varela , Rafael Gutierrez , Gianaurelio Cuniberti , Ernesto Medina , Vladimiro Mujica

The helical distribution of the electronic density in chiral molecules, such as DNA and bacteriorhodopsin, has been suggested to induce a spin-orbit coupling interaction that may lead to the so-called chirality-induced spin selectivity…

Mesoscale and Nanoscale Physics · Physics 2020-01-01 Miguel A. Sierra , David Sanchez , Rafael Gutierrez , Gianaurelio Cuniberti , Francisco Dominguez-Adame , Elena Diaz

Coupling between light and material excitations underlies a wide range of optical phenomena. Polaritons are eigenstates of a coupled system with hybridized wave function. Owing to their hybrid composition, polaritons exhibit at the same…

Optics · Physics 2022-12-27 Denis G. Baranov , Christian Schäfer , Maxim V. Gorkunov

The spin properties of excitons and charge carriers in CsPbBr$_3$ lead halide perovskite crystals are investigated by spin-dependent light scattering in magnetic fields up to 10 T. Spin-flip Raman scattering spectra measured under resonant…

Controlling the spin degree of freedom of light at the microscale is crucial for advancing photonic information processing. Spin polarized light propagation, combined with strong optical nonlinearities, unlocks new functionalities in…

Other Condensed Matter · Physics 2025-10-20 Mateusz Kędziora , Andrzej Opala , Maciej Zaremba , Helgi Sigurðsson , Barbara Piętka

The exciton spin dynamics and polarization properties of the related emission are investigated in colloidal CdSe/CdS dot-in-rod (DiR) and spherical core/shell nanocrystal (NC) ensembles by magneto-optical photoluminescence (PL) spectroscopy…

Mesoscale and Nanoscale Physics · Physics 2015-06-23 B. Siebers , L. Biadala , D. R. Yakovlev , A. V. Rodina , T. Aubert , Z. Hens , M. Bayer

The Rashba effect, i.e., the splitting of electronic spin-polarized bands in the momentum space of a crystal with broken inversion symmetry, has enabled the realization of spin-orbitronic devices, in which spins are manipulated by…

The broken mirror symmetry in subwavelength photonic systems has manifested many interesting chiroptical effects such as optical rotation and circular dichroism. When such systems are placed periodically in a lattice form, in addition to…

Optics · Physics 2021-02-24 X. Guo , C. Liu , H. C. Ong

We derive exciton-spin interactions from a microscopic correlated model that captures important aspects of the physics of charge-transfer (CT) insulators to address magnetism associated with exciton creation. We present a minimal model…

Strongly Correlated Electrons · Physics 2023-11-16 Tatsuya Kaneko , Yuta Murakami , Denis Golež , Zhiyuan Sun , Andrew J. Millis

Mirror symmetry is among the most fundamental concepts of physics and its spontaneous breaking at the molecular level allows chiral molecules to exist in two enantiomers that are mirror images of each other. The majority of chiro-optical…

Optics · Physics 2021-09-29 Alessandro Ciattoni

We investigate a geometrically symmetric gold-silicon sphere heterodimer and reveal its extrinsic chiroptical response caused by the interaction with a substrate. The chiroptical response is obtained for oblique incidence owing to the…

Dark-field illumination is shown to make planar chiral nanoparticle arrangements exhibit circular dichroism in extinction analogous to true chiral scatterers. Circular dichrosim is experimentally observed at the maximum scattering of single…

Spin-orbit coupling (SOC) is responsible for a range of spintronic and topological processes in condensed matter. Here we show photonic analogs of SOCs in exciton-polaritons and their condensates in microcavities composed of birefringent…

Polariton states with high levels of chiral dissymmetry offer exciting prospects for quantum information, sensing, and lasing applications. Such dissymmetry must emanate from either the involved optical resonators or the quantum emitters.…

Chemical Physics · Physics 2022-09-28 Andrew H. Salij , Randall H. Goldsmith , Roel Tempelaar

We introduce and theoretically analyze the concept of manipulating optical chirality via strong coupling of the optical modes of chiral nanostructures with excitonic transitions in molecular layers or semiconductors. With chirality being…

The plasmonic chirality has drawn a lot of attention because of the tunable circular dichroism (CD) and the enhancement for the signal of chiral molecules. Different mechanisms have been proposed for explaining the plasmonic CD, however, a…

Mesoscale and Nanoscale Physics · Physics 2016-03-23 Li Hu , Xiaorui Tian , Yingzhou Huang , Xinqiang Wang , Yurui Fang

We develop a model of the coherent exciton spin-valley dynamics in two-dimensional transition metal dichalcogenides under elastic strain. The strain splits the exciton radiative doublet in linearly polarized states. Consequently, it induces…

Mesoscale and Nanoscale Physics · Physics 2023-01-04 M. M. Glazov

We have observed a large spin splitting between "spin" $+1$ and $-1$ heavy-hole excitons, having unbalanced populations, in undoped GaAs/AlAs quantum wells in the absence of any external magnetic field. Time-resolved photoluminescence…

Condensed Matter · Physics 2016-08-31 L. Vina , L. Munoz , E. Perez , J. Fernandez-Rossier , C. Tejedor , K. Ploog

We theoretically investigate exciton-polaritons in a two-dimensional (2D) semiconductor heterostructure, where a static magnetic field is applied perpendicular to the plane. To explore the interplay between magnetic field and a strong…

Mesoscale and Nanoscale Physics · Physics 2024-12-12 Emma Laird , Francesca M. Marchetti , Dmitry K. Efimkin , Meera M. Parish , Jesper Levinsen