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We investigate the lattice dynamics in the spin-1/2 frustrated kagome compound herbertsmithite ZnCu$_3$(OH)$_6$Cl$_2$ by a combination of infrared spectroscopy measurements and ab initio density functional theory calculations, and provide…

Strongly Correlated Electrons · Physics 2020-04-29 Ying Li , A. Pustogow , M. Bories , P. Puphal , C. Krellner , M. Dressel , Roser Valenti

Y-kapellasite (Y$_3$Cu$_9$(OH)$_{19}$Cl$_8$), which hosts an original anisotropic kagome sublattice, is a promising candidate for studying elusive and complex correlated physics. It exhibits a theoretically predicted in-plane $(1/3, 1/3)$…

We present the crystal structure and magnetic properties of Y$_{3}$Cu$_{9}$(OH)$_{19}$Cl$_{8}$, a stoichiometric frustrated quantum spin system with slightly distorted kagome layers. Single crystals of Y$_{3}$Cu$_{9}$(OH)$_{19}$Cl$_{8}$…

It is predicted that strongly interacting spins on a frustrated lattice may lead to a quantum disordered ground state or even form a quantum spin liquid with exotic low-energy excitations. However, a thorough tuning of the frustration…

Strongly Correlated Electrons · Physics 2024-01-08 Jierong Wang , Y. -S. Su , M. Spitaler , P. Puphal , C. Krellner , S. E. Brown , A. Pustogow

The kapellasite family $A$Cu$_3$(OH)$_{6+x}$(Cl,Br)$_{3-x}$ forms a series of compounds, wherein the chemical pressure realized by the $A-$site cation tunes the spin exchange in the frustrated distorted kagome lattice. Via hydrothermal…

Strongly Correlated Electrons · Physics 2025-08-12 Jonas Andreas Krieger , Thomas James Hicken , Hubertus Luetkens , Reinhard K. Kremer , Pascal Puphal

The static and dynamic magnetic properties of the Nd$_3$Ga$_5$SiO$_{14}$ compound, which appears as the first materialization of a rare-earth kagome-type lattice, were re-examined, owing to contradictory results in the previous studies.…

Experimental studies of high-purity kagome-lattice antiferromagnets (KAFM) are of great importance in attempting to better understand the predicted enigmatic quantum spin-liquid ground state of the KAFM model. However, realizations of this…

Strongly Correlated Electrons · Physics 2021-06-02 W. Sun , T. Arh , M. Gomilšek , P. Koželj , S. Vrtnik , M. Herak , J. -X. Mi , A. Zorko

We present a Raman scattering study of Ca$_2$RuO$_4$, in which we investigate the temperature-dependence of the lattice dynamics and the electron-phonon interaction below the metal-insulator transition temperature ({\it T}$_{\rm MI}$).…

Strongly Correlated Electrons · Physics 2009-11-11 H. Rho , S. L. Cooper , S. Nakatsuji , H. Fukazawa , Y. Maeno

One of the key questions concerning frustrated lattices that has lately emerged is the role of disorder in inducing spin-liquid-like properties. In this context, the quantum kagome antiferromagnets YCu$_3$(OH)$_6$Cl$_3$, which has been…

Strongly Correlated Electrons · Physics 2019-07-02 A. Zorko , M. Pregelj , M. Klanjšek , M. Gomilšek , Z. Jagličić , J. S. Lord , J. A. T. Verezhak , T. Shang , W. Sun , J. -X. Mi

We report the local probe investigation of a frustrated antiferromagnet Pr$_3$BWO$_9$ with the distorted kagome lattice. Absence of magnetic order or spin freezing is indicated by the spectral analysis down to 0.3 K and specific heat…

Strongly Correlated Electrons · Physics 2021-11-02 K. Y. Zeng , F. Y. Song , Z. M. Tian , Qiao Chen , Shun Wang , Bo Liu , Shiliang Li , L. S. Ling , W. Tong , Long Ma , Li Pi

Results of high resolution x-ray diffraction experiments are presented for single crystals of the spin gap compound BaCuSi$_2$O$_6$ in the temperature range from 16 to 300 K. The data show clear evidence of a transition from the room…

Strongly Correlated Electrons · Physics 2009-11-11 E. C. Samulon , Z. Islam , S. E. Sebastian , P. B. Brooks , M. K. McCourt , J. Ilavsky , I. R. Fisher

The collective behavior of interacting magnetic moments can be strongly influenced by the topology of the underlying lattice. In geometrically frustrated spin systems, interesting chiral correlations may develop that are related to the spin…

Strongly Correlated Electrons · Physics 2007-05-23 D. Grohol , K. Matan , J. H. Cho , S. -H. Lee , J. W. Lynn , D. G. Nocera , Y. S. Lee

Y3Cu9(OH)19Cl8 realizes an original anisotropic kagome model hosting a rich magnetic phase diagram [M. Hering et al, npj Computational Materials 8, 1 (2022)]. We present an improved synthesis of large phase-pure single crystals via an…

We present a systematic study of the structure and lattice dynamics at room temperature, and the phonon behavior at low temperatures in orthorhombic Gd$_{1-x}$Y$_{x}$MnO$_{3}$ manganites, with 0 $\leq$ x $\leq$ 0.4, using powder x-ray…

Strongly Correlated Electrons · Physics 2014-12-31 R. Vilarinho , E. C. Queirós , A. Almeida , P. B. Tavares , J. Agostinho Moreira

Frustrated lattices1-3, characterized by minor breakdown in local order in an otherwise periodic lattice, lead to simultaneous possibilities of several ground states which can trigger unique physical properties, in condensed matter systems.…

Mesoscale and Nanoscale Physics · Physics 2014-04-07 Satyendra Prakash Pal , P. Sen

The Kagome lattice is an important fundamental structure in condensed matter physics for investigating the interplay of electron correlation, topology, and frustrated magnetism. Recent work on Kagome metals in the AV3Sb5 (A = K, Rb, Cs)…

We investigate the interplay between lattice symmetry, phonons, and magnetism in the quasi-one-dimensional ladder compound BaFe$_2$S$_3$ by combining polarized synchrotron infrared spectroscopy, hybrid-functional density functional theory…

Strongly Correlated Electrons · Physics 2026-03-20 Y. Oubaid , S. Deng , NS. Dhami , M. Verseils , D. Bounoua , A. Forget , D. Colson , P. Foury-Leylekian , M. B. Lepetit , V. Balédent

Ultrasound velocity measurements were performed on a single crystal of spin-frustrated ferrite spinel ZnFe$_2$O$_4$ from 300 K down to 2 K. In this cubic crystal, all the symmetrically-independent elastic moduli exhibit softening with a…

Strongly Correlated Electrons · Physics 2015-11-26 Tadataka Watanabe , Shota Takita , Keisuke Tomiyasu , Kazuya Kamazawa

Nickel orthoborate $Ni_{3}(BO_{3})_{2}$ having a complex orthorhombic structure $P_{nnm}$ (#58, Z=2) of the kotoite type is known for quite a long time as an antiferromagnetic material below $T_{N}$ = 46 K, but up to now its physical…

We report a detailed study of the magnetic properties, critical analysis of magnetization, and magnetocaloric effect of a spin-$2$ kagome lattice YCa$_3$(MnO)$_3$(BO$_3$)$_4$. The experiments are complemented by the density functional band…

Materials Science · Physics 2025-07-29 A. Choudhary , A. Magar , S. Ghosh , S. Kanungo , R. Nath
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