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The liquid, plastic crystalline and ordered crystalline phases of CBr$_4$ were studied using neutron powder diffraction. The measured total scattering differential cross-sections were modelled by Reverse Monte Carlo simulation techniques…

Chemical Physics · Physics 2010-04-06 László Temleitner , László Pusztai

For particles confined to two dimensions, any curvature of the surface affects the structural, kinetic and thermodynamic properties of the system. If the curvature is non-uniform, an even richer range of behaviours can emerge. Using a…

Soft Condensed Matter · Physics 2020-08-10 Jack O. Law , Jacob M. Dean , Mark A. Miller , Halim Kusumaatmaja

Entropic self-assembly is governed by the shape of the constituent particles, yet a priori prediction of crystal structures from particle shape alone is non-trivial for anything but the simplest of space-filling shapes. At the same time,…

Soft Condensed Matter · Physics 2023-05-16 Philipp W. A. Schönhöfer , Kai Sun , Xiaoming Mao , Sharon C. Glotzer

We investigate the phase behavior of a system of hard equilateral and right-angled triangles in two dimensions using Monte Carlo simulations. Hard equilateral triangles undergo a continuous isotropic-triatic liquid crystal phase transition…

Soft Condensed Matter · Physics 2015-04-14 Anjan P. Gantapara , Weikai Qi , Marjolein Dijkstra

Progressive deformation of upper mantle rocks via dislocation creep causes their constituent crystals to take on a non-random orientation distribution (crystallographic preferred orientation or CPO) whose observable signatures include…

We used the Density Functional formalism, in particular the Scaled Particle Theory, applied to a length-polydisperse hard-rectangular fluid to study its phase behavior as a function of the mean particle aspect ratio ($\kappa_0$) and…

Soft Condensed Matter · Physics 2017-05-23 Ariel Diaz-De Armas , Yuri Martinez-Raton

Colloidal crystal structures with complexity and diversity rivaling atomic and molecular crystals have been predicted and obtained for hard particles by entropy maximization. However, so far homochiral colloidal crystals, which are…

Soft Condensed Matter · Physics 2015-10-13 Pablo F. Damasceno , Andrew S. Karas , Benjamin A. Schultz , Michael Engel , Sharon C. Glotzer

Using the classical density functional theory of freezing and Monte Carlo computer simulations, we explore the liquid-crystalline phase behavior of hard rectangles on flat and cylindrical manifolds. Moreover, we study the effect of a static…

Soft Condensed Matter · Physics 2018-02-19 Christoph E. Sitta , Frank Smallenburg , Raphael Wittkowski , Hartmut Löwen

We study mutual alignment and interactions between colloidal particles of dissimilar shapes and dimensions when dispersed in a nematic host fluid. Convex pentagonal and concave starfruit-shaped nanoprisms and microspheres induce dipolar or…

Soft Condensed Matter · Physics 2016-12-28 Bohdan Senyuk , Ivan I. Smalyukh

We use a series of molecular dynamics simulations, and analytical theory, to demonstrate that a system of hard spheres confined to a narrow cylindrical channel exhibits a continuous phase transition from an isotropic fluid at low densities,…

Soft Condensed Matter · Physics 2014-09-18 Mahdi Zaeifi Yamchi , Richard K. Bowles

We investigate the isotropic-to-nematic phase transition in systems of hard helical particles, using Onsager theory and Monte Carlo computer simulations. Motivation of this work resides in the ubiquity of the helical shape motif in many…

Soft Condensed Matter · Physics 2013-05-01 Elisa Frezza , Alberta Ferrarini , Hima Bindu Kolli , Achille Giacometti , Giorgio Cinacchi

It has been a long-standing materials science challenge to establish structure-property relations in amorphous solids. Here we introduce a rotation-variant local structure representation that enables different predictions for different…

Materials Science · Physics 2022-03-15 Zhao Fan , Evan Ma

Colloidal particles can spontaneously self-assemble into ordered structures, which not only can manipulate the propagation of light, but also vibration or phonons. Using Monte Carlo simulation, we study the self-assembly of perfectly…

Soft Condensed Matter · Physics 2024-03-11 Ji-Dong Hu , Ting Wang , Qun-Li Lei , Yu-qiang Ma

Effects of three-point direct correlation on properties of the phase field crystal (PFC) modeling are examined, for the control of various ordered and disordered phases and their coexistence in both three-dimensional and two-dimensional…

Materials Science · Physics 2022-04-15 Zi-Le Wang , Zhirong Liu , Wenhui Duan , Zhi-Feng Huang

Crystallization of the amorphous phases into metastable crystals plays a fundamental role in the formation of new matter, from geological to biological processes in nature to synthesis and development of new materials in the laboratory.…

Materials Science · Physics 2023-10-03 Muratahan Aykol , Amil Merchant , Simon Batzner , Jennifer N. Wei , Ekin Dogus Cubuk

We review the impact of tetrahedral order on the macroscopic dynamics of bent-core liquid crystals. We discuss tetrahedral order comparing with other types of orientational order, like nematic, polar nematic, polar smectic, and active polar…

Soft Condensed Matter · Physics 2016-10-21 H. Pleiner , H. R. Brand

Sought-after ordered structures of mixtures of hard anisotropic nanoparticles can often be thermodynamically unfavorable due to the components' geometric incompatibility to densely pack into regular lattices. A simple compatibilization rule…

Soft Condensed Matter · Physics 2014-10-22 Mihir R. Khadilkar , Fernando A. Escobedo

We propose a simple microscopic model of molecular dynamics simulation to study orientational glass in three dimensions. We present simulation results for mixtures of mildly anisotropic particles and spherical impurities. We realize fcc…

Soft Condensed Matter · Physics 2012-10-29 Kyohei Takae , Akira Onuki

We investigate the orientational order of transverse polarization vectors of long, stiff polymer molecules and their coupling to bond orientational and positional order in high density mesophases. Homogeneous ordering of transverse…

Soft Condensed Matter · Physics 2009-11-07 V. Lorman , R. Podgornik , B. Žekš

We numerically study structural properties of mechanically stable packings of hard spheres (HS), in a wide range of packing fractions $0.53 \le \phi \le 0.72$. Detailed structural information is obtained from the analysis of orientational…

Soft Condensed Matter · Physics 2014-07-30 Boris A. Klumov , Yuliang Jin , Hernan A. Makse