Related papers: Chiral Phonons in 2D Halide Perovskites
Halide perovskites emerged as a revolutionary family of high-quality semiconductors for solar energy harvesting and energy-efficient lighting. There is mounting evidence that the exceptional optoelectronic properties of these materials…
We experimentally study magnetic resonances in the helical and conical magnetic phases of the chiral magnetic insulator Cu$_2$OSeO$_3$ at the temperature $T$=5 K. Using a broadband microwave spectroscopy technique based on vector network…
Charge transport is crucial to the performance of hybrid halide perovskite solar cells. A theoretical model based on large polarons is proposed to elucidate charge transport properties in the perovskites. Critical new physical insights are…
Realizing semiconductors with high symmetry of their crystallographic structures has been a virtue of inorganic materials and has resulted in novel physical behaviors. In contrast, hybrid (organic and inorganic) crystals such as…
Chiral crystals have recently garnered significant interest in condensed matter physics due to their unique electronic and optical properties. In this paper, we explore the connection between the chirality of crystal structures and the…
We present a computational investigation, in conjunction with synthesis and experimental characterization, into the structural, electronic, and optical properties of layered 2D organic lead bromide perovskites. We contrast materials based…
A pure spin current formed by opposite spins moving in opposite directions is a rank-2 axial tensor which breaks the inversion symmetry. Thus a spin current has a second-order optical susceptibility, with unique polarization-dependence…
Hexagonal and kagome lattices exhibit extraordinary electronic properties. It is a natural consequence of additional discrete degree of freedom associated with a valley or the occurence of electronic flat-bands. Combination of both types of…
We have studied the magnetic response of transverse optical phonons in Pb$_{1-x}$Sn$_{x}$Te films. Polarization-dependent terahertz magnetospectroscopy measurements revealed Zeeman splittings and diamagnetic shifts, demonstrating that these…
Two-dimensional (2D) halide perovskites offer a unique platform to investigate the ground-state of materials possessing significant anharmonicity. In contrast to three-dimensional perovskites, their 2D counterparts offer substantially fewer…
We present a microscopic theory of the inverse chiral phonon Zeeman effect in noncentrosymmetric crystals. Within micropolar elasticity, coupled translational displacements and microrotations give rise to intrinsically chiral phonons, which…
Understanding the interplay of strong correlation and temperature in nodal-line semimetals can offer novel ways to control spin currents. Here we consider the 3d-5d double-perovskite Ba$_{2}$CoWO$_{6}$, which features…
In recent years, metal halide perovskites have generated tremendous interest for optoelectronic applications and their underlying fundamental properties. Due to the large electron-phonon coupling characteristic of soft lattices,…
The generation, manipulation and detection of spin-polarized electrons in nanostructures define the main challenges of spin-based electronics[1]. Amongst the different approaches for spin generation and manipulation, spin-orbit coupling,…
We demonstrate through first-principles calculations applied to the K$_{3}$NiO$_{2}$ crystal that a structural phase transition from an achiral to a chiral phase can be mediated by a degenerate soft phonon mode and controlled by pressure…
Hybrid organic-inorganic semiconductors feature complex lattice dynamics due to the ionic character of the crystal and the softness arising from non-covalent bonds between molecular moieties and the inorganic network. Here we establish that…
Optically active defects often play a crucial role in governing the light emission as well as the electronic properties of materials. Moreover, defect-mediated states in the mid-gap region can trap electrons, thus opening a path for the…
In this paper, the chiral Hall effect of strained Weyl semimetals without any external magnetic field is proposed. Electron-phonon coupling emerges in the low-energy fermionic sector through a pseudogauge potential. We show that, by using…
Two-dimensional (2D) organic-inorganic hybrid perovskites emerged as a versatile platform for light-emitting and photovol-taic applications due to their unique structural design and chemical flexibility. Their properties depend heavily on…
Chiral functionalities exhibited by systems lacking any mirror symmetry encompass natural optical activity, magnetochiral effect, diagonal current-induced magnetization, chirality-selective spin-polarized current of charged electrons or…