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We report a room-temperature optical reflectivity study performed on [112]-oriented Cd$_3$As$_2$ single crystals over a broad energy range under external pressure up to 10 GPa. The abrupt drop of the band dispersion parameter…

Materials Science · Physics 2018-05-23 E. Uykur , R. Sankar , D. Schmitz , C. A. Kuntscher

Revealing the ultrafast dynamics of three-dimensional (3D) Dirac fermions upon photoexcitation is critical for both fundamental science and device applications. So far, how the cooling of 3D Dirac fermions differs from that of…

Mesoscale and Nanoscale Physics · Physics 2022-02-16 Changhua Bao , Qian Li , Sheng Xu , Shaohua Zhou , Xiang-Yu Zeng , Haoyuan Zhong , Qixuan Gao , Laipeng Luo , Dong Sun , Tian-Long Xia , Shuyun Zhou

We report ultrafast transient-grating measurements of crystals of the three-dimensional Dirac semimetal cadmium arsenide, Cd3As2, at both room temperature and 80 K. After photoexcitation with 1.5-eV photons, charge-carriers relax by two…

Ultrafast time-resolved differential reflectivity of Bi2Se3 crystals is studied using optical pump-probe spectroscopy. Three distinct relaxation processes are found to contribute to the initial transient reflectivity changes. The deduced…

Materials Science · Physics 2010-11-09 J. Qi , X. Chen , W. Yu , P. Cadden-Zimansky , D. Smirnov , N. H. Tolk , I. Miotkowski , H. Cao , Y. P. Chen , Y. Wu , S. Qiao , Z. Jiang

The topological three-dimensional Dirac semimetal Cd3As2 has drawn great attention for the novel physics and promising applications in optoelectronic devices operating in the infrared and THz regimes. Among the extensive studies in the past…

Strongly Correlated Electrons · Physics 2022-06-17 Wenjie Zhang , Yunkun Yang , Peng Suo , Kaiwen Sun , Jun Peng , Xian Lin , Faxian Xiu , Guohong Ma

Pulsed lasers operating in the 2-5 {\mu}m band are important for a wide range of applications in sensing, spectroscopy, imaging and communications. Despite recent advances with mid-infrared gain media, the lack of a capable pulse generation…

Using atomic-force microscopy (AFM) and wide-band (0.02-8.5 eV) spectroscopic ellipsometry techniques we investigated morphology and optical properties of Cd3As2 films grown by non-reactive rf magnetron sputtering on two types of oriented…

Materials Science · Physics 2023-01-16 Natalia Kovaleva , Ladislav Fekete , Dagmar Chvostova , Andrei Muratov

Three dimensional (3D) Dirac semimetals are 3D analogue of graphene, which display Dirac points with linear dispersion in k-space, stabilized by crystal symmetry. Cd3As2 and Na3Bi were predicted to be 3D Dirac semimetals and were…

Materials Science · Physics 2015-08-28 Zhi-Gang Chen , Cheng Zhang , Yichao Zou , Enze Zhang , Lei Yang , Faxian Xiu , Jin Zou

The recently discovered Dirac and Weyl semimetals are new members of topological materials. Starting from them, topological superconductivity may be achieved, e.g. by carrier doping or applying pressure. Here we report high-pressure…

Superconductivity · Physics 2016-09-27 L. P. He , Y. T. Jia , S. J. Zhang , X. C. Hong , C. Q. Jin , S. Y. Li

The electromagnetic response of Dirac semimetals in the infrared and terahertz frequency ranges is attracting growing interest for potential applications in optoelectronics and nonlinear optics. The interplay between the free-carrier…

Three-dimensional topological Dirac semimetals have hitherto stimulated unprecedented research interests as a new class of quantum materials. Breaking certain types of symmetries has been proposed to enable the manipulation of Dirac…

Three-dimensional (3D) semimetals have been predicted and demonstrated to have a wide variety of interesting properties associated with its linear energy dispersion. In analogy to two-dimensional (2D) Dirac semimetals, such as graphene,…

The three dimensional (3D) Dirac semimetal, which has been predicted theoretically, is a new electronic state of matter. It can be viewed as 3D generalization of graphene, with a unique electronic structure in which conduction and valence…

Mesoscale and Nanoscale Physics · Physics 2014-07-10 Sergey Borisenko , Quinn Gibson , Danil Evtushinsky , Volodymyr Zabolotnyy , Bernd Buechner , Robert J. Cava

Raman scattering in the three-dimensional Dirac semimetal Cd3As2 shows an intricate interplay of electronic and phonon degrees of freedom. We observe resonant phonon scattering due to interband transitions, an anomalous anharmonicity of…

Materials Science · Physics 2017-07-05 A. Sharafeev , V. Gnezdilov , R. Sankar , F. C. Chou , P. Lemmens

Cadmium arsenide Cd$_3$As$_2$ hosts massless Dirac electrons in its ambient-conditions tetragonal phase. We report X-ray diffraction and electrical resistivity measurements of Cd$_3$As$_2$ upon cycling pressure beyond the critical pressure…

We have extended the range of the high-pressure optical spectroscopy to the far-infrared region keeping the accuracy of ambient-pressure experiments. The newly-developed method offers a powerful tool for the study of pressure-induced phase…

Strongly Correlated Electrons · Physics 2014-01-15 I. Kezsmarki , R. Gaal , C. C. Homes , B. Sipos , H. Berger , S. Bordacs , G. Mihaly , L. Forro

We report the first observation of a pressure-induced breakdown of the 3D-DSM state in Cd3As2, evidenced by a series of in-situ high-pressure synchrotron X-ray diffraction (XRD) and single crystal transport measurements. We find that Cd3As2…

Time-reversal invariance and inversion symmetry are responsible for the topological band structure in Dirac semimetals. These symmetries can be broken by applying an external magnetic or electric field, resulting in fundamental changes to…

Mesoscale and Nanoscale Physics · Physics 2023-06-28 Run Xiao , Saurav Islam , Wilson Yanez , Yongxi Ou , Nitin Samarth , Haiwen Liu , X. C. Xie , Juan Chamorro , Tyrel M. McQueen

We study the all-optical switching behavior of one-dimensional metal-dielectric photonic crystals due to the nonlinearity of the free metal electrons. A polychromatic pump-probe setup is used to determine the wavelength and pump intensity…

Other Condensed Matter · Physics 2015-05-13 Tolga Ergin , Tilman Höner zu Siederdissen , Harald Giessen , Markus Lippitz

We have used a combination of linear response time-domain THz spectroscopy (TDTS) and high-field non-linear THz spectroscopy to separately probe the electronic momentum and energy relaxation rates respectively of the Dirac semimetal…

Strongly Correlated Electrons · Physics 2024-08-19 Rishi Bhandia , David Barbalas , Run Xiao , Juan R. Chamorro , Tanya Berry , Tyrel M. McQueen , Nitin Samarth , N. P. Armitage
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